The soft glassy rheology (SGR) model has successfully described the time dependent simple shear rheology of a broad class of complex fluids including foams, concentrated emulsions, colloidal glasses, and solvent-free nanoparticle-organic hybrid materials (NOHMs). The model considers a distribution of mesoscopic fluid elements that hop from trap to trap at a rate which is enhanced by the work done to strain the fluid element. While an SGR fluid has a broad exponential distribution of trap energies, the rheology of NOHMs is better described by a narrower energy distribution and we consider both types of trap energy distributions in this study. We introduce a tensorial version of these models with a hopping rate that depends on the orientation of the element relative to the mean stress field, allowing a range of relative strengths of the extensional and simple shear responses of the fluid. As an application of these models we consider the flow of a soft glassy material through a dilute fixed bed of fibers. The dilute fixed bed exhibits a range of local linear flows which alternate in a chaotic manner with time in a Lagrangian reference frame. It is amenable to an analytical treatment and has been used to characterize the strong flow response of many complex fluids including fiber suspensions, dilute polymer solutions and emulsions. We show that the accumulated strain in the fluid elements has an abrupt nonlinear growth at a Deborah number of order one in a manner similar to that observed for polymer solutions. The exponential dependence of the hopping rate on strain leads to a fluid element deformation that grows logarithmically with Deborah number at high Deborah numbers. SGR fluids having a broad range of trap energies flowing through fixed beds can exhibit a range of rheological behaviors at small Deborah numbers ranging from a yield stress, to a power law response and finally to Newtonian behavior.
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November 2015
Research Article|
November 01 2015
A model for complex flows of soft glassy materials with application to flows through fixed fiber beds
Arijit Sarkar;
Arijit Sarkar
School of Chemical and Biomolecular Engineering,
Cornell University
, 120 Olin Hall, Ithaca, New York 14853-5201
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Donald L. Koch
Donald L. Koch
a)
School of Chemical and Biomolecular Engineering,
Cornell University
, 120 Olin Hall, Ithaca, New York 14853-5201
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a)
Author to whom correspondence should be addressed; electronic mail: [email protected]
J. Rheol. 59, 1487–1505 (2015)
Article history
Received:
March 24 2015
Accepted:
October 03 2015
Citation
Arijit Sarkar, Donald L. Koch; A model for complex flows of soft glassy materials with application to flows through fixed fiber beds. J. Rheol. 1 November 2015; 59 (6): 1487–1505. https://doi.org/10.1122/1.4934367
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