To reduce carbon emission and satisfy strict regulations in an automotive sector, hybrid-electric vehicles have been developed using lithium-ion battery technology due to its superior performance. However, the relatively expensive price of the vehicles is still a critical issue. One reason is high manufacturing cost, especially the cutting process. Currently, the anode cutting process utilizes rotary knives and dies. These require relatively expensive tooling that degrades over time. The degradation results in poor cut quality. This cut quality leads to short circuits and significant heat generation during battery operation. Furthermore, a redesign of mechanical cutting processes demands extra expense due to various cell specifications. Laser cutting provides faster cutting speed, good consistent cut quality, and the possibility of flexible design due to its fast processing time, high precision, and flexible range of laser power. However, these advantages cannot be fully utilized without understanding the underlying physics. A 3D self-consistent mathematical model of anode laser cutting is developed including multiple physical phenomena. This study analyzes temperature and composition distributions, melt pool geometry, and melt pool flow around the interface between copper and graphite. In addition, the effect of these physical properties on the cut quality of an anode is discussed.

1.
Alamgir
M
,
Sastry
AM
. Efficient Batteries for Transportation Applications.
SAE Convergence
.
Detroit, MI
2008
.
2.
Winter
M
,
Brodd
RJ
.
What are batteries, fuel cells, and supercapacitors?
Chemical Reviews.
2004
;
104
:
4245
69
.
3.
Communications W
. Lithium Battery Manufacturing.
4.
Herfurth
HJ
,
Patwa
R
,
Pantsar
H
,
Heinemann
S
,
Newaz
G.
LASER PROCESSING FOR ALTERNATIVES ENERGY DEVICES: ADVANCED BATTERY AND FUEL CELL APPLICATIONS
.
Proceedings of the ICALEO
.
Temecula, CA USA
2008
.
5.
Herfurth
HJ
,
Patwa
R
,
Pantsar
H.
Laser Cutting of Electrodes for Advanced Batteries
.
Proceedings of the LPM
.
Germany
2010
.
6.
Patwa
R
,
Herfurth
HJ
,
Pantsar
H
,
Heinemann
S
,
Mazumder
J
,
Lee
D.
High speed laser cutting of electrodes for advanced batteries
.
Proceedings of the ICALEO
.
Anaheim, CA
2010
.
7.
Steen
WM
,
Mazumder
J
, SpringerLink (Online service).
Laser Material Processing
. 4th Edition. ed.
London
:
Springer-Verlag London
;
2010
.
8.
Broussely
M
,
Biensan
P
,
Simon
B.
Lithium insertion into host materials: the key to success for Li ion batteries
.
Electrochimica Acta.
1999
;
45
:
3
22
.
9.
Wang
Q
,
Zhang
W
,
Yang
Z
,
Weng
S
,
Jin
Z.
Solvothermal synthesis of hierarchical LiFePO(4) microflowers as cathode materials for lithium ion batteries
.
Journal of Power Sources.
2011
;
196
:
10176
82
.
10.
Muraliganth
T
,
Murugan
AV
,
Manthiram
A.
Nanoscale networking of LiFePO(4) nanorods synthesized by a microwave-solvothermal route with carbon nanotubes for lithium ion batteries
.
Journal of Materials Chemistry.
2008
;
18
:
5661
8
.
11.
Amin
R
,
Balaya
P
,
Maier
J.
Anisotropy of electronic and ionic transport in LiFePO4 single crystals
.
Electrochemical and Solid State Letters.
2007
;
10
:
A13
A6
.
12.
Kim
H
,
Cho
J.
Superior Lithium Electroactive Mesoporous Si@Carbon Core-Shell Nanowires for Lithium Battery Anode Material
.
Nano Letters
.
2008
;
8
:
3688
91
.
13.
Nguyen
CC
,
Song
S-W.
Characterization of SEI layer formed on high performance Si-Cu anode in ionic liquid battery electrolyte
.
Electrochemistry Communications.
2010
;
12
:
1593
5
.
14.
Guo
H
,
Zhao
H
,
Yin
C
,
Qiu
W.
Si/SnSb alloy composite as high capacity anode materials for Li-ion batteries
.
Journal of Alloys and Compounds.
2006
;
426
:
277
80
.
15.
Obrovac
MN
,
Christensen
L.
Structural changes in silicon anodes during lithium insertion/extraction
.
Electrochemical and Solid State Letters.
2004
;
7
:
A93
A6
.
16.
Zhang
T
,
Gao
J
,
Fu
LJ
,
Yang
LC
,
Wu
YP
,
Wu
HQ
.
Natural graphite coated by Si nanoparticles as anode materials for lithium ion batteries
.
Journal of Materials Chemistry
.
2007
;
17
:
1321
5
.
17.
Luetke
M
,
Franke
V
,
Techel
A
,
Himmer
T
,
Klotzbach
U
,
Wetzig
A
, et al
A Comparative Study on Cutting Electrodes for Batteries with Lasers
.
Physics Procedia.
2011
;
12
:
286
91
.
18.
Lee
D
,
Mazumder
J.
The Numerical Studies of the Laser Processing Parameters on Copper and Aluminum during Laser Cutting
.
Proceedings of the ICALEO
.
Anaheim, California
:
Laser institute of America
;
2010
.
19.
Lee
D
,
Mazumder
J.
Numerical Studies of Laser Cutting on an Active Electrode Material for Lithiumion Batteries
.
Proceedings of the ICALEO
.
Orlando, Florida
:
Laser institute of America
;
2011
.
20.
Lee
D
,
Patwa
R
,
Herfurth
H
,
Mazumder
J.
Computational and experimental studies of laser cutting of the current collectors for lithium-ion batteries
.
Journal of Power Sources.
2012
;
210
:
327
38
.
21.
Ki
H
,
Mohanty
PS
,
Mazumder
J.
A numerical method for multiphase incompressible thermal flows with solid-liquid and liquid-vapor phase transformations
.
Numerical Heat Transfer Part B-Fundamentals.
2005
;
48
:
125
45
.
22.
Bennon
WD
,
Incropera
FP
.
A CONTINUUM MODEL FOR MOMENTUM, HEAT AND SPECIES TRANSPORT IN BINARY SOLID LIQUID-PHASE CHANGE SYSTEMS .1. MODEL FORMULATION
.
International Journal of Heat and Mass Transfer.
1987
;
30
:
2161
70
.
23.
Asai
S
,
Muchi
I.
Theoretical analysis and model experiments on the formation mechanism of channel teyp segregation
.
Trasaction ISIJ.
1978
;
18
:
90
8
.
24.
Bennon
WD
,
Incropera
FP
.
A continuum model for momentum, heat and species transport in binary solid-liquid phase change systems--I. Model formulation
.
International Journal of Heat and Mass Transfer.
1987
;
30
:
2161
70
.
25.
Ki
H.
Modeling and measurement of processes with liquid-vapor interface created by high power density lasers
2001
.
26.
Knight
CJ
.
THEORETICAL MODELING OF RAPID SURFACE VAPORIZATION WITH BACK PRESSURE
.
Aiaa Journal
.
1979
;
17
:
519
23
.
27.
Ytrehus
T
,
Ostmo
S.
Kinetic theory approach to interphase processes
.
International Journal of Multiphase Flow.
1996
;
22
:
133
55
.
28.
Ki
H
,
Mohanty
PS
,
Mazumder
J.
Modelling of high-density laser-material interaction using fast level set method
.
Journal of Physics D-Applied Physics
.
2001
;
34
:
364
72
.
29.
Ki
H
,
Mohanty
PS
,
Mazumder
J.
Multiple reflection and its influence on keyhole evolution
.
20th Icaleo 2001, Vols 92 & 93, Congress Proceedings
.
2001
:
933
42
.
30.
Fabbro
R
,
Chouf
K.
Keyhole modeling during laser welding
.
Journal of Applied Physics.
2000
;
87
:
4075
83
.
31.
Patankar
SV
.
Numerical heat transfer and fluid flow
.
Washington New York
:
Hemisphere Pub. Corp.; McGraw-Hill
;
1980
.
32.
Sethian
JA
.
Level set methods and fast marching methods : evolving interfaces in computational geometry, fluid mechanics, computer vision, and materials science
. 2nd ed.
Cambridge, U.K.; New York
:
Cambridge University Press
;
1999
.
This content is only available via PDF.
You do not currently have access to this content.