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The Ever-Expanding Optics of Single-Molecules and Nanoparticles

Our traditional approach of understanding the properties of an individual object is often based on an extrapolation from the properties of an ensemble. This approach naturally arises from the ease to access ensembles in an experiment. With new experimental developments this extrapolation appeared to be an oversimplification and with the advent of single-molecule optics around 1990, this idea of homogeneity and isotropy at the smallest scales finally disappeared. The world has become more interesting at the smallest scales and better understood since then and the field of single-molecule optics has rapidly evolved. In the early 1990s pioneering experiments still targeted single molecules as objects of interest themselves. This seemingly small step has revolutionized biology, sparked a new era for optical microscopy and quantum optics and provided an indispensable tool for materials science and physics. The ability to optically image, study and therefore also to manipulate single molecules created new opportunities for uncovering previously unknown phenomena. In the 2000s this field has spread out to many other systems and nanoscale objects, that can now be accessed at the single-particle level exploring new physical principles directly on the most fundamental, single-object level.

This virtual special issue attempts to attract a collection of works that will represent an adequate sampling snapshot for the expanding creativity that shares a single conceptual spark made possible by the pioneering experiments some three decades ago: think single-molecule.

To represent the developments, we suggest contributions from the following fields:

1. Photothermal phenomena
2. Quantum optics
3. Plasmonics
4. Single-molecule spectroscopy
5. Single-particle spectroscopy
6. Single-molecule biophysics and enzymology
7. Laser tweezers
8. Molecular imaging

Guest Editors: Frank Cichos, Peter Zijlstra, Tie Xia, and Haw Yang with JCP Editors Emily Weiss, Jennifer Ogilvie, Lasse Jensen, John Straub, and Editor-in-Chief Tim Lian

Subhasis Adhikari; Michel Orrit
Christine A. Carlson; Xavier S. Udad; Quintus Owen; Alaknanda P. Amin-Patel; Woo-Jin Chang; Jörg C. Woehl
Thomas Liu; Baptiste Carles; Christine Elias; Claire Tonnelé; Daniel Medina-Lopez; Akimitsu Narita; Yannick Chassagneux; Christophe Voisin; David Beljonne; Stéphane Campidelli; Loïc Rondin; Jean-Sébastien Lauret
Jörg Enderlein; Damir Sakhapov; Ingo Gregor; Matteo Croci; Narain Karedla
Johannes Zirkelbach; Masoud Mirzaei; Irena Deperasińska; Boleslaw Kozankiewicz; Burak Gurlek; Alexey Shkarin; Tobias Utikal; Stephan Götzinger; Vahid Sandoghdar
Anastasiia Misiura; Chayan Dutta; Wesley Leung; Jorge Zepeda O; Tanguy Terlier; Christy F. Landes
Redmar C. Vlieg; John van Noort
Hayri E. Balcioglu; Rolf Harkes; Erik H. J. Danen; Thomas Schmidt
Julien Lombard; Thierry Biben; Samy Merabia
Debjit Roy; Zehavit Shapira; Shimon Weiss
Juanzi Shi; Rafael Camacho; Ivan G. Scheblykin
Hao Yan; Tzu-Wei Tseng; Shun Omagari; Iain Hamilton; Tomonori Nakamura; Martin Vacha; Ji-Seon Kim
Stephen A. Lee; Behnaz Ostovar; Christy F. Landes; Stephan Link
Sunidhi Jaiswal; Yufan He; H. Peter Lu
Eli Barkai; Günter Radons; Takuma Akimoto
Simon J. Hauschildt; Zehua Wu; Daniel Uersfeld; Paul Schmid; Christian Götz; Volker Engel; Bernd Engels; Klaus Müllen; Thomas Basché
Cla Duri Tschannen; Thiago L. Vasconcelos; Lukas Novotny
Ianina L. Violi; Luciana P. Martinez; Mariano Barella; Cecilia Zaza; Lukáš Chvátal; Pavel Zemánek; Marina V. Gutiérrez; María Y. Paredes; Alberto F. Scarpettini; Jorge Olmos-Trigo; Valeria R. Pais; Iván Díaz Nóblega; Emiliano Cortes; Juan José Sáenz; Andrea V. Bragas; Julian Gargiulo; Fernando D. Stefani
N. P. Kovalets; E. P. Kozhina; I. V. Razumovskaya; S. A. Bedin; A. A. Piryazev; Yu. V. Grigoriev; A. V. Naumov
Megan A. Steves; Kenneth L. Knappenberger, Jr.
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