Hydrogen production by catalytic steam reforming of the bio-oil, naphtha, and CH4 was investigated over a novel metal-doped catalyst of (Ca24Al28O64)4+4O/Mg (C12A7-Mg). The catalytic steam reforming was investigated from 250 to 850C in the fixed-bed continuous flow reactor. For the reforming of bio-oil, the yield of hydrogen of 80% was obtained at 750C, and the maximum carbon conversion is nearly close to 95% under the optimum steam reforming condition. For the reforming of naphtha and CH4, the hydrogen yield and carbon conversion are lower than that of bio-oil at the same temperature. The characteristics of catalyst were also investigated by XPS. The catalyst deactivation was mainly caused by the deposition of carbon in the catalytic steam reforming process.
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June 2006
Research Article|
June 01 2006
Hydrogen Production by Catalytic Steam Reforming of Bio-oil, Naphtha and CH4 over C12A7-Mg Catalyst
Yue Pan;
Yue Pan
Department of Chemical Physics, Lab of Biomass Clean Energy, University of Science and Technology of China, Hefei 230026,
China
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Zhao-xiang Wang;
Zhao-xiang Wang
Department of Chemical Physics, Lab of Biomass Clean Energy, University of Science and Technology of China, Hefei 230026,
China
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Tao Kan;
Tao Kan
Department of Chemical Physics, Lab of Biomass Clean Energy, University of Science and Technology of China, Hefei 230026,
China
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Xi-feng Zhu;
Xi-feng Zhu
Department of Chemical Physics, Lab of Biomass Clean Energy, University of Science and Technology of China, Hefei 230026,
China
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Quan-xin Li
Quan-xin Li
Department of Chemical Physics, Lab of Biomass Clean Energy, University of Science and Technology of China, Hefei 230026,
China
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Chin. J. Chem. Phys. 19, 190–192 (2006)
Article history
Received:
April 29 2006
Accepted:
May 19 2006
Citation
Yue Pan, Zhao-xiang Wang, Tao Kan, Xi-feng Zhu, Quan-xin Li; Hydrogen Production by Catalytic Steam Reforming of Bio-oil, Naphtha and CH4 over C12A7-Mg Catalyst. Chin. J. Chem. Phys. 1 June 2006; 19 (3): 190–192. https://doi.org/10.1360/cjcp2006.19(3).190.3
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