Monochromatic Cr Kα radiation (5414.8 eV) was used to acquire high-energy photoelectron spectroscopy (HAXPES) data on pure bulk MoS2. The reported spectra include a survey scan, high-resolution spectra of Mo 2s, Mo 2p, Mo 3s, Mo 3p, Mo 3d, Mo 4s, Mo 4p, S 1s, S 2p, and S 2s core-levels, and x-ray excited Auger spectra. The data will be useful for HAXPES studies of Mo compounds.

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