Ferroelastic 90° a-domain dynamics in epitaxial Pb(Zr0.2Ti0.8)O3 (lead zirconium titanate, PZT) films is investigated using lateral and vertical piezoelectric force microscopies. The PZT film consists of out-of-plane polarized c-domains separated by a cross-hatch network of in-plane polarized a-domains. When an electric field is applied across the PZT film, the a-domains are rearranged on the nanoscale. Depending on the direction of the electric field, this results either in larger or more fragmented c-domains. Both lateral and vertical piezoelectric force signals demonstrate the importance of ferroelastic a-domain movement since their dynamics will determine the final polarization retention time and stability of ferroelectric capacitors.

1.
Hiroshi
Ishiwara
,
Masanori
Okuyama
, and
Yoshihiro
Arimoto
,
Ferroelectric Random Access Memories: Fundamentals and Applications
(
Springer
,
New York
,
2004
), Vol.
93
, p.
31
.
2.
P.
Paruch
,
T.
Giamarchi
, and
J. -M.
Triscone
,
Phys. Rev. Lett.
94
,
197601
(
2005
).
3.
N.
Balke
,
I.
Bdikin
,
S.
Kalinin
, and
A. L.
Kholkin
,
J. Am. Ceram. Soc.
92
,
1629
(
2009
).
4.
A.
Roelofs
,
N. A.
Pertsev
,
R.
Waser
,
F.
Schlaphof
,
L. M.
Eng
,
C.
Ganpule
,
V.
Nagarajan
, and
R.
Ramesh
,
Appl. Phys. Lett.
80
,
1424
(
2002
).
5.
C. S.
Ganpule
,
V.
Nagarajan
,
S. B.
Ogale
,
A. L.
Roytburd
,
E. D.
Williams
, and
R.
Ramesh
,
Appl. Phys. Lett.
77
,
3275
(
2000
).
6.
T.
Tybell
,
P.
Paruch
,
T.
Giamarchi
, and
J. -M.
Triscone
,
Phys. Rev. Lett.
89
,
097601
(
2002
).
7.
D. A.
Scrymgeour
and
V.
Gopalan
,
Phys. Rev. B
72
,
024103
(
2005
).
8.
P.
Paruch
,
T.
Giamarchi
,
T.
Tybell
, and
J. -M.
Triscone
,
J. Appl. Phys.
100
,
051608
(
2006
).
9.
P.
Paruch
,
T.
Tybell
, and
J. -M.
Triscone
,
Appl. Phys. Lett.
79
,
530
(
2001
).
10.
T.
Tybell
,
C. H.
Ahn
, and
J. -M.
Triscone
,
Appl. Phys. Lett.
72
,
1454
(
1998
).
11.
F.
Xu
,
F.
Chu
, and
S.
Trolier-McKinstry
,
J. Appl. Phys.
86
,
588
(
1999
).
12.
V.
Nagarajan
A.
Roytburg
,
A.
Stanishevsky
,
S.
Prasertchoung
,
T.
Zhao
,
L.
Chen
,
J.
Melngailis
,
O.
Auciello
, and
R.
Ramesh
,
Nature Mater.
2
,
43
(
2003
).
13.
G.
Le Rhun
,
I.
Vrejoiu
,
L.
Pintilie
,
D.
Hesse
,
M.
Alexe
, and
U.
Gösele
,
Nanotechnology
17
,
3154
(
2006
).
14.
X.
Hong
,
A.
Posadas
,
A.
Lin
, and
C. H.
Ahn
,
Phys. Rev. B
68
,
134415
(
2003
).
15.
T.
Tybell
,
C. H.
Ahn
,
M.
Foeth
, and
J. M.
Triscone
,
Proceedings of the 11th IEEE International Symposium on Applications of Ferroelectrics
,
1998
(unpublished), p.
431
.
16.
C. H.
Ahn
,
T.
Tybell
,
L.
Antognazza
,
K.
Char
,
R. H.
Hammond
,
M. R.
Beasley
,
Ø.
Fischer
, and
J. -M.
Triscone
,
Science
276
,
1100
(
1997
).
17.
J.
Guyonnet
,
H.
Béa
,
F.
Guy
,
S.
Gariglio
,
S.
Fusil
,
K.
Bouzehouane
,
J. -M.
Triscone
, and
P.
Paruch
,
Appl. Phys. Lett.
95
,
132902
(
2009
);
T.
Jungk
,
Á.
Hoffmann
, and
E.
Soergel
,
Appl. Phys. Lett.
89
,
042901
(
2006
).
18.
A.
Wu
,
P. M.
Vilarinho
,
D.
Wu
, and
A.
Gruverman
,
Appl. Phys. Lett.
93
,
262906
(
2008
).
19.
C. S.
Ganpule
,
A. L.
Roytburd
,
V.
Nagarajan
,
B. K.
Hill
,
S. B.
Ogale
,
E. D.
Williams
,
R.
Ramesh
, and
J. F.
Scott
,
Phys. Rev. B
65
,
014101
(
2001
).
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