We experimentally study the occurrence of pattern formation during the slot-die coating of partially wetting liquids onto polyethylenterephthalat-substrates outside the coating window. The experimental investigation is supported by numerical simulations of a dynamical model. Our results demonstrate that beyond a critical coating speed, the deposition of homogeneous coating layers undergoes an instability resulting in the self-organized emergence of patterned coatings, i.e., stripes of different orientation and droplet patterns. We investigate the transitions between the different patterns as triggered by changes in the control parameters inherent to slot-die coating, e.g., the liquid viscosity and the coating gap height. The relatively simple theoretical approach is based on lubrication theory. It is already able to reproduce most of the patterns observed experimentally and reveals a wettability-driven instability mechanism.
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Pattern formation in slot-die coating
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July 2023
Research Article|
July 24 2023
Pattern formation in slot-die coating
Special Collection:
Paint and Coating Physics
Maren Kasischke
;
Maren Kasischke
(Investigation, Visualization, Writing – original draft, Writing – review & editing)
1
Chair of Applied Laser Technology, Ruhr-Universität Bochum
, Universitätsstraße 150, 44801 Bochum, Germany
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Simon Hartmann
;
Simon Hartmann
a)
(Investigation, Software, Visualization, Writing – original draft, Writing – review & editing)
2
Institut für Theoretische Physik, Westfälische Wilhelms-Universität Münster
, Wilhelm-Klemm-Str. 9, 48149 Münster, Germany
3
Center for Nonlinear Science (CeNoS), Westfälische Wilhelms-Universität Münster
, Corrensstr. 2, 48149 Münster, Germany
a)Author to whom correspondence should be addressed: s.hartmann@wwu.de
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Kevin Niermann;
Kevin Niermann
(Investigation, Visualization)
1
Chair of Applied Laser Technology, Ruhr-Universität Bochum
, Universitätsstraße 150, 44801 Bochum, Germany
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Marco Smarra
;
Marco Smarra
(Investigation, Visualization)
1
Chair of Applied Laser Technology, Ruhr-Universität Bochum
, Universitätsstraße 150, 44801 Bochum, Germany
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Denis Kostyrin;
Denis Kostyrin
(Investigation, Visualization)
1
Chair of Applied Laser Technology, Ruhr-Universität Bochum
, Universitätsstraße 150, 44801 Bochum, Germany
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Uwe Thiele
;
Uwe Thiele
b)
(Funding acquisition, Supervision, Writing – review & editing)
2
Institut für Theoretische Physik, Westfälische Wilhelms-Universität Münster
, Wilhelm-Klemm-Str. 9, 48149 Münster, Germany
3
Center for Nonlinear Science (CeNoS), Westfälische Wilhelms-Universität Münster
, Corrensstr. 2, 48149 Münster, Germany
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Evgeny L. Gurevich
Evgeny L. Gurevich
c)
(Funding acquisition, Project administration, Supervision, Writing – original draft, Writing – review & editing)
1
Chair of Applied Laser Technology, Ruhr-Universität Bochum
, Universitätsstraße 150, 44801 Bochum, Germany
4
Laser Center (LFM), University of Applied Sciences Münster
, Stegerwaldstraße 39, 48565 Steinfurt, Germany
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a)Author to whom correspondence should be addressed: s.hartmann@wwu.de
b)
Electronic mail: u.thiele@uni-muenster.de
c)
Electronic mail: gurevich@lat.rub.de
Physics of Fluids 35, 074117 (2023)
Article history
Received:
March 14 2023
Accepted:
June 24 2023
Citation
Maren Kasischke, Simon Hartmann, Kevin Niermann, Marco Smarra, Denis Kostyrin, Uwe Thiele, Evgeny L. Gurevich; Pattern formation in slot-die coating. Physics of Fluids 1 July 2023; 35 (7): 074117. https://doi.org/10.1063/5.0150340
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