In this study, two series of pressurized turbulent jet sooting flames at 1, 3, and 5 bar with either fixed jet velocity or fixed Reynolds number are simulated to study the pressure effects on soot formation and evolution. Through a radiation flamelet progress variable approach with a conditional soot subfilter probability density function (PDF) model to consider the turbulence–chemistry–soot interactions, quantitatively good agreements are achieved for soot volume fraction (SVF) predictions compared with the experimental data, regardless different turbulent intensities and residence times. SVF source terms are then discussed to show the pressure effects on nucleation, condensation, surface growth, and oxidation at different axial positions in these flames. It is found that surface growth and oxidation increase by about three orders of magnitude from 1 to 5 bar, while nucleation and condensation only increase within one order of magnitude. The stronger SVF scaling on pressure than measured data is found to be attributed to the inaccurate surface growth and oxidation scaling on pressure. Further analysis indicates that (i) the uncertainty of C2H2 prediction at elevated pressures is likely a major reason for the too strong surface growth scaling; and (ii) taking account of pressure effects in the conditional subfilter PDF modeling for turbulence–soot–chemistry interactions is likely a key to improve oxidation prediction. The results in this study open up the possibilities for improving future turbulent sooting flame modeling by improving C2H2 chemistry and turbulence–chemistry–soot modeling at elevated pressures.
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January 2023
Research Article|
January 04 2023
Pressure effects on soot formation and evolution in turbulent jet flames
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Dezhi Zhou
;
Dezhi Zhou
(Conceptualization, Data curation, Formal analysis, Investigation, Methodology, Software, Validation, Visualization, Writing – original draft, Writing – review & editing)
1
Department of Mechanical Engineering, University of Minnesota–Twin Cities
, Minneapolis, Minnesota 55455, USA
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Shufan Zou;
Shufan Zou
(Data curation, Formal analysis, Investigation, Methodology, Software, Validation, Visualization, Writing – review & editing)
1
Department of Mechanical Engineering, University of Minnesota–Twin Cities
, Minneapolis, Minnesota 55455, USA
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Wesley R. Boyette
;
Wesley R. Boyette
(Conceptualization, Data curation, Formal analysis, Investigation, Methodology, Visualization, Writing – review & editing)
2
King Abdullah University of Science and Technology (KAUST), CCRC
, Thuwal 23955-6900, Saudi Arabia
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Thibault F. Guiberti
;
Thibault F. Guiberti
(Data curation, Formal analysis, Investigation)
2
King Abdullah University of Science and Technology (KAUST), CCRC
, Thuwal 23955-6900, Saudi Arabia
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William L. Roberts;
William L. Roberts
(Conceptualization, Methodology, Project administration, Supervision)
2
King Abdullah University of Science and Technology (KAUST), CCRC
, Thuwal 23955-6900, Saudi Arabia
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Suo Yang
Suo Yang
a)
(Conceptualization, Data curation, Formal analysis, Funding acquisition, Investigation, Methodology, Project administration, Resources, Software, Supervision, Writing – review & editing)
1
Department of Mechanical Engineering, University of Minnesota–Twin Cities
, Minneapolis, Minnesota 55455, USA
a)Author to whom correspondence should be addressed: [email protected]
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Dezhi Zhou
1
Shufan Zou
1
Wesley R. Boyette
2
Thibault F. Guiberti
2
William L. Roberts
2
Suo Yang
1,a)
1
Department of Mechanical Engineering, University of Minnesota–Twin Cities
, Minneapolis, Minnesota 55455, USA
2
King Abdullah University of Science and Technology (KAUST), CCRC
, Thuwal 23955-6900, Saudi Arabia
a)Author to whom correspondence should be addressed: [email protected]
Physics of Fluids 35, 015105 (2023)
Article history
Received:
November 12 2022
Accepted:
December 14 2022
Citation
Dezhi Zhou, Shufan Zou, Wesley R. Boyette, Thibault F. Guiberti, William L. Roberts, Suo Yang; Pressure effects on soot formation and evolution in turbulent jet flames. Physics of Fluids 1 January 2023; 35 (1): 015105. https://doi.org/10.1063/5.0134674
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