In this work a systematic experimental study was performed to understand the process of liquid drop impact onto a thin film made of a different liquid from drop. The drop and film liquids can be miscible or immiscible. Three general outcomes of deposition, crown formation without splashing, and splashing, were observed in the advancing phase of the drop impact onto a solid surface covered by either a miscible or an immiscible thin film. However, for a miscible film, a larger Weber number and film thickness are needed for the formation of a crown and splashing comparing with immiscible cases. The advancing phase of drop impact onto a thin immiscible film with a large viscosity is similar to that of drop impact onto a dry surface; for a miscible film viscous film, the behavior is far from that of a dry surface. The behavior of liquid lamella in the receding phase of drop impact onto a thin miscible film is reported for the first time. The results show that immiscibility is not a necessary condition for the existence of a receding phase. The existence of a receding phase is highly dependent on the interfacial tension between the drop and the film. The miscibility can significantly affect the receding morphology as it will cause mixing of the two liquids.

1.
A. L.
Yarin
, “
Drop impact dynamics: Splashing, spreading, receding, bouncing…
,”
Annu. Rev. Fluid Mech.
38
,
159
(
2006
).
2.
G.
Liang
and
I.
Mudawar
, “
Review of mass and momentum interactions during drop impact on a liquid film
,”
Int. J. Heat Mass Transfer
101
,
577
(
2016
).
3.
D. A.
Weiss
and
A. L.
Yarin
, “
Single drop impact onto liquid films: Neck distortion, jetting, tiny bubble entrainment, and crown formation
,”
J. Fluid Mech.
385
,
229
(
1999
).
4.
A. B.
Wang
and
C. C.
Chen
, “
Splashing impact of a single drop onto very thin liquid films
,”
Phys. Fluids
12
,
2155
(
2000
).
5.
R.
Rioboo
,
C.
Bauthier
,
J.
Conti
,
M.
Voué
, and
J.
Coninck
, “
Experimental investigation of splash and crown formation during single drop impact on wetted surfaces
,”
Exp. Fluids
35
,
648
(
2003
).
6.
A. L.
Yarin
and
D. A.
Weiss
, “
Impact of drops on solid surfaces: Self-similar capillary waves, and splashing as a new type of kinematic discontinuity
,”
J. Fluid Mech.
283
,
141
(
1995
).
7.
G. E.
Cossali
,
A.
Coghe
, and
M.
Marengo
, “
The impact of a single drop on a wetted solid surface
,”
Exp. Fluids
22
,
463
472
(
1997
).
8.
D. G.
Weldon
,
A.
Bochan
, and
M.
Schleiden
, “
The effect of oil, grease, and salts on coating performance—A laboratory evaluation
,”
J. Protect. Coat. Linings
4
,
46
(
1987
), ISSN: 8755–1985.
9.
P. G.
Smith
,
T. G.
Van De Ven
, and
S. G.
Mason
, “
The transient interfacial tension between two miscible fluids
,”
J. Colloid Interface Sci.
80
,
302
(
1981
).
10.
S. T.
Thoroddsen
,
T. G.
Etoh
, and
K.
Takehara
, “
Crown breakup by Marangoni instability
,”
J. Fluid Mech.
557
,
63
(
2006
).
11.
A.
Geppert
,
A.
Štrbac
,
M.
Marengo
,
G.
Lamanna
, and
B.
Weigand
, “
Two-component droplet wall-film interaction: Crown morphology as a function of liquids viscosity and surface tension
,” in
13th ICLASS Americas
,
Tainan, Taiwan
,
23–27 August 2015
.
12.
A.
Geppert
,
A.
Terzis
,
G.
Lamanna
,
M.
Marengo
, and
B.
Weigand
, “
On the formation of secondary droplets from crown bottom breakdown during drop impact on very thin films
,” in
27th Annual Conference on Liquid Atomization and Spray Systems
,
Brighton, UK
,
4–7 September 2016
.
13.
C.
Lee
,
H.
Kim
, and
Y.
Nam
, “
Drop impact dynamics on oil-infused nanostructured surfaces
,”
Langmuir
30
,
8400
(
2014
).
14.
J. H.
Kim
and
J. P.
Rothstein
, “
Droplet impact dynamics on lubricant-infused superhydrophobic surfaces: The role of viscosity ratio
,”
Langmuir
32
,
10166
(
2016
).
15.
D.
Sohounhloue
,
L.
Tenebre
,
M.
Privat
,
J. M.
Douillard
,
R.
Bennes
, and
E.
Tronel-Peyroz
, “
Thermodynamic properties and structure of the water-ethanol silicone oil interface
,”
Can. J. Chem.
65
,
2299
(
1987
).
16.
S.
Mangili
,
C.
Antonini
,
M.
Marengo
, and
A.
Amirfazli
, “
Understanding the drop impact phenomenon on soft PDMS substrates
,”
Soft Matter
8
,
10045
(
2012
).
17.
I. S.
Khattab
,
F.
Bandarkar
,
M. A. A.
Fakhree
, and
A.
Jouyban
, “
Density, viscosity, and surface tension of water+ ethanol mixtures from 293 to 323 K
,”
Korean J. Chem. Eng.
29
,
812
(
2012
).
18.
M.
Dinc
and
D. D.
Gray
, “
Drop impingement onto a wetted surface: Effect of gravity and shape
,” in
Proceedings of the 10th WSEAS International Conference on Fluid Mechanics and Aerodynamics (FMA12), Istanbul, Turkey
, pp.
374
379
(
2012
), ISBN: 978-1-61804-114-2.
19.
C.
Antonini
,
A.
Amirfazli
, and
M.
Marengo
, “
Drop impact and wettability: From hydrophilic to superhydrophobic surfaces
,”
Phys. Fluids
24
,
102104
(
2012
).
20.
A.
Carlson
,
P.
Kim
,
G.
Amberg
, and
H. A.
Stone
, “
Short and long time drop dynamics on lubricated substrates
,”
Europhys. Lett.
104
,
34008
(
2013
).

Supplementary Material

You do not currently have access to this content.