Ultrasound and magnetization studies of bond frustrated spinel HgCr2S4 are performed as a function of temperature in static magnetic fields. Beside the anharmonic effect, the sound velocity shows pronounced anomaly at the antiferromagnetic (AFM) transition at TN = 23 K with an additional significant increase of the order of 0.5% indicating a strong spin-lattice coupling. External magnetic fields enhance the ferromagnetic (FM) correlations and shift the anomalies to lower temperatures concomitantly with the reduction of the Néel temperature. The constructed H–T phase diagram beside the long-range AFM states reveals the state with induced FM order and regimes with short-range AFM and FM correlations as well.
References
1.
P. K.
Baltzer
, P. J.
Wojtowicz
, M.
Robbins
, and E.
Lopatin
, Phys. Rev.
151
, 367
(1966
).2.
V.
Tsurkan
, H.-A.
Krug von Nidda
, A.
Krimmel
, P.
Lunkenheimer
, J.
Hemberger
, T.
Rudolf
, and A.
Loidl
, Phys. Status Solidi A
206
, 1082
(2009
).3.
S.-H.
Lee
, C.
Broholm
, W.
Ratcliff
, G.
Gasparovic
, Q.
Huang
, T. H.
Kim
, and S.-W.
Cheong
, Nature
418
, 856
(2002
).4.
J.
Hemberger
, P.
Lunkenheimer
, R.
Ficht
, H.-A.
Krug von Nidda
, V.
Tsurkan
, and A.
Loidl
, Nature
434
, 364
(2005
).5.
A. P.
Ramirez
, R. J.
Cava
, and J.
Krajewski
, Nature
386
, 156
(1997
).6.
V.
Fritsch
, J.
Deisenhofer
, R.
Fichtl
, J.
Hemberger
, H.-A.
Krug von Nidda
, M.
Mucksch
, M.
Nicklas
, D.
Samusi
, J. D.
Thompson
, R.
Tidecks
, V.
Tsurkan
, and A.
Loidl
, Phys. Rev. B
67
, 144419
(2003
).7.
A. P.
Ramirez
, in Handbook of Magnetic Materials
, edited by K. H. J.
Buschow
(Elsevier Science
, New York/North-Holland, Amsterdam
, 2001
), Vol. 13
, p. 423
.8.
T.
Rudolf
, Ch.
Kant
, F.
Mayr
, J.
Hemberger
, V.
Tsurkan
, and A.
Loidl
, New J. Phys.
9
, 76
(2007
).9.
Y.
Yamashita
and K.
Ueda
, Phys. Rev. Lett.
85
, 4960
(2000
).10.
O.
Tchernyshyov
, R.
Moessner
, and S. L.
Sondhi
, Phys. Rev. Lett.
88
, 067203
(2002
).11.
J.
Hemberger
, T.
Rudolf
, H.-A.
Krug von Nidda
, F.
Mayr
, A.
Pimenov
, V.
Tsurkan
, and A.
Loidl
, Phys. Rev. Lett.
97
, 087204
(2006
).12.
J.
Hemberger
, H. A.
Krug von Nidda
, V.
Tsurkan
, and A.
Loidl
, Phys. Rev. Lett.
98
, 147203
(2007
).13.
T.
Rudolf
, C.
Kant
, F.
Mayr
, J.
Hemberger
, V.
Tsurkan
, and A.
Loidl
, Phys. Rev. B
75
, 052410
(2007
).14.
T.
Rudolf
, Ch.
Kant
, F.
Mayr
, J.
Hemberger
, V.
Tsurkan
, and A.
Loidl
, Phys. Rev. B
76
, 174307
(2007
).15.
S.
Weber
, P.
Lunkenheimer
, R.
Fichtl
, J.
Hemberger
, V.
Tsurkan
, and A.
Loidl
, Phys. Rev. Lett.
96
, 157202
(2006
).16.
M.
Fiebig
, J. Phys. D
38
, R123
(2005
).17.
S.-W.
Cheong
and M.
Mostovoy
, Nat. Mater.
6
, 13
(2007
).18.
R.
Ramesh
and N. A.
Spaldin
, Nat. Mater.
6
, 21
(2007
).19.
Y.
Tokura
and S.
Seki
, Adv. Mater.
22
, 1554
(2010
).20.
B.
Lüthi
, Physical Acoustics in the Solid State
(Springer
, Berlin
, 2005
).21.
P. K.
Baltzer
, P. J.
Wojtowicz
, M.
Robbins
, and E.
Lopatin
, Phys. Rev.
151
, 367
(1966
).22.
J. M.
Hasting
and L. M.
Corliss
, J. Phys. Chem. Solids
29
, 9
(1968
).23.
H. W.
Lehmann
and G.
Harbeke
, Phys. Rev. B
1
, 319
(1970
).24.
V.
Tsurkan
, J.
Hemberger
, A.
Krimmel
, H.-A.
Krug von Nidda
, P.
Lunkenheimer
, S.
Weber
, V.
Zestrea
, and A.
Loidl
, Phys. Rev. B
73
, 224442
(2006
).25.
L. C.
Chapon
, P. G.
Radaelli
, Y. S.
Hor
, M. T. F.
Telling
, and J. F.
Mitchell
, preprint arXiv:cond-mat/060803 (2006
).26.
J.
Rodriguez-Carvajal
, Physica B
192
, 55
(1993
).27.
S.
Zherlitsyn
, S.
Yasin
, J.
Wosnitza
, A. A.
Zvyagin
, A. V.
Andreev
, and V.
Tsurkan
, Fiz. Nizk. Temp.
40
, 160
(2014
).S.
Zherlitsyn
, S.
Yasin
, J.
Wosnitza
, A. A.
Zvyagin
, A. V.
Andreev
, and V.
Tsurkan
, [Low Temp. Phys.
40
, 123
(2014
)].© 2017 Author(s).
2017
Author(s)
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