We report on viscous adhesion measurements conducted in sphere-plane geometry between a rigid sphere and soft surfaces submerged in silicone oils. Increasing the surface compliance leads to a decrease in the adhesive strength due to elastohydrodynamic deformation of the soft surface during debonding. The force-displacement and fluid film thickness-time data are compared to an elastohydrodynamic model that incorporates the force measuring spring and finds good agreement between the model and data. We calculate the pressure distribution in the fluid and find that, in contrast to debonding from rigid surfaces, the pressure drop is non-monotonic and includes the presence of stagnation points within the fluid film when a soft surface is present. In addition, viscous adhesion in the presence of a soft surface leads to a debonding process that occurs via a peeling front (located at a stagnation point), even in the absence of solid–solid contact. As a result of mass conservation, the elastohydrodynamic deformation of the soft surface during detachment leads to surfaces that come closer as the surfaces are separated. During detachment, there is a region with fluid drainage between the centerpoint and the stagnation point, while there is fluid infusion further out. Understanding and harnessing the coupling between lubrication pressure, elasticity, and surface interactions provides material design strategies for applications such as adhesives, coatings, microsensors, and biomaterials.
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Out-of-contact peeling caused by elastohydrodynamic deformation during viscous adhesion
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7 October 2023
Research Article|
October 03 2023
Out-of-contact peeling caused by elastohydrodynamic deformation during viscous adhesion
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Adhesion and Friction
Xingchen Shao
;
Xingchen Shao
(Conceptualization, Data curation, Formal analysis, Investigation, Methodology, Visualization, Writing – original draft, Writing – review & editing)
1
Chemical and Biomolecular Engineering Department, University of California
, Berkeley, California 94720, USA
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Yumo Wang
;
Yumo Wang
(Conceptualization, Formal analysis, Investigation, Methodology, Writing – original draft, Writing – review & editing)
2
National Engineering Laboratory for Pipeline Safety, Beijing Key Laboratory of Urban Oil and Gas Distribution Technology, China University of Petroleum, Beijing
, 18# Fuxue Road, Changping District, 102249 Beijing, China
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Joelle Frechette
Joelle Frechette
a)
(Conceptualization, Funding acquisition, Investigation, Methodology, Project administration, Supervision, Writing – original draft, Writing – review & editing)
1
Chemical and Biomolecular Engineering Department, University of California
, Berkeley, California 94720, USA
a)Author to whom correspondence should be addressed: [email protected]
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Xingchen Shao
1
Yumo Wang
2
Joelle Frechette
1,a)
1
Chemical and Biomolecular Engineering Department, University of California
, Berkeley, California 94720, USA
2
National Engineering Laboratory for Pipeline Safety, Beijing Key Laboratory of Urban Oil and Gas Distribution Technology, China University of Petroleum, Beijing
, 18# Fuxue Road, Changping District, 102249 Beijing, China
a)Author to whom correspondence should be addressed: [email protected]
J. Chem. Phys. 159, 134904 (2023)
Article history
Received:
July 11 2023
Accepted:
September 12 2023
Citation
Xingchen Shao, Yumo Wang, Joelle Frechette; Out-of-contact peeling caused by elastohydrodynamic deformation during viscous adhesion. J. Chem. Phys. 7 October 2023; 159 (13): 134904. https://doi.org/10.1063/5.0167300
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