In this work, we study the magnetic phases of a spatially modulated chain of spin-1 Rydberg excitons. Using the Density Matrix Renormalization Group (DMRG) technique, we study various magnetic and topologically nontrivial phases using both single-particle properties, such as local magnetization and quantum entropy, and many-body ones, such as pair-wise Néel and long-range string correlations. In particular, we investigate the emergence and robustness of the Haldane phase, a topological phase of anti-ferromagnetic spin-1 chains. Furthermore, we devise a hybrid quantum algorithm employing restricted Boltzmann machine to simulate the ground state of such a system that shows very good agreement with the results of exact diagonalization and DMRG.
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14 December 2022
Research Article|
December 14 2022
Magnetic phases of spatially modulated spin-1 chains in Rydberg excitons: Classical and quantum simulations
Manas Sajjan
;
Manas Sajjan
a)
(Conceptualization, Data curation, Formal analysis, Investigation, Methodology, Writing – original draft, Writing – review & editing)
1
Department of Chemistry, Purdue University
, West Lafayette, Indiana 47907, USA
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Hadiseh Alaeian
;
Hadiseh Alaeian
b)
(Formal analysis, Supervision, Writing – original draft, Writing – review & editing)
2
Elmore Family School of Electrical and Computer Engineering, Purdue University
, West Lafayette, Indiana 47907, USA
3
Department of Physics and Astronomy, Purdue University
, West Lafayette, Indiana 47907, USA
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Sabre Kais
Sabre Kais
c)
(Formal analysis, Funding acquisition, Supervision)
1
Department of Chemistry, Purdue University
, West Lafayette, Indiana 47907, USA
2
Elmore Family School of Electrical and Computer Engineering, Purdue University
, West Lafayette, Indiana 47907, USA
3
Department of Physics and Astronomy, Purdue University
, West Lafayette, Indiana 47907, USA
c)Author to whom correspondence should be addressed: kais@purdue.edu
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a)
Electronic mail: msajjan@purdue.edu
b)
Electronic mail: halaeian@purdue.edu
c)Author to whom correspondence should be addressed: kais@purdue.edu
J. Chem. Phys. 157, 224111 (2022)
Article history
Received:
September 27 2022
Accepted:
November 29 2022
Citation
Manas Sajjan, Hadiseh Alaeian, Sabre Kais; Magnetic phases of spatially modulated spin-1 chains in Rydberg excitons: Classical and quantum simulations. J. Chem. Phys. 14 December 2022; 157 (22): 224111. https://doi.org/10.1063/5.0128283
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