We report a surprising result, established by numerical simulations and analytical arguments for a one-dimensional lattice model of random sequential adsorption, that even an arbitrarily small imprecision in the lattice-site localization changes the convergence to jamming from fast, exponential, to slow, power-law, with, for some parameter values, a discontinuous jump in the jamming coverage value. This finding has implications for irreversible deposition on patterned substrates with pre-made landing sites for particle attachment. We also consider a general problem of the particle (depositing object) size not an exact multiple of the lattice spacing, and the lattice sites themselves imprecise, broadened into allowed-deposition intervals. Regions of exponential vs. power-law convergence to jamming are identified, and certain conclusions regarding the jamming coverage are argued for analytically and confirmed numerically.
Skip Nav Destination
Random sequential adsorption on imprecise lattice
Article navigation
28 June 2016
Research Article|
June 28 2016
Random sequential adsorption on imprecise lattice
Vladimir Privman
;
Vladimir Privman
a)
Department of Physics,
Clarkson University
, Potsdam, New York 13699, USA
Search for other works by this author on:
Han Yan
Han Yan
Department of Physics,
Clarkson University
, Potsdam, New York 13699, USA
Search for other works by this author on:
a)
Author to whom correspondence should be addressed. Electronic mail: privman@clarkson.edu
J. Chem. Phys. 144, 244704 (2016)
Article history
Received:
April 29 2016
Accepted:
May 27 2016
Citation
Vladimir Privman, Han Yan; Random sequential adsorption on imprecise lattice. J. Chem. Phys. 28 June 2016; 144 (24): 244704. https://doi.org/10.1063/1.4954332
Download citation file:
Sign in
Don't already have an account? Register
Sign In
You could not be signed in. Please check your credentials and make sure you have an active account and try again.
Sign in via your Institution
Sign in via your InstitutionPay-Per-View Access
$40.00
Citing articles via
Related Content
The phi meter: A simple, fuel‐independent instrument for monitoring combustion equivalence ratio
Rev Sci Instrum (July 1994)
Surface fine structure influence on saturated random packings
J. Chem. Phys. (February 2017)
Structures of fused-dimer fluids: A new closure based on the potential distribution theorems
J. Chem. Phys. (May 2001)
Electron affinity of the sodium atom within the coupled-channel hyperspherical approach
J. Chem. Phys. (February 2004)
Optimal intermediates in staged free energy calculations
J. Chem. Phys. (September 1999)