This paper introduces and analyses a general statistical model, termed the RAndom RElaxations (RARE) model, of random relaxation processes in disordered systems. The model considers excitations that are randomly scattered around a reaction center in a general embedding space. The model's input quantities are the spatial scattering statistics of the excitations around the reaction center, and the chemical reaction rates between the excitations and the reaction center as a function of their mutual distance. The framework of the RARE model is versatile and a detailed stochastic analysis of the random relaxation processes is established. Analytic results regarding the duration and the range of the random relaxation processes, as well as the model's thermodynamic limit, are obtained in closed form. In particular, the case of power-law inputs, which turn out to yield stretched exponential relaxation patterns and asymptotically Paretian relaxation ranges, is addressed in detail.
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21 December 2012
Research Article|
December 19 2012
The RARE model: A generalized approach to random relaxation processes in disordered systems Available to Purchase
Iddo Eliazar;
Iddo Eliazar
a)
1
Holon Institute of Technology
, P.O. Box 305, Holon 58102, Israel
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Ralf Metzler
Ralf Metzler
b)
2Institute for Physics and Astronomy,
University of Potsdam
, 14476 Potsdam-Golm, Germany
3Physics Department,
Tampere University of Technology
, FI-33101 Tampere, Finland
Search for other works by this author on:
Iddo Eliazar
1,a)
Ralf Metzler
2,3,b)
1
Holon Institute of Technology
, P.O. Box 305, Holon 58102, Israel
2Institute for Physics and Astronomy,
University of Potsdam
, 14476 Potsdam-Golm, Germany
3Physics Department,
Tampere University of Technology
, FI-33101 Tampere, Finland
a)
Electronic mail: [email protected].
b)
Electronic mail: [email protected].
J. Chem. Phys. 137, 234106 (2012)
Article history
Received:
September 21 2012
Accepted:
November 26 2012
Citation
Iddo Eliazar, Ralf Metzler; The RARE model: A generalized approach to random relaxation processes in disordered systems. J. Chem. Phys. 21 December 2012; 137 (23): 234106. https://doi.org/10.1063/1.4770266
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