With the nonstochastic quantum mechanical study of a quantum dot light emitter, we find that fluorescence intermittency statistics are universal and insensitive to the microscopic nature of the tunneling fluctuation between quantum dot and trapping state. We also investigate the power-law exponent and the crossover time of the on-time probability (for ) and (for ) under an optical field of given energy and strength. For easy off-resonance excitation, it is found in both numerical and analytic ways that is proportional to the intensity of the optical field (i.e., the square of the field strength) independent of the internal parameters of a quantum dot. Furthermore, it is also found that in the limit of vanishing field strength is the upper bound of the exponent and becomes less than 2 as the field strength increases.
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21 August 2010
Research Article|
August 17 2010
Field-induced control of universal fluorescence intermittency of a quantum dot light emitter Available to Purchase
J. D. Lee;
J. D. Lee
a)
School of Materials Science,
Japan Advanced Institute of Science and Technology
, Ishikawa 923-1292, Japan
Search for other works by this author on:
S. Maenosono
S. Maenosono
School of Materials Science,
Japan Advanced Institute of Science and Technology
, Ishikawa 923-1292, Japan
Search for other works by this author on:
J. D. Lee
a)
School of Materials Science,
Japan Advanced Institute of Science and Technology
, Ishikawa 923-1292, Japan
S. Maenosono
School of Materials Science,
Japan Advanced Institute of Science and Technology
, Ishikawa 923-1292, Japan
a)
Electronic mail: [email protected].
J. Chem. Phys. 133, 074703 (2010)
Article history
Received:
June 07 2010
Accepted:
July 25 2010
Citation
J. D. Lee, S. Maenosono; Field-induced control of universal fluorescence intermittency of a quantum dot light emitter. J. Chem. Phys. 21 August 2010; 133 (7): 074703. https://doi.org/10.1063/1.3479578
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