We introduce a method for the all-electron calculation of the NMR chemical shifts and the EPR tensor using the Gaussian and augmented-plane-wave method. The presented approach is based on the generalized density functional perturbation theory. The method is validated by comparison with other theoretical methods for a selection of small molecules. We also present two exemplary applications that involve the calculation of the chemical shifts of a hydrated adenine and the tensor for the center in -quartz using a quantum mechanical/molecular mechanical approach.
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