Thermophysical properties of molten refractory metals (titanium, zirconium, hafnium, and niobium) have been measured using a containerless method. Using an in-house developed electrostatic levitator, the density, the heat capacity, the entropy, the surface tension, and the viscosity of liquid phases have been measured over a wide temperature range. The measured data showed good agreement with theoretical calculations based on the hard sphere model.

1.
CRC Handbook of Chemistry and Physics, 78th ed., edited by D. R. Lide and H. P. R. Frederikse (CRC, Boca Raton, FL, 1997).
2.
H.-J. Fecht and R. K. Wunderlich, Proceedings of the 13th International Symposium on experimental methods for microgravity materials science, 2001, p. 545.
3.
T. Itami, in Condensed Matter Disordered Solids, edited by S. K. Srivastava and N. H. March (World Scientific, Singapore, 1995), p. 123.
4.
T.
Itami
and
M.
Shimoji
,
J. Phys. F: Met. Phys.
14
,
L15
(
1984
).
5.
H.
Itoh
,
I.
Yokoyama
, and
Y.
Waseda
,
J. Phys. F: Met. Phys.
16
,
L113
(
1986
).
6.
T.
Ishikawa
,
P.-F.
Paradis
, and
S.
Yoda
,
J. Japan Soc. Microgavity Appl.
17
,
98
(
2000
).
7.
T.
Ishikawa
,
P.-F.
Paradis
, and
S.
Yoda
,
J. Japan Soc. Microgavity Appl.
18
,
106
(
2001
).
8.
W. K.
Rhim
,
S. K.
Chung
,
D.
Barber
,
K. F.
Man
,
G.
Gutt
,
A. A.
Rulison
, and
R. E.
Spjut
,
Rev. Sci. Instrum.
64
,
2961
(
1993
).
9.
T.
Ishikawa
,
P.-F.
Paradis
, and
S.
Yoda
,
Rev. Sci. Instrum.
72
,
2490
(
2001
).
10.
W. K.
Rhim
and
T.
Ishikawa
,
Rev. Sci. Instrum.
69
,
3628
(
1998
).
11.
W. K.
Rhim
and
P.-F.
Paradis
,
Rev. Sci. Instrum.
70
,
4652
(
1999
).
12.
S. K.
Chung
,
D. B.
Thiessen
, and
W. K.
Rhim
,
Rev. Sci. Instrum.
67
,
3175
(
1996
).
13.
A. J.
Rulison
and
W. K.
Rhim
,
Rev. Sci. Instrum.
65
,
695
(
1994
).
14.
W. K.
Rhim
,
K.
Ohsaka
,
P.-F.
Paradis
, and
R. E.
Spjut
,
Rev. Sci. Instrum.
70
,
2796
(
1999
).
15.
J. Q.
Feng
and
K. V.
Beard
,
Proc. R. Soc. London, Ser. A
430
,
133
(
1990
).
16.
H. Lamb, Hydrodynamics, 6th ed. (Cambridge University Press, Cambridge, 1932), p. 473.
17.
N. F.
Carnahan
and
K. E.
Starling
,
J. Chem. Phys.
51
,
635
(
1969
).
18.
J. K.
Norskov
,
Phys. Rev. B
26
,
2875
(
1982
).
19.
R. J.
Speedy
,
Mol. Phys.
66
,
577
(
1989
).
20.
R. C.
Brown
and
N. H.
March
,
J. Phys. C
5
,
L363
(
1973
).
21.
P. A.
Egelstaff
and
B. J.
Widom
,
J. Chem. Phys.
53
,
2667
(
1970
).
22.
J. A.
Alonso
and
M.
Silbert
,
Phys. Chem. Liq.
17
,
209
(
1987
).
23.
J. A.
Alonso
,
Phys. Chem. Liq.
21
,
257
(
1990
).
24.
T. Ishikawa, P.-F. Paradis, and S. Yoda, 2nd Pan-Pacific Basin workshop on microgravity sciences, 2001, p. TP-1019.
25.
P.-F.
Paradis
,
T.
Ishikawa
, and
S.
Yoda
,
Int. J. Thermophys.
23
,
825
(
2002
).
26.
P.-F.
Paradis
,
T.
Ishikawa
, and
S.
Yoda
,
Int. J. Thermophys.
23
,
555
(
2002
).
27.
I. Barin, O. Knacke, and O. Kubaschewski, Thermochemical Properties of Inorganic Substances (Springer-Verlag, New York, 1977).
28.
Y.
Waseda
and
S.
Tamaki
,
Philos. Mag.
32
,
273
(
1975
).
29.
C. M.
Varma
and
A. J.
Wilson
,
Phys. Rev. B
22
,
3795
(
1980
).
30.
S. N.
Khanna
and
F.
Cyrot-Lackmann
,
J. Phys. (Paris)
40
,
L45
(
1979
).
31.
I.
Egry
,
A.
Diefenbach
,
W.
Dreier
, and
J.
Piller
,
Int. J. Thermophys.
22
,
569
(
2001
).
32.
S.
Ansell
,
S.
Krishnan
,
J. K. R.
Weber
,
J. J.
Felten
,
P. C.
Nordine
,
M. A.
Beno
,
D. L.
Price
, and
M.-L.
Saboungi
,
Phys. Rev. Lett.
78
,
464
(
1997
).
33.
G.
Jacobs
and
I.
Egry
,
Phys. Rev. B
59
,
3961
(
1999
).
34.
T.
Schenk
,
D.
Holland-Moritz
,
V.
Simonet
,
R.
Bellissent
, and
D. M.
Herlach
,
Phys. Rev. Lett.
89
,
075507
(
2002
).
35.
P.-F.
Paradis
,
T.
Ishikawa
, and
S.
Yoda
,
J. Non-Cryst. Solids
312–314
,
309
(
2002
).
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