In this paper, the dynamics of a magnetization undergoing a radiation-damping based feedback radio-frequency field is investigated both theoretically and experimentally. It is shown that due to the presence of T1 relaxation the evolution equations predict the existence of self-sustained maser pulses. This phenomenon is a consequence of the competition between two different processes, namely, T1 relaxation and a precession about a magnetization-dependent radio-frequency field. Experiments show the existence of periodic revivals of the free induction decay over unusually long periods of time, on the order of tens of seconds.

1.
N.
Bloembergen
and
R. V.
Pound
,
Phys. Rev.
95
,
8
(
1954
).
2.
A. Abragam, The Principles of Nuclear Magnetism (Clarendon, Oxford, 1961).
3.
V. J.
Sklenar
,
J. Magn. Reson.
114
,
132
(
1995
).
4.
P.
Broakaert
and
J.
Jeener
,
J. Magn. Reson.
113
,
60
(
1995
).
5.
A.
Louis-Joseph
,
D.
Abergel
, and
J.-Y.
Lallemand
,
J. Biomol. NMR
5
,
212
(
1995
).
6.
C.
Anklin
,
M.
Rindlisbacher
,
G.
Otting
, and
F. H.
Laukien
,
J. Magn. Reson.
106
,
199
(
1995
).
7.
D.
Abergel
,
A.
Louis-Joseph
, and
J.-Y.
Lallemand
,
Chem. Phys. Lett.
262
,
465
(
1996
).
8.
D.
Abergel
,
A.
Louis-Joseph
, and
J.-Y.
Lallemand
,
J. Chem. Phys.
112
,
6365
(
2000
).
9.
S.
Bloom
,
J. Appl. Phys.
28
,
800
(
1957
).
10.
R.
Hobson
and
R.
Kayser
,
J. Magn. Reson.
20
,
458
(
1975
).
11.
T.
Barbara
,
J. Magn. Reson.
98
,
608
(
1992
).
12.
J. A. Guckenheimer and P. Holmes, Nonlinear Oscillations, Dynamical Systems, and Bifurcations of Vector Fields (Springer, New York, 1983).
13.
D. K. Arrowsmith and M. Place, Differential Systems: Differential Equations, Maps, and Chaotic Behavior (Chapman and Hall, New York, 1992).
14.
This effect was in fact anticipated some time ago; see J. Jeener, P. Broakaert, and A. Vlassenbroek, Collective effects in high resolution liquid NMR, Lecture Notes for the 14th Waterloo NMR Summer School, June 16–21, 1997.
15.
J.
Jeener
,
A.
Vlassenbroek
, and
P.
Broakaert
,
J. Chem. Phys.
103
,
1309
(
1995
).
16.
M. P.
Augustine
and
E. L.
Hahn
,
J. Chem. Phys.
107
,
3324
(
1997
).
This content is only available via PDF.
You do not currently have access to this content.