We report magnetic and thermodynamic measurements for Nd2Ni2Pb, one of the recently discovered R2Ni2Pb family of layered intermetallics. A specific heat jump at 19 K corresponds to an antiferromagnetic transition involving crystal-field-split Nd levels. Magnetization measurements show this phase to have a canted structure, with a metamagnetic transition to an aligned phase occurring in H=3T at low temperatures. The single antiferromagnetic phase stands in contrast to the more complex magnetic structures and multiple transitions in the heavy-rare-earth members of this family.

1.
L. D.
Gulay
,
Y. M.
Kalychak
, and
M.
Wolcyrz
,
J. Alloys Compd.
311
,
228
(
2000
).
2.
A. D.
Chinchure
,
E.
Munoz-Sandoval
, and
J. A.
Mydosh
,
Phys. Rev. B
66
,
020409
(
2002
).
3.
E.
Munoz-Sandoval
,
A.
Diaz-Ortiz
,
A. D.
Chinchure
, and
J. A.
Mydosh
,
J. Alloys Compd.
369
,
260
(
2004
).
4.
L. D.
Gulay
and
M.
Wolcyrz
,
Pol. J. Chem.
75
,
1073
(
2001
).
5.
B. H.
Toby
,
J. Appl. Crystallogr.
34
,
210
(
2001
).
6.
C.
Kittel
,
Introduction to Solid State Physics
(
Wiley
,
New York
,
1986
).
7.
S.
Chikazumi
,
Physics of Ferromagnetism
(
Oxford University Press
, New York,
1997
).
8.
A. D.
Chinchure
,
E.
Munoz-Sandoval
, and
J. A.
Mydosh
,
Phys. Rev. B
64
,
020404
(
2001
).
9.
M.
Endo
,
I.
Umehara
,
Y.
Adachi
,
Y.
Isikawa
, and
K.
Sato
,
Mater. Trans., JIM
41
,
452
(
2000
).
10.
A.
Tari
,
The Specific Heat of Matter at Low Temperatures
(
Imperial College Press
, London,
2003
).
You do not currently have access to this content.