In recent years, the implementation of thin-film Ta has led to improved coherence times in superconducting circuits. Efforts to further optimize this materials set have become a focus of the subfield of materials for superconducting quantum computing. It has been previously hypothesized that grain size could be correlated with device performance. In this work, we perform a comparative grain size experiment with -Ta on axis sapphire. Our evaluation methods include both room-temperature chemical and structural characterization and cryogenic microwave measurements, and we report no statistical difference in device performance between smaller- and larger-grain-size devices with grain sizes of 924 and 1700 nm , respectively. These findings suggest that grain size is not correlated with loss in the parameter regime of interest for Ta grown on c axis sapphire, narrowing the parameter space for optimization of this materials set.
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14 October 2023
Research Article|
October 09 2023
Grain size in low loss superconducting Ta thin films on c axis sapphire
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2023 Early Career Investigator Selection
Sarah Garcia Jones
;
Sarah Garcia Jones
(Investigation, Writing – review & editing)
1
Department of Electrical, Computer, and Energy Engineering, University of Colorado Boulder
, Boulder, Colorado 80309, USA
2
Department of Physics, University of Colorado
, Boulder, Colorado 80309, USA
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Nicholas Materise
;
Nicholas Materise
(Investigation, Software, Writing – original draft, Writing – review & editing)
3
Department of Physics, Colorado School of Mines
, Golden, Colorado 80401, USA
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Ka Wun Leung
;
Ka Wun Leung
(Investigation)
4
Department of Physics, The Hong Kong University of Science and Technology
, Clear Water Bay, Kowloon, Hong Kong, China
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Joel C. Weber
;
Joel C. Weber
(Investigation, Methodology)
5
National Institute of Standards and Technology
, Boulder, Colorado 80305, USA
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Brian D. Isakov;
Brian D. Isakov
(Writing – review & editing)
1
Department of Electrical, Computer, and Energy Engineering, University of Colorado Boulder
, Boulder, Colorado 80309, USA
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Xi Chen;
Xi Chen
(Investigation)
4
Department of Physics, The Hong Kong University of Science and Technology
, Clear Water Bay, Kowloon, Hong Kong, China
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Jiangchang Zheng;
Jiangchang Zheng
(Investigation)
4
Department of Physics, The Hong Kong University of Science and Technology
, Clear Water Bay, Kowloon, Hong Kong, China
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András Gyenis
;
András Gyenis
(Funding acquisition, Investigation, Writing – review & editing)
1
Department of Electrical, Computer, and Energy Engineering, University of Colorado Boulder
, Boulder, Colorado 80309, USA
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Berthold Jaeck
;
Berthold Jaeck
a)
(Conceptualization, Formal analysis, Funding acquisition, Methodology, Visualization, Writing – review & editing)
4
Department of Physics, The Hong Kong University of Science and Technology
, Clear Water Bay, Kowloon, Hong Kong, China
6
HKUST IAS Center for Quantum Technologies, The Hong Kong University of Science and Technology
, Clear Water Bay, Kowloon, Hong Kong, China
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Corey Rae H. McRae
Corey Rae H. McRae
b)
(Conceptualization, Data curation, Formal analysis, Funding acquisition, Methodology, Project administration, Software, Supervision, Visualization, Writing – review & editing)
1
Department of Electrical, Computer, and Energy Engineering, University of Colorado Boulder
, Boulder, Colorado 80309, USA
2
Department of Physics, University of Colorado
, Boulder, Colorado 80309, USA
5
National Institute of Standards and Technology
, Boulder, Colorado 80305, USA
b)Author to whom correspondence should be addressed: [email protected]
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b)Author to whom correspondence should be addressed: [email protected]
J. Appl. Phys. 134, 144402 (2023)
Article history
Received:
July 25 2023
Accepted:
September 18 2023
Citation
Sarah Garcia Jones, Nicholas Materise, Ka Wun Leung, Joel C. Weber, Brian D. Isakov, Xi Chen, Jiangchang Zheng, András Gyenis, Berthold Jaeck, Corey Rae H. McRae; Grain size in low loss superconducting Ta thin films on c axis sapphire. J. Appl. Phys. 14 October 2023; 134 (14): 144402. https://doi.org/10.1063/5.0169391
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