Magnetically ordered insulators are of key interest for spintronics applications, but most of them have not yet been explored in depth regarding their magnetic properties, in particular with respect to their dynamic response. We study the static and dynamic magnetic properties of epitaxially strained -Fe2O3 (maghemite) thin films grown via pulsed-laser deposition on MgO substrates by SQUID magnetometry and cryogenic broadband ferromagnetic resonance experiments. SQUID magnetometry measurements reveal hysteretic magnetization curves for magnetic fields applied both in- and out of the sample plane. From the magnetization dynamics of our thin films, we find a small negative effective magnetization in agreement with a strain induced perpendicular magnetic anisotropy. Moreover, we observe a non-linear evolution of the ferromagnetic resonance-linewidth as a function of the microwave frequency and explain this finding with the so-called slow relaxor model. We investigate the magnetization dynamics and non-linear damping mechanisms present in our samples as a function of frequency and temperature and in particular, observe a sign change in the effective magnetization from the transition of the magnetic anisotropy from a perpendicular easy axis to an easy in-plane anisotropy for reduced temperatures. Its nonlinear damping properties and strain-induced perpendicular anisotropy render -Fe2O3 an interesting material platform for spintronics devices.
Skip Nav Destination
Article navigation
21 December 2022
Research Article|
December 15 2022
Reduced effective magnetization and damping by slowly relaxing impurities in strained γ-Fe2O3 thin films
Manuel Müller
;
Manuel Müller
a)
(Conceptualization, Data curation, Formal analysis, Investigation, Methodology, Writing – original draft)
1
Walther-Meißner-Institut, Bayerische Akademie der Wissenschaften
, 85748 Garching, Germany
2
Physik-Department, Technische Universität München
, 85748 Garching, Germany
a)Author to whom correspondence should be addressed: manuel.mueller@wmi.badw.de
Search for other works by this author on:
Monika Scheufele
;
Monika Scheufele
(Data curation, Methodology, Writing – review & editing)
1
Walther-Meißner-Institut, Bayerische Akademie der Wissenschaften
, 85748 Garching, Germany
2
Physik-Department, Technische Universität München
, 85748 Garching, Germany
Search for other works by this author on:
Janine Gückelhorn
;
Janine Gückelhorn
(Methodology, Writing – review & editing)
1
Walther-Meißner-Institut, Bayerische Akademie der Wissenschaften
, 85748 Garching, Germany
2
Physik-Department, Technische Universität München
, 85748 Garching, Germany
Search for other works by this author on:
Luis Flacke
;
Luis Flacke
(Data curation, Writing – review & editing)
1
Walther-Meißner-Institut, Bayerische Akademie der Wissenschaften
, 85748 Garching, Germany
2
Physik-Department, Technische Universität München
, 85748 Garching, Germany
Search for other works by this author on:
Mathias Weiler
;
Mathias Weiler
(Data curation, Formal analysis, Writing – review & editing)
3
Fachbereich Physik and Landesforschungszentrum OPTIMAS, Technische Universität Kaiserslautern
, 67663 Kaiserslautern, Germany
Search for other works by this author on:
Hans Huebl
;
Hans Huebl
(Data curation, Formal analysis, Supervision, Writing – review & editing)
1
Walther-Meißner-Institut, Bayerische Akademie der Wissenschaften
, 85748 Garching, Germany
2
Physik-Department, Technische Universität München
, 85748 Garching, Germany
4
Munich Center for Quantum Science and Technology (MCQST)
, 80799 München, Germany
Search for other works by this author on:
Stephan Gepraegs
;
Stephan Gepraegs
(Conceptualization, Data curation, Formal analysis, Project administration, Supervision, Writing – review & editing)
1
Walther-Meißner-Institut, Bayerische Akademie der Wissenschaften
, 85748 Garching, Germany
Search for other works by this author on:
Rudolf Gross
;
Rudolf Gross
(Data curation, Formal analysis, Funding acquisition, Project administration, Writing – review & editing)
1
Walther-Meißner-Institut, Bayerische Akademie der Wissenschaften
, 85748 Garching, Germany
2
Physik-Department, Technische Universität München
, 85748 Garching, Germany
4
Munich Center for Quantum Science and Technology (MCQST)
, 80799 München, Germany
Search for other works by this author on:
Matthias Althammer
Matthias Althammer
b)
(Conceptualization, Data curation, Formal analysis, Funding acquisition, Project administration, Supervision, Writing – review & editing)
1
Walther-Meißner-Institut, Bayerische Akademie der Wissenschaften
, 85748 Garching, Germany
2
Physik-Department, Technische Universität München
, 85748 Garching, Germany
Search for other works by this author on:
a)Author to whom correspondence should be addressed: manuel.mueller@wmi.badw.de
J. Appl. Phys. 132, 233905 (2022)
Article history
Received:
September 29 2022
Accepted:
November 23 2022
Citation
Manuel Müller, Monika Scheufele, Janine Gückelhorn, Luis Flacke, Mathias Weiler, Hans Huebl, Stephan Gepraegs, Rudolf Gross, Matthias Althammer; Reduced effective magnetization and damping by slowly relaxing impurities in strained γ-Fe2O3 thin films. J. Appl. Phys. 21 December 2022; 132 (23): 233905. https://doi.org/10.1063/5.0128596
Download citation file:
Sign in
Don't already have an account? Register
Sign In
You could not be signed in. Please check your credentials and make sure you have an active account and try again.
Sign in via your Institution
Sign in via your InstitutionPay-Per-View Access
$40.00