We report the first example of magnetic pair distribution function (mPDF) data obtained through the use of neutron polarization analysis. Using the antiferromagnetic semiconductor MnTe as a test case, we present high-quality mPDF data collected on the HYSPEC instrument at the Spallation Neutron Source using longitudinal polarization analysis to isolate the magnetic scattering cross section. Clean mPDF patterns are obtained for MnTe in both the magnetically ordered state and the correlated paramagnet state, where only short-range magnetic order is present. We also demonstrate significant improvement in the quality of high-resolution mPDF data through the application of ad hoc corrections that require only minimal human input, minimizing potential sources of error in the data processing procedure. We briefly discuss the current limitations and future outlook of mPDF analysis using polarized neutrons. Overall, this work provides a useful benchmark for mPDF analysis using polarized neutrons and provides an encouraging picture of the potential for routine collection of high-quality mPDF data.
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14 December 2022
Research Article|
December 13 2022
Magnetic pair distribution function data using polarized neutrons and ad hoc corrections Available to Purchase
Benjamin A. Frandsen
;
Benjamin A. Frandsen
a)
(Conceptualization, Formal analysis, Funding acquisition, Investigation, Methodology, Project administration, Software, Supervision, Writing – original draft, Writing – review & editing)
1
Department of Physics and Astronomy, Brigham Young University
, Provo, Utah 84602, USA
a)Author to whom correspondence should be addressed: [email protected]
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Raju Baral
;
Raju Baral
(Investigation, Methodology)
1
Department of Physics and Astronomy, Brigham Young University
, Provo, Utah 84602, USA
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Barry Winn
;
Barry Winn
(Data curation)
2
Neutron Scattering Division, Oak Ridge National Laboratory
, Oak Ridge, Tennessee 37831, USA
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V. Ovidiu Garlea
V. Ovidiu Garlea
(Data curation, Writing – review & editing)
2
Neutron Scattering Division, Oak Ridge National Laboratory
, Oak Ridge, Tennessee 37831, USA
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Benjamin A. Frandsen
1,a)
Raju Baral
1
Barry Winn
2
V. Ovidiu Garlea
2
1
Department of Physics and Astronomy, Brigham Young University
, Provo, Utah 84602, USA
2
Neutron Scattering Division, Oak Ridge National Laboratory
, Oak Ridge, Tennessee 37831, USA
a)Author to whom correspondence should be addressed: [email protected]
J. Appl. Phys. 132, 223909 (2022)
Article history
Received:
October 11 2022
Accepted:
November 27 2022
Citation
Benjamin A. Frandsen, Raju Baral, Barry Winn, V. Ovidiu Garlea; Magnetic pair distribution function data using polarized neutrons and ad hoc corrections. J. Appl. Phys. 14 December 2022; 132 (22): 223909. https://doi.org/10.1063/5.0130400
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