Plasmonic nanostructures attract tremendous attention as they confine electromagnetic fields well below the diffraction limit while simultaneously sustaining extreme local field enhancements. To fully exploit these properties, the identification and classification of resonances in such nanostructures is crucial. Recently, a novel figure of merit for resonance classification has been proposed [Müller et al., J. Phys. Chem. C 124, 24331–24343 (2020)] and its applicability was demonstrated mostly to toy model systems. This novel measure, the energy-based plasmonicity index (EPI), characterizes the nature of resonances in molecular nanostructures. The EPI distinguishes between either a single-particle-like or a plasmonic nature of resonances based on the energy space coherence dynamics of the excitation. To advance the further development of this newly established measure, we present here its exemplary application to characterize the resonances of graphene nanoantennas. In particular, we focus on resonances in a doped nanoantenna. The structure is of interest, as a consideration of the electron dynamics in real space might suggest a plasmonic nature of selected resonances in the low doping limit but our analysis reveals the opposite. We find that in the undoped and moderately doped nanoantenna, the EPI classifies all emerging resonances as predominantly single-particle-like, and only after doping the structure heavily, the EPI observes plasmonic response.
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7 March 2021
Research Article|
March 04 2021
From single-particle-like to interaction-mediated plasmonic resonances in graphene nanoantennas
Special Collection:
Plasmonics: Enabling Functionalities with Novel Materials
Marvin M. Müller
;
Marvin M. Müller
a)
1
Institute of Theoretical Solid State Physics, Karlsruhe Institute of Technology (KIT)
, 76131 Karlsruhe, Germany
a)Author to whom correspondence should be addressed: marvin.mueller@kit.edu
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Miriam Kosik
;
Miriam Kosik
b)
2
Institute of Physics, Nicolaus Copernicus University in Toruń
, Grudziadzka 5, 87-100 Toruń, Poland
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Marta Pelc
;
Marta Pelc
2
Institute of Physics, Nicolaus Copernicus University in Toruń
, Grudziadzka 5, 87-100 Toruń, Poland
3
Donostia International Physics Center (DIPC)
, Paseo Manuel Lardizabal 4, 20018 Donostia-San Sebastián, Spain
4
Centro de Física de Materiales, CFM-MPC CSIC-UPV/EHU
, Paseo Manuel Lardizabal 5, 20018 Donostia-San Sebastián, Spain
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Garnett W. Bryant
;
Garnett W. Bryant
5
Joint Quantum Institute, University of Maryland and National Institute of Standards and Technology
, College Park, Maryland 20742, USA
6
Nanoscale Device Characterization Division, National Institute of Standards and Technology
, Gaithersburg, Maryland 20899, USA
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Andrés Ayuela
;
Andrés Ayuela
3
Donostia International Physics Center (DIPC)
, Paseo Manuel Lardizabal 4, 20018 Donostia-San Sebastián, Spain
4
Centro de Física de Materiales, CFM-MPC CSIC-UPV/EHU
, Paseo Manuel Lardizabal 5, 20018 Donostia-San Sebastián, Spain
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Carsten Rockstuhl
;
Carsten Rockstuhl
1
Institute of Theoretical Solid State Physics, Karlsruhe Institute of Technology (KIT)
, 76131 Karlsruhe, Germany
7
Institute of Nanotechnology, Karlsruhe Institute of Technology (KIT)
, 76021 Karlsruhe, Germany
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Karolina Słowik
Karolina Słowik
2
Institute of Physics, Nicolaus Copernicus University in Toruń
, Grudziadzka 5, 87-100 Toruń, Poland
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a)Author to whom correspondence should be addressed: marvin.mueller@kit.edu
b)
Electronic mail: mkosik@doktorant.umk.pl
Note: This paper is part of the Special Topic on Plasmonics: Enabling Functionalities with Novel Materials.
J. Appl. Phys. 129, 093103 (2021)
Article history
Received:
November 27 2020
Accepted:
February 12 2021
Citation
Marvin M. Müller, Miriam Kosik, Marta Pelc, Garnett W. Bryant, Andrés Ayuela, Carsten Rockstuhl, Karolina Słowik; From single-particle-like to interaction-mediated plasmonic resonances in graphene nanoantennas. J. Appl. Phys. 7 March 2021; 129 (9): 093103. https://doi.org/10.1063/5.0038883
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