We present a theoretical formulation of the frequency domain multidimensional pump-probe analog spectroscopy, which utilizes the spectral–temporal entanglement features of the biphoton sources. It has been shown, via a compact multi-time, convolutional Green’s function expression and the accompanying numerical simulations, that utilizing the correlation properties of non-classical sources offers a viable scheme for the exploration of dissipative kinetics of the cavity confined quantum aggregates. The cooperative and competitive modifications brought in by the photonic cavity mode and the auxiliary vibrational modes into the scattering and dephasing properties of the exciton–polaritons have been explored via their signatures in the multidimensional correlation maps. The study offers a new parameter window for the investigation of the dynamical polariton characteristics and warrants the usage of multi-mode entanglement properties of the external photonic sources in future studies.
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21 September 2020
Research Article|
September 18 2020
Entangled photon assisted multidimensional nonlinear optics of exciton–polaritons
Special Collection:
Materials for Quantum Technologies: Computing, Information, and Sensing
Arunangshu Debnath
;
Arunangshu Debnath
a)
1
Max Planck Institute for the Structure and Dynamics of Matter and Center for Free-Electron Laser Science
, Luruper Chaussee 149, 22761 Hamburg, Germany
a)Author to whom correspondence should be addressed: arunangshu.debnath@desy.de
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Angel Rubio
Angel Rubio
b)
1
Max Planck Institute for the Structure and Dynamics of Matter and Center for Free-Electron Laser Science
, Luruper Chaussee 149, 22761 Hamburg, Germany
2
Center for Computational Quantum Physics (CCQ), The Flatiron Institute
, 162 Fifth Avenue, New York, New York 10010, USA
Search for other works by this author on:
a)Author to whom correspondence should be addressed: arunangshu.debnath@desy.de
b)
Electronic mail: angel.rubio@mpsd.mpg.de
Note: This paper is part of the special collection on Materials for Quantum Technologies: Computing, Information, and Sensing.
J. Appl. Phys. 128, 113102 (2020)
Article history
Received:
May 04 2020
Accepted:
September 03 2020
Citation
Arunangshu Debnath, Angel Rubio; Entangled photon assisted multidimensional nonlinear optics of exciton–polaritons. J. Appl. Phys. 21 September 2020; 128 (11): 113102. https://doi.org/10.1063/5.0012754
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