Thermophysical characterization of graphene is very important for both fundamental and technological research. While most of the existing thermal conductivity measurements are for graphene sheets with sizes larger than 1 μm, the thermal conductivities for suspended submicron graphene ribbons are still very few, although the thermal conductivity of graphene ribbons at the submicron scale is predicted to be much smaller than large graphene and strongly size dependent for both length and width due to the 2D nature of phonon transport. Here, we report the temperature dependent thermal conductivity of a 169-nm wide and 846-nm long graphene ribbon measured by the electrical self-heating method. The measured thermal conductivities range from (12.7 ± 2.95) W/m/K at 80 K to (932 ± 333) W/m/K at 380 K, being (349 ± 63) W/m/K at 300 K, following a ∼ T2.79 law for the full temperature range of 80 K to 380 K and a ∼ T1.23 law at low temperatures. The comparison of the measured thermal conductance with the ballistic transport limit indicates diffusive transport in this narrow and short ribbon due to phonon-edge as well as phonon-defect scattering. The data were also combined with an empirical model to predict possible width dependence of thermal conductivity for suspended graphene ribbons. These results help understand the 2D phonon transport in suspended submicron graphene ribbons and provide knowledge for controlling thermophysical properties of suspended graphene nanoribbons through size manipulation.
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14 February 2015
Research Article|
February 10 2015
Temperature dependent thermal conductivity of a suspended submicron graphene ribbon
Qin-Yi Li
;
Qin-Yi Li
1Key Laboratory for Thermal Science and Power Engineering of Ministry of Education, Department of Engineering Mechanics,
Tsinghua University
, Beijing 100084, China
2International Institute for Carbon Neutral Energy Research (WPI-I2CNER),
Kyushu University
, 744 Moto-oka, Nishi-ku, Fukuoka 819-0395, Japan
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Koji Takahashi;
Koji Takahashi
2International Institute for Carbon Neutral Energy Research (WPI-I2CNER),
Kyushu University
, 744 Moto-oka, Nishi-ku, Fukuoka 819-0395, Japan
3Department of Aeronautics and Astronautics,
Kyushu University
, Fukuoka 819-0395, Japan
4JST, CREST,
Kyushu University
, Fukuoka 819-0395, Japan
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Hiroki Ago;
Hiroki Ago
5Institute for Material Chemistry and Engineering,
Kyushu University
, Fukuoka 816-8508, Japan
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Xing Zhang;
Xing Zhang
a)
1Key Laboratory for Thermal Science and Power Engineering of Ministry of Education, Department of Engineering Mechanics,
Tsinghua University
, Beijing 100084, China
2International Institute for Carbon Neutral Energy Research (WPI-I2CNER),
Kyushu University
, 744 Moto-oka, Nishi-ku, Fukuoka 819-0395, Japan
4JST, CREST,
Kyushu University
, Fukuoka 819-0395, Japan
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Tatsuya Ikuta;
Tatsuya Ikuta
3Department of Aeronautics and Astronautics,
Kyushu University
, Fukuoka 819-0395, Japan
4JST, CREST,
Kyushu University
, Fukuoka 819-0395, Japan
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Takashi Nishiyama;
Takashi Nishiyama
3Department of Aeronautics and Astronautics,
Kyushu University
, Fukuoka 819-0395, Japan
4JST, CREST,
Kyushu University
, Fukuoka 819-0395, Japan
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Kenji Kawahara
Kenji Kawahara
5Institute for Material Chemistry and Engineering,
Kyushu University
, Fukuoka 816-8508, Japan
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a)
Author to whom correspondence should be addressed. Electronic mail: x-zhang@tsinghua.edu.cn. Tel./Fax: 86-10-62772668.
J. Appl. Phys. 117, 065102 (2015)
Article history
Received:
January 04 2015
Accepted:
January 24 2015
Citation
Qin-Yi Li, Koji Takahashi, Hiroki Ago, Xing Zhang, Tatsuya Ikuta, Takashi Nishiyama, Kenji Kawahara; Temperature dependent thermal conductivity of a suspended submicron graphene ribbon. J. Appl. Phys. 14 February 2015; 117 (6): 065102. https://doi.org/10.1063/1.4907699
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