Graphene deposited on planar surfaces often exhibits sharp and localized folds delimiting seemingly planar regions, as a result of compressive stresses transmitted by the substrate. Such folds alter the electronic and chemical properties of graphene, and therefore, it is important to understand their emergence, to either suppress them or control their morphology. Here, we study the emergence of out-of-plane deformations in supported and laterally strained graphene with high-fidelity simulations and a simpler theoretical model. We characterize the onset of buckling and the nonlinear behavior after the instability in terms of the adhesion and frictional material parameters of the graphene-substrate interface. We find that localized folds evolve from a distributed wrinkling linear instability due to the nonlinearity in the van der Waals graphene-substrate interactions. We identify friction as a selection mechanism for the separation between folds, as the formation of far apart folds is penalized by the work of friction. Our systematic analysis is a first step towards strain engineering of supported graphene, and is applicable to other compressed thin elastic films weakly coupled to a substrate.
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21 May 2013
Research Article|
May 15 2013
Adhesion and friction control localized folding in supported graphene
K. Zhang;
K. Zhang
LaCàN, Universitat Politècnica de Catalunya-BarcelonaTech (UPC)
, Barcelona 08034, Spain
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Electronic mail: marino.arroyo@upc.edu
J. Appl. Phys. 113, 193501 (2013)
Article history
Received:
March 21 2013
Accepted:
April 22 2013
Citation
K. Zhang, M. Arroyo; Adhesion and friction control localized folding in supported graphene. J. Appl. Phys. 21 May 2013; 113 (19): 193501. https://doi.org/10.1063/1.4804265
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