Fe50Pt50−xRhx films have attracted much interest recently due to their potential usage in heat assisted magnetic recording media and the ferromagnetic (FM) to antiferromagnetic (AFM) transition as Rh concentration is increased. In this study, we present an investigation of the spin moment (ms) and orbital moment (ml) of Fe in Fe50Pt50−xRhx films using x-ray magnetic circular dichroism. The measurements were made in the soft x-ray region along the film normal, which corresponds to the easy axis of the (001) textured L10 FePt with uni-axial magnetic anisotropy. They show that the magnetic moment of Fe mainly contributes to the whole magnetization of the films. The decrease of ml with Rh doping concentration implies a decrease of magneto-crystalline anisotropy, whereas the significant decrease of ms is consistent with the FM to AFM transition at above 15 at. % of Rh.

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