The frequency and temperature dependences of the magnetic susceptibility and the ac electrical conductivity in magnetoelectric were investigated. The zero-field-cooled-field-heated magnetic susceptibility reveals phase transitions at 14.2 and 36.6 K. The phase below 36.6 K is ferromagnetic. At temperatures below 200 K, the ac conductivity and dielectric constant follow the universal dielectric response (UDR), being typical for hopping or tunneling of localized charge carriers. A detailed analysis of the temperature dependence of the UDR parameter in terms of the theoretical model for tunneling of small polarons revealed that below 200 K, this mechanism governs the charge transport in the magnetoelectric fluoride system.
REFERENCES
1.
D.
Emin
, Phys. Rev. B
48
, 13691
(1993
).2.
S.
Bhattacharya
and A.
Ghosh
, Phys. Rev. B
68
, 224202
(2003
).3.
C.
Hartinger
, F.
Mayr
, A.
Loidl
, and T.
Kopp
, Phys. Rev. B
73
, 024408
(2006
).4.
Ch.
Jooss
, L.
Wu
, T.
Beetz
, R. F.
Klie
, M.
Beleggia
, M. A.
Schofield
, S.
Schramm
, J.
Hoffmann
, and Y.
Zhu
, Proc. Natl. Acad. Sci. U.S.A.
104
, 13597
(2007
).5.
J.
Geck
, P.
Wochner
, S.
Kiele
, R.
Klingeler
, P.
Reutler
, A.
Revcolevschi
, and B.
Buchner
, Phys. Rev. Lett.
95
, 236401
(2005
).6.
A.
Levstik
, C.
Filipič
, V.
Bobnar
, G.
Tavčar
, and B.
Žemva
, Europhys. Lett.
83
, 27001
(2008
).7.
R.
Blinc
, G.
Tavčar
, B.
Žemva
, D.
Hanžel
, P.
Cevc
, C.
Filipič
, A.
Levstik
, Z.
Jagličić
, Z.
Trontelj
, N.
Dalal
, V.
Ramachandran
, S.
Nellutla
, and J. F.
Scott
, J. Appl. Phys.
103
, 074114
(2008
).8.
N. F.
Mott
and E. A.
Davis
, Electronic Processes in Non- Crystalline Materials
(Oxford University Press
, New York
, 1979
).9.
M.
Dumm
, P.
Lunkenheimer
, A.
Loidl
, B.
Assmann
, H.
Homborg
, and P.
Fulde
, J. Chem. Phys.
104
, 5048
(1996
).10.
B. I.
Shklovskii
and A. L.
Efros
, Electronic Properties of Doped Semiconductors
(Springer-Verlag
, Berlin
, 1984
).11.
A.
Ghosh
, Phys. Rev. B
41
, 1479
(1990
).12.
A.
Ghosh
, Phys. Rev. B
42
, 1388
(1990
).13.
A.
Ghosh
, Phys. Rev. B
42
, 5665
(1990
).14.
15.
R. D.
Gould
and A. K.
Hasan
, Thin Solid Films
223
, 334
(1993
).16.
J.
Sichelschmidt
, M.
Paraskevopoulos
, T.
Brando
, R.
Wehn
, D.
Ivannikov
, F.
Mayr
, K.
Pucher
, J.
Hemberger
, A.
Pimenov
, H. -A.
Krug von Nidda
, P.
Lunkenheimer
, V. Yu.
Ivanov
, A. A.
Mukhin
, A. M.
Balbashov
, and A.
Loidl
, Eur. Phys. J. B
20
, 7
(2001
).17.
S. R.
Elliott
, Adv. Phys.
36
, 135
(1987
).18.
M. P. J.
van Staveren
, H. B.
Brom
, and L. J.
de Jongh
, Phys. Rep.
208
, 1
(1991
).© 2009 American Institute of Physics.
2009
American Institute of Physics
You do not currently have access to this content.