We report the ultrafast switching of the magnetic state in the course of photoinduced phase transition from an insulator with short-range charge and orbital order (CO/OO) to a ferromagnetic metal in perovskite-type Gd0.55Sr0.45MnO3. The femtosecond Kerr rotation and reflectivity measurements, which detect the spin and charge dynamics, respectively, have revealed that the metallic state is formed within the time resolution (200fs); however, magnetization increases with the time constant of 0.5ps. The relatively slow increase of the magnetization is attributable to the magnetic-field-induced alignment of ferromagnetic domains in the initially produced metallic state.

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