Here, we report the characterization of the transport of micro- and nanospheres in a simple two-dimensional square nanoscale plasmonic optical lattice. The optical potential was created by exciting plasmon resonance by way of illuminating an array of gold nanodiscs with a loosely focused Gaussian beam. This optical potential produced both in-lattice particle transport behavior, which was due to near-field optical gradient forces, and high-velocity (∼μm/s) out-of-lattice particle transport. As a comparison, the natural convection velocity field from a delocalized temperature profile produced by the photothermal heating of the nanoplasmonic array was computed in numerical simulations. This work elucidates the role of photothermal effects on micro- and nanoparticle transport in plasmonic optical lattices.

1.
A.
Ashkin
,
J. M.
Dziedzic
,
J. E.
Bjorkholm
, and
S.
Chu
,
Opt. Lett.
11
,
288
(
1986
).
3.
M. L.
Juan
,
M.
Righini
, and
R.
Quidant
,
Nat. Photonics
5
,
349
(
2011
).
4.
T.
Shoji
and
Y.
Tsuboi
,
J. Phys. Chem. Lett.
5
,
2957
(
2014
).
5.
J. S.
Huang
and
Y. T.
Yang
,
Nanomaterials
5
,
1048
(
2015
).
6.
W. H.
Wright
,
G. J.
Sonek
, and
M. W.
Berns
,
Appl. Rev. Lett.
63
,
715
(
1993
).
7.
G.
Volpe
,
R.
Quidant
,
G.
Badenes
, and
D.
Petrov
,
Phys. Rev. Lett.
96
,
238101
(
2006
).
8.
M.
Righini
,
A. S.
Zelenina
,
C.
Girard
, and
R.
Quidant
,
Nat. Phys.
3
,
477
(
2007
).
9.
M.
Righini
,
G.
Volpe
,
C.
Girard
,
D.
Petrov
, and
R.
Quidant
,
Phys. Rev. Lett.
100
,
186804
(
2008
).
10.
T.
Shoji
 et al.,
J. Am. Chem. Soc.
135
,
6643
(
2013
).
11.
Y.
Pang
and
R.
Gordon
,
Nano Lett.
12
,
402
(
2012
).
12.
A.
Kotnala
and
R.
Gordon
,
Biomed. Opt. Express
5
,
1886
(
2014
).
13.
A. A.
Al Balushi
and
R.
Gordon
,
ACS Photonics
1
,
389
(
2014
).
14.
A. A.
Al Balushi
and
R.
Gordon
,
Nano Lett.
14
,
5787
(
2014
).
15.
S.
Wheaton
,
R. M.
Gelfand
, and
R.
Gordon
,
Nat. Photonics
9
,
68
(
2015
).
16.
P. T.
Korda
,
M. B.
Taylor
, and
D. G.
Grier
,
Phys. Rev. Lett.
89
,
128301
(
2002
).
17.
K.
Ladavac
,
K.
Kasza
, and
D. G.
Grier
,
Phys. Rev. E.
70
,
010901
(
2004
).
18.
G. C.
MacDonald
,
G. C.
Spalding
, and
K.
Dholakia
,
Nature
426
,
421
(
2003
).
19.
A.
Cuche
,
B.
Stein
,
A.
Canguier-Durand
,
E.
Devaux
,
C.
Genet
, and
T. W.
Ebbesen
,
Nano Lett.
12
,
4329
(
2012
).
20.
K. Y.
Chen
,
A. T.
Lee
,
C. C.
Hung
,
J. S.
Huang
, and
Y. T.
Yang
,
Nano Lett.
13
,
4118
(
2013
).
21.
G.
Baffou
,
R.
Quidant
, and
J. F.
Garcia de Abajo
,
ACS Nano
4
,
709
(
2010
).
22.
G.
Baffou
,
R.
Quidant
, and
C.
Girad
,
Phys. Rev. B
82
,
165424
(
2010
).
23.
J. S.
Donner
,
G.
Baffou
,
D.
McCloskey
, and
R.
Quidant
,
ACS Nano
5
,
5457
(
2011
).
24.
G.
Baffou
 et al.,
ACS Nano
7
,
6478
(
2013
).
25.
B. J.
Roxworthy
,
A. M.
Bhuiya
,
S. P.
Vanka
, and
K. C.
Toussant
, Jr.
,
Nat. Commun.
5
,
3173
(
2014
).
26.
B. J.
Roxworthy
,
K. D.
Ko
,
A.
Kumar
,
K. H.
Fung
,
E. K. C.
Chow
,
G. L.
Liu
,
N. X.
Fang
, and
K. C.
Toussaint
, Jr.
,
Nano Lett.
12
,
796
(
2012
).
27.
J. C.
Ndukaife
 et al.,
ACS Nano
8
,
9035
(
2014
).
28.
M.
Pelton
,
K.
Ladavac
, and
D.
Grier
,
Phys. Rev. E
70
,
031108
(
2004
).
29.
See supplementary material at http://dx.doi.org/10.1063/1.4948775 for Matlab codes and additional data.
30.
D.
Ross
,
M.
Gaitan
, and
L. E.
Locascio
,
Anal. Chem.
73
,
4117
(
2001
).
31.
F. P.
Incropera
and
D. P.
DeWitt
,
Fundamentals of Heat and Mass Transfer
, 4th ed. (
John Wiley & Sons
,
New York
,
1996
).
32.
F.
Reif
,
Fundamentals of Statistical and Thermal Physics
, 1st ed. (
McGraw-Hill
,
New York
,
1965
).
33.
A.
Pralle
,
E.-L.
Florin
,
E. H. K.
Stelzer
, and
J. K. H.
Hörber
,
Appl. Phys. A
66
,
S71
(
1998
).
34.
J.
Happel
and
H.
Brenner
,
Low Reynolds Number Hydrodynamics
(
Kluwer
,
Dordrecht
,
1991
).
35.
J.
Kestin
,
M.
Sokolv
, and
W. A.
Wakeham
,
J. Phys. Chem. Ref. Data
7
,
941
(
1978
).
36.
S.
Kawata
and
T.
Sugirua
,
Opt. Lett.
17
,
772
774
(
1992
).
37.
H.
Kim
 et al.,
J. Appl. Phys.
86
,
6451
6461
(
1999
).
38.
A.
Yariv
,
Quantum Electronics
(
John Wiley & Sons
,
New York
,
1988
).
39.
S.
Murai
,
M. A.
Verschuuren
,
G.
Lozano
,
G.
Pirruccio
,
S. R. K.
Rodriguez
, and
J.
Gómez Rivas
,
Opt. Express
21
,
4250
4262
(
2013
).
40.
S.
Jane Flint
,
W.
Enquist
,
V. R.
Racaniello
, and
A. M.
Skalka
,
Principles of Virology
(
ASM Press
,
Washington
,
2009
).
41.
E.
Van der Pol
,
A. N.
Böing
,
P.
Harrison
,
A.
Sturk
, and
R.
Nieuwland
,
Pharm. Rev.
64
,
676
705
(
2012
).
42.
M. D.
Ooms
,
L.
Bajin
, and
D.
Sinton
,
Appl. Phys. Lett.
101
,
253701
(
2012
).
43.
D.
Erickson
,
D.
Sinton
, and
D.
Psaltis
,
Nat. Photonics
5
,
583
590
(
2011
).
44.
R. A.
Anderson
,
Algal Culturing Technique
, 1st ed. (
Academic Press
,
London
,
2005
).
45.
K.
Wang
,
E.
Schonbrun
,
P.
Steinvurzel
, and
K. B.
Crozier
,
Nat. Commun.
2
,
469
(
2011
).

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