Optical fibers are an excellent sensor platform. However, the detection and analysis of media outside the cladding and coating of standard fibers represent a long-standing challenge: light that is guided in the single optical core mode does not reach these media. Cladding modes help work around this difficulty, as their transverse profiles span the entire cross-section of the fiber cladding and reach its outer boundary. In this tutorial, we introduce and discuss in detail two recent advances in optical fiber sensors that make use of cladding modes. Both concepts share optomechanics as a common underlying theme. First, we describe a spatially continuous distributed analysis using the optical cladding modes of the fiber. Light is coupled to these modes using Brillouin dynamic gratings, which are index perturbations associated with acoustic waves in the core that are stimulated by light. Unlike permanent gratings, which are routinely used to couple light with cladding modes, Brillouin dynamic gratings may be switched on and off at will and can be confined to short fiber sections at arbitrary locations in a random-access manner. Second, we present the extension of the cladding mode sensor concept to include acoustic rather than optical modes. The acoustic cladding modes may be stimulated and monitored by guided light in the single core mode, and their linewidths are modified by the elastic properties of surrounding media. The principles and analyses of both concepts are provided in detail, alongside examples of experimental setups and results.
I. INTRODUCTION
Standard optical fibers constitute an exceptional sensing platform.1–4 Their low cost and low propagation losses allow for installation over long reaches and for remote measurements from a long stand-off distance. Their small cross-section permits their installation within many structures with little disruption of function. Fibers are comparatively immune to electromagnetic interference, and they are suitable for installation in harsh and hazardous environments where the use of electricity might be prohibited. In addition, optical fibers support spatially continuous distributed analysis, in which each fiber section becomes an independent node in a sensor network.5 Optical fiber sensors have, therefore, been studied and employed for almost fifty years.
Most sensors over standard, single-mode optical fibers observe the effect of a quantity of interest on the light that is guided in the core of the fiber. Examples include the monitoring of temperature, static strain, sound and vibrations, electrical and magnetic fields, gamma radiation, and more.1–5 The condition being observed may alter the magnitude, frequency, phase, or polarization of guided light, and those changes in turn may vary with the optical frequency.1–5 Optical fiber sensors progress rapidly and become increasingly sensitive, sophisticated, and useful. However, the fundamental sensing configuration over single-mode fibers faces a significant limitation: the condition being observed must prevail in spatial overlap with the inner core. While this requirement is more easily fulfilled in the measurements of temperature and axial strain, for example, it restricts the detection and sensing of media outside the boundaries of the fiber cladding and coating. The optical fiber sensing of chemical reagents and biological species represents an inherent, long-standing difficulty.
Over the last decades, a large number of clever, sensitive, and target-specific optical fiber sensors for the analysis of outside media have nevertheless been proposed, demonstrated, and successfully employed. For an excellent review, see Ref. 6. The sensing concepts may be broadly classified into several categories. One useful approach is that of indirect sensing, in which a transduction mechanism converts the presence or concentration of a target reagent to a secondary signal that may be picked up by light in the core of the fiber, most often a change in temperature or strain.6 Although the sensors directly measure modifications induced within the core, they may indirectly identify conditions prevailing outside the cladding or coating. An example of indirect sensing is the monitoring of hydrogen through strain induced by the swelling of palladium coating layers.7 In many cases, the implementation of the transduction mechanism requires local modifications, and it is difficult to scale to long distances and spatially distributed analysis.
A second category relies on structural modifications to the standard fiber geometry that bring the guided light into direct spatial overlap with the medium under test. Modifications may take the form of etching, tapering, cleaving of facets, the formation of through holes, and more.6–14 This strategy can be very effective. However, similar to most indirect approaches, it is difficult to scale beyond point-measurements at a few discrete and pre-selected locations. A third approach is based on moving away from the standard single-mode fiber altogether. Instead, sensors are implemented in non-standard cross-sections, such as photonic crystals and nano-structured fibers,15–19 in which test liquids and gases may flow through holes. Alternatively, the fiber can be made of reactive, biologically sensitive materials instead of silica.20–23 The lengths of non-standard fibers are sometimes limited, and their availability to the broader community can be restricted as well.
All sensing approaches described earlier rely on the propagation of light in the fundamental, single optical core-mode supported by the fiber. However, the transverse profiles of standard fibers also support a large category of so-called cladding modes. These include optical cladding modes that guide light24–29 as well as mechanical (acoustic) cladding modes for the propagation of elastic perturbations.30–33 Unlike the single optical core mode, the transverse profiles of both optical and acoustic cladding modes span the entire cross-section of the fiber cladding and reach its outer boundaries. Therefore, the propagation of optical and/or acoustic waves in the cladding modes of the fiber provides unique opportunities for the sensing of outside media beyond those available through the optical core mode.
Of the two categories of cladding modes, the optical ones are much better known in the fiber-optics community. While these modes represent a distraction from a telecommunication standpoint, their potential in fiber sensing applications is widely recognized and employed. The transverse profiles of the optical cladding modes include evanescent tails, which may overlap with the media under test. Therefore, the coupling of light to the cladding modes and the propagation in these modes may be affected by the properties of outside substances. Cladding-mode-based sensors have been used in thousands of works over the past thirty years.24,26–28
The main challenge associated with optical cladding mode sensors revolves around the coupling of light to and from the single optical core mode. In most cases, light is launched and collected at the ends of the fiber in the single core mode only. Coupling to the cladding modes takes place along the fiber through the inscription of permanent gratings in the core.24,25,29,34,35 Short period gratings can couple light between a core mode and a counter-propagating cladding mode.24,25,29 Long-period gratings can do the same between co-propagating core and cladding modes.25,29 However, gratings are implemented in discrete, specific locations. As a result, cladding-mode sensors that are based on grating interfaces provide point measurements only. The sensors can be cascaded to form quasi-distributed networks; however, their extension toward spatially continuous distributed analysis is inherently difficult.
The acoustic cladding modes of standard optical fibers have been analyzed and characterized experimentally for the first time in 1985.30 Like their optical counterparts, the transverse profiles of acoustic cladding modes reach the outer boundary of the cladding, and their propagation may be affected by outside conditions. Compared with optical cladding modes, optical fiber sensing through guided acoustic modes is difficult to carry out directly: acoustic waves in fibers are seldom launched or detected in the mechanical domain, as interfaces at the ends of the fibers are optical. Instead, acoustic waves in fibers can be stimulated by guided optical waves through electrostriction and may be monitored based on photoelastic scattering of light.30–33,36,37
The combination of electrostriction and/or photoelasticity, often referred to as Brillouin scattering in fibers,36,37 is highly useful for the indirect sensing of parameters of interest based on their effect on acoustic waves, which serve as mediators. This prospect is best realized in backward Brillouin scattering optical fiber sensors, which are successfully commercialized for spatially distributed measurements of temperature and strain.5,38 However, the acoustic modes involved in traditional backward Brillouin scattering sensors are guided by the core of the fiber, similar to the single optical core mode. These sensors are, therefore, not suitable for the analysis of media outside the cladding. The potential of Brillouin scattering processes involving acoustic cladding modes toward sensing applications has not been considered until recently.
This tutorial is intended to introduce and describe two recent developments in the field of optical fiber sensing, which share the use of guided cladding modes and opto-mechanical interactions as common themes. One concept is based on the coupling spectra of light between the optical core mode and an optical cladding mode.39,40 Unlike established sensing protocols based on optical cladding modes, the coupling of light to these modes does not rely on the inscription of permanent gratings. Instead, the coupling is realized by photoelastic perturbations that are induced through a backward Brillouin scattering process in the core mode.41,42 The second concept involves the guided acoustic cladding modes of the fiber.43–54 These modes are stimulated and monitored by guided light in the core mode, and their oscillations indirectly convey information regarding conditions outside the cladding.43–54
In contrast to most traditional strategies for sensing chemicals using optical fibers, the two concepts are realized over standard, unmodified single-mode fibers. Both methods are suitable for spatially continuous distributed analysis, and both also support operation in fibers with certain types of coatings. Brought together, the new sensors allow for monitoring the optical and elastic properties of media where light in the core mode does not reach, thereby addressing long-standing challenges. Current performance, in terms of the number of resolution points, measurement range, sensitivity, and specificity, remains modest. Yet the measurement protocols hold much promise for further progress. We hope the following will help researchers and engineers working in fiber optics become familiar with these developments.
II. CLADDING MODES OF STANDARD OPTICAL FIBERS
The cross-section of standard optical fibers used in cladding mode sensing experiments consists of three distinct regions: an inner core of few-micrometers radius made of germanium-doped silica, a pure silica cladding with a standard diameter of 125 µm, and a protective polymer coating with thickness between a few micrometers and tens of micrometers [see Fig. 1(a)]. The fiber is placed in a medium under test, which is assumed to extend infinitely. Cladding modes are guided along the fiber axis due to the index contrast between the cladding and coating and the surrounding environment. Guiding requires that the refractive index of the coating ncoat be lower than that of pure silica, nSiO2 = 1.444 refractive index units (RIU) at 1550 nm wavelength, and that optical absorption in the coating not be exceedingly high within one resolution cell.
(a): Illustration of the transverse cross-section of a standard, coated step-index fiber in an infinite external medium. (b) Illustration of the three-layer model used in analysis. The medium outside the cladding is taken to be infinite and uniform (see text). The refractive indices of the core, cladding, coating, and outside medium are noted by ncore, nSiO2, ncoat, and next, respectively.
(a): Illustration of the transverse cross-section of a standard, coated step-index fiber in an infinite external medium. (b) Illustration of the three-layer model used in analysis. The medium outside the cladding is taken to be infinite and uniform (see text). The refractive indices of the core, cladding, coating, and outside medium are noted by ncore, nSiO2, ncoat, and next, respectively.
Unfortunately, many of the standard coating layers, such as the most common acrylate layers, are characterized by ncoat > nSiO2. This condition is beneficial for telecommunications and is, therefore, the norm in commercial fiber. Such coating layers must be removed for cladding modes to be guided. Certain types of polymers were developed to serve as secondary claddings with a refractive index below that of silica.55 Fibers coated with these polymers support the propagation of cladding modes and may be used for sensing purposes with their coating intact. Examples shown later in this tutorial make use of fluoroacrylate coating layers with an ncoat of 1.405 RIU.55 It is assumed below that the refractive index next of the medium outside the coating is lower than ncoat.
The analysis and modeling of cladding mode sensors are based on calculations of the normalized transverse profiles and effective indices of the cladding modes. In the most general case, the electromagnetic wave equation needs to be solved in four distinct domains: core, cladding, coating, and outside medium, and the boundary conditions at the three interfaces between adjacent domains must be satisfied. Yet, simplifying assumptions will be made for the purpose of this discussion. As explained below, these assumptions do not compromise the validity of the analysis for cases of practical interest. The reader is referred to earlier literature for a more complete analysis.25
Let us consider the functional form of the optical field transverse profile within the coating layer. If the effective index of a cladding mode neff is higher than ncoat, the modal profile decays exponentially within the coating. Decay takes place typically at sub-micron depths. Therefore, the evanescent tails of this category of modes do not reach into the surrounding medium, even for the thinnest of polymer coatings. If instead neff < ncoat, the cladding mode profile is oscillating across the coating layer and reaches into the outside substance. In principle, this latter category of optical cladding modes could have a large advantage in chemical sensing.
However, the contrast in refractive indices between nSiO2 and ncoat is comparatively large: about 0.04 RIU in the above-mentioned example. Consequently, the order m of cladding modes for which neff < ncoat is high: several tens or even higher. The transverse profiles of these very high-order modes oscillate rapidly across the silica cladding and even within the small inner core. Due to these rapid radial oscillations, the spatial overlap between the transverse profiles of these high-order cladding modes and the single core mode cancels out almost entirely. As will be discussed in Sec. III, such overlap is essential for the coupling of light between core and cladding modes. Therefore, in most practical scenarios with coated fibers, the cladding modes that reach outside the coating remain largely inaccessible. We, therefore, restrict the analysis to cladding modes for which neff > ncoat.
Referring again to the fluoroacrylate coating, the cladding modes with the largest spatial overlap with the core mode decay within less than a micron of the coating. We may, therefore, consider that layer to be infinitely wide and disregard the medium beyond the coating [Fig. 1(b)]. Note that cladding mode sensing of chemicals with coated fibers is still possible, even if indirectly, based on modifications to ncoat induced by target reagents (see Sec. IV). Direct sensing of media outside the coating would require coating layers with an index much closer to nSiO2. In what follows, we consider an infinite and uniform medium outside the silica fiber cladding, with index next or ncoat for bare or coated fibers, respectively. For simplicity, we refer below to the index outside the cladding as next for both cases.
We restrict our discussions to cladding modes with transverse profiles that are radially symmetric and independent of the transverse azimuthal coordinate. While cladding modes with azimuthal symmetries of any discrete order are supported by the fiber, their spatial overlap integrals with the radially symmetric single core mode and/or the transverse profiles of radially symmetric grating perturbations vanish. The coupling of light to cladding modes of general azimuthal symmetry is, therefore, more difficult, and they are disregarded in the subsequent treatment.
(a) Calculated normalized transverse profile of electromagnetic intensity in a cladding mode of order m = 5, in a step-index, single-core-mode fiber. The radii of the core and cladding were 4.1 and 62.5 µm, respectively. The indices of the core, cladding, and surrounding medium were 1.449, 1.444, and 1.405 RIU, respectively. (b) Calculated effective indices of the cladding modes guided by the same fiber as a function of modal order. (c) Calculated relative fraction of the electromagnetic intensity in overlap with the outside medium for the cladding modes of the same fiber as a function of modal order.
(a) Calculated normalized transverse profile of electromagnetic intensity in a cladding mode of order m = 5, in a step-index, single-core-mode fiber. The radii of the core and cladding were 4.1 and 62.5 µm, respectively. The indices of the core, cladding, and surrounding medium were 1.449, 1.444, and 1.405 RIU, respectively. (b) Calculated effective indices of the cladding modes guided by the same fiber as a function of modal order. (c) Calculated relative fraction of the electromagnetic intensity in overlap with the outside medium for the cladding modes of the same fiber as a function of modal order.
Figure 3(a) shows the calculated variation in the effective index as a function of changes to next about a baseline value of 1.405 RIU. The changes in are smaller than those in next by a factor of about 1000 due to the small fraction of the modal intensity in overlap with the outside medium. The small changes in are nevertheless measurable. Possible variations in the exact value of aclad may introduce ambiguity in data analysis. Figure 3(b) presents the changes in the same effective index as a function of aclad. Radius variations of 0.1 µm modify the effective index by about 10−5 RIU.
(a) Changes to the effective index of a cladding mode of order m = 15 as a function of variations in the refractive index of the outside medium. For the fiber parameters, see Fig. 2. The dashed red line denotes the index of fluoroacrylate coating used in this work. (b) Changes to the same effective index as a function of variations in the cladding radius. The dashed red line denotes the nominal radius of 62.5 µm.
(a) Changes to the effective index of a cladding mode of order m = 15 as a function of variations in the refractive index of the outside medium. For the fiber parameters, see Fig. 2. The dashed red line denotes the index of fluoroacrylate coating used in this work. (b) Changes to the same effective index as a function of variations in the cladding radius. The dashed red line denotes the nominal radius of 62.5 µm.
III. COUPLING OF LIGHT FROM THE CORE MODE TO A CLADDING MODE USING BRILLOUIN DYNAMIC GRATINGS
As an alternative to the inscription of permanent gratings, coupling between the core and cladding modes can be based on so-called Brillouin dynamic gratings: the traveling photoelastic perturbations in the refractive index associated with backward stimulated Brillouin scattering.36,37 To introduce this concept, let us first consider the coupling of light between counter-propagating optical core and cladding modes using standard, permanent fiber Bragg gratings. Figure 4(a) illustrates the dispersion relations between the temporal angular frequencies ω and axial wavenumbers of optical waves in the fiber. Here is the vacuum wavenumber. Each point represents a valid solution to the optical wave equation. The points connect to form continuous traces, corresponding to distinct spatial guided modes. The exact dependence of in each mode can become rather complex. For the sake of this discussion, however, we may well approximate the dispersion relation of a given optical mode as a straight line with a slope that equals its phase velocity: c/neff. Here, c is the speed of light in a vacuum.
(a) Dispersion relations between axial wavenumber and angular optical frequency in the optical core mode in one direction and an optical cladding mode in the opposite direction. The two are characterized by straight lines in the dispersion map, with slopes given by their respective phase velocities. Light is coupled between the two modes by a fixed Bragg grating, represented by a horizontal line corresponding to its wavenumber contribution. (b) Illustration of backward Brillouin stimulation of a guided acoustic core mode by two optical pump waves, which propagate in the single optical core mode in opposite directions. The two pumps are spectrally detuned by the Brillouin frequency shift of the fiber. With that choice, the frequency and wavenumber of the electrostrictive force induced by the two pump waves match those of a dilatational, axial acoustic core mode with phase velocity vL. (c) Photoelastic scattering of a probe wave from the optical core mode to a counter-propagating cladding mode by the acoustic wave stimulated by the two pumps. The frequency and wavenumber of the nonlinear polarization term due to photoelasticity match those of an optical cladding mode for a specific choice of the probe optical frequency.
(a) Dispersion relations between axial wavenumber and angular optical frequency in the optical core mode in one direction and an optical cladding mode in the opposite direction. The two are characterized by straight lines in the dispersion map, with slopes given by their respective phase velocities. Light is coupled between the two modes by a fixed Bragg grating, represented by a horizontal line corresponding to its wavenumber contribution. (b) Illustration of backward Brillouin stimulation of a guided acoustic core mode by two optical pump waves, which propagate in the single optical core mode in opposite directions. The two pumps are spectrally detuned by the Brillouin frequency shift of the fiber. With that choice, the frequency and wavenumber of the electrostrictive force induced by the two pump waves match those of a dilatational, axial acoustic core mode with phase velocity vL. (c) Photoelastic scattering of a probe wave from the optical core mode to a counter-propagating cladding mode by the acoustic wave stimulated by the two pumps. The frequency and wavenumber of the nonlinear polarization term due to photoelasticity match those of an optical cladding mode for a specific choice of the probe optical frequency.
A. Stimulation of Brillouin dynamic gratings by optical pump waves
The propagation of acoustic waves in a medium is associated with moving perturbations to its refractive index by virtue of photoelasticity. Therefore, the stimulation of acoustic waves with the necessary wavenumber Δk could, in principle, replace permanent inscription in the coupling of guided light between spatial modes. Such stimulation is possible through the widely known and employed process of backward Brillouin scattering in fibers.41,42 The dispersion relations of the waves involved in the process are illustrated in Fig. 4(b). A first optical pump wave of angular frequency ωp1 propagates in the core mode in the positive direction. We denote the transverse profile of the optical field in the core mode as (m−1) and the magnitude of the first pump wave in volts as Ap1. A second pump wave is counter-propagated in the core mode in the negative direction, with magnitude Ap2 and optical angular frequency ωp2 = ωp1 − Ω.
The angular frequency offset Ω is chosen near the Brillouin frequency shift of the fiber, ΩB (see further below). We assume, for the time being, that both pump waves are continuous with fixed magnitudes. We also assume for simplicity that the two waves are co-polarized along the entire fiber (for vector analysis of backward stimulated Brillouin scattering in standard, weakly birefringent fibers, see Ref. 56; for mitigation of polarization-induced fading, see Refs. 38 and 57).
B. The scattering of an optical probe wave by Brillouin dynamic gratings
Calculated relative efficiency of Brillouin dynamic grating coupling of light from the optical core mode to optical cladding modes as a function of the cladding mode order.
Calculated relative efficiency of Brillouin dynamic grating coupling of light from the optical core mode to optical cladding modes as a function of the cladding mode order.
The direct measurement of power that is coupled to a cladding mode is challenging. These modes often dissipate away before they might reach a detector at the end of the fiber. Alternatively, the probe wave in the core mode may be detected instead. Any coupling to a cladding mode would manifest in a loss of optical power in such a reading.
C. Spatially distributed analysis
Thus far, we have assumed both pump waves to be continuous. Therefore, Brillouin dynamic gratings could be formed over the entire length L of a fiber under test, and measurements of the output probe power would represent the spectrum of accumulated coupling, end to end. Local information cannot be retrieved in this manner. Spatially distributed analysis requires that the formation of Brillouin dynamic gratings be confined to short fiber sections at known locations in either transient or stationary manners.
Distributed sensing protocols based on Brillouin dynamic gratings follow those of standard Brillouin analysis in the core mode, which has been known for thirty years.38,61 In Brillouin optical time-domain analysis, the intensity of the second pump wave, which counter-propagates with respect to the continuous probe, is modulated by repeating short and isolated pulses [Fig. 6(a)]. The first pump wave remains continuous. The Brillouin dynamic grating, therefore, propagates with the second pump in the form of a pulsed perturbation. Consider a fiber section located at a distance z from the launch point of the pulsed pump wave. We denote the time in which the pulse is launched as t = 0. The Brillouin dynamic grating is formed at that point following a delay t = z/vg, where vg is the group velocity of light in the fiber. The probe wavefront at position z may be attenuated at that time due to coupling to a cladding mode. The modified probe front reaches its output end of the fiber, the same position where the pump pulse is launched, following a two-way propagation delay of 2z/vg. The detected probe power at that instance is unambiguously related to the coupling that took place at position z.
Calculated magnitude of the acoustic wave in backward stimulated Brillouin scattering processes as a function of time and position along a fiber under test. (a): Time-domain analysis, in which the amplitude of one pump is modulated by a single pulse of 10 ns duration and the other pump is continuous. The acoustic perturbation propagates along the fiber alongside the pulsed pump and reaches different positions at different times.62 (b): Correlation domain analysis, in which the magnitudes of both pumps are fixed and they are jointly modulated by a binary phase sequence with a symbol duration of 0.1 ns. The magnitude of the acoustic wave is spatially confined to a narrow correlation peak of 1 cm width, where it is stationary, and its complex magnitude is rapidly oscillating about zero expectation value everywhere else.63
Calculated magnitude of the acoustic wave in backward stimulated Brillouin scattering processes as a function of time and position along a fiber under test. (a): Time-domain analysis, in which the amplitude of one pump is modulated by a single pulse of 10 ns duration and the other pump is continuous. The acoustic perturbation propagates along the fiber alongside the pulsed pump and reaches different positions at different times.62 (b): Correlation domain analysis, in which the magnitudes of both pumps are fixed and they are jointly modulated by a binary phase sequence with a symbol duration of 0.1 ns. The magnitude of the acoustic wave is spatially confined to a narrow correlation peak of 1 cm width, where it is stationary, and its complex magnitude is rapidly oscillating about zero expectation value everywhere else.63
The spatial resolution of the analysis is given by Δz = Δt · vg/2, where Δt is the duration of the pump pulse. That duration, in turn, must exceed the lifetime of backward Brillouin stimulation 1/ΓB, on the order of 5–10 ns.36,37 The spatial resolution of the basic Brillouin optical time-domain analysis configuration is about 1 m.38 Several advanced protocols successfully pushed that resolution to the centimeter scale.38,64,65 These protocols, which will not be discussed here, are equally applicable to spatially distributed sensing through cladding modes that are excited by Brillouin dynamic gratings.
The power levels of the two pump waves, and hence the measurement signal-to-noise ratio, are limited by excessive Brillouin amplification or depletion, modulation instability, and the onset of amplified spontaneous Brillouin scattering.66,67 These detrimental effects accumulate over the length of the fiber. Therefore, a longer measurement range would impose more stringent restrictions on pump power levels, and the signal-to-noise ratio would deteriorate accordingly.68 Compared with standard Brillouin sensing protocols, the Brillouin dynamic grating cladding mode sensors face more severe limitations: Competing nonlinear mechanisms occur within the core mode with higher efficiency due to complete spatial overlap among all waves involved, whereas the coupling signal of interest is subject to the transverse inefficiency penalty of . The maximum reflectivity of the cladding modes, subject to the limits imposed by the nonlinear propagation of the pump waves, is inversely proportional to the number of resolution points squared: .40
Compared with time domain analysis, the correlation domain protocols can confine the stimulation of the acoustic waves to shorter sections, down to 1.6 mm in standard fiber, providing superior resolution.71 On the downside, point-by-point scanning of the correlation peak positions considerably extends the experimental duration, whereas time-domain analysis covers the entire length of the fiber in every trace. More elaborate variants of correlation domain analysis reduced the number of necessary position scans.72 Finally, note that both time-domain and correlation-domain analysis protocols must be repeated for multiple choices of the probe angular frequency to obtain a two-dimensional map of the local coupling spectra to the cladding modes.
IV. EXPERIMENTAL RESULTS OF SPATIALLY DISTRIBUTED OPTICAL CLADDING MODE SENSING
In this section, experimental methods and results of Brillouin dynamic grating coupling to the cladding modes of standard fibers are briefly presented. The reader is referred to recent references for complete detail.39,40 A schematic illustration of the setup is shown in Fig. 7. The two pump waves were drawn from a common laser diode with a 1563.3 nm wavelength.39,40 The exact optical frequency of the pumps was fine-tuned using a suppressed-carrier single-sideband (SC-SSB) electro-optic modulator driven by a microwave generator. The small-scale frequency offsets adjusted the difference between the optical frequencies of the pump waves and the probe field. The pump light was split into two branches. A first pump wave was amplified by an erbium-doped fiber amplifier to 30 dBm power and launched into one end of the fiber under test. The frequency of the second pump wave in the other branch was downshifted using a second SC-SSB modulator driven by a sine wave from a second microwave generator. The angular frequency difference Ω between the pump waves was chosen to match the Brillouin shift ΩB ≈ 2π × 10.890 GHz of the fiber under test. The second pump wave was amplified by another fiber amplifier to 27 dBm power and launched from the opposite end of the fiber under test.
Experimental setup for Brillouin optical time-domain analysis of dynamic grating coupling to the optical cladding modes of standard, single-mode fibers. BPF: tunable optical bandpass filter; SSB: single-sideband electro-optic modulator; EDFA: erbium-doped fiber amplifier; MZM: Mach-Zehnder electro-optic intensity modulator; Circ.: fiber-optic circulator.
Experimental setup for Brillouin optical time-domain analysis of dynamic grating coupling to the optical cladding modes of standard, single-mode fibers. BPF: tunable optical bandpass filter; SSB: single-sideband electro-optic modulator; EDFA: erbium-doped fiber amplifier; MZM: Mach-Zehnder electro-optic intensity modulator; Circ.: fiber-optic circulator.
A continuous probe wave of 13 dBm power was provided by another laser diode. Its wavelength could be tuned in 8 pm steps (1 GHz frequency steps) over several nanometers. Combined with the small-scale frequency offsets of the pump source mentioned earlier, the difference between pump and probe frequencies could be adjusted over a broad range with high accuracy. The probe was launched into the fiber under test in the same direction as the first pump wave. The Brillouin dynamic grating stimulated by the two pumps could couple light from the probe wave into counter-propagating cladding modes. The probe wave was detected by a photo-receiver at the output end of the fiber. A tunable optical bandpass filter blocked off the pump waves from reaching the detector.
The coupling to the cladding modes of the fiber under test was first characterized in a non-distributed manner. To that end, the second pump wave was amplitude-modulated by a sine wave of 50 kHz frequency. The strength of the stimulated Brillouin dynamic gratings was therefore modulated at the same rate. The dynamic grating coupling imposed a weak modulation at a 50 kHz rate on the detected power of the output probe wave. The modulation of the received signal was monitored by a lock-in amplifier. Figure 8(a) shows the measured and calculated spectra for a 50 cm-long, standard single mode fiber that was stripped off its protective coating and kept in air.39 The lock-in signal exhibits multiple sharp peaks at specific probe wavelengths, which represent the coupling of the probe wave to cladding modes of consecutive odd orders between 11 and 21. Note that coupling to the even order modes vanishes, in agreement with calculations (Fig. 5). The observed wavelengths of probe wave coupling to the cladding modes agree very well with predictions.
(a) Red: measured, normalized lock-in modulation signal of the output probe wave as a function of the probe wavelength. The pump’s wavelength is noted with a black dashed arrow. The standard, single-mode fiber under test was 50 cm long, stripped of its protective coating, and kept in air. The frequency difference between the two pump waves was adjusted to match the Brillouin frequency shift of the fiber. Multiple peaks are observed, corresponding to the coupling of the probe wave to cladding modes of odd orders between 11 and 21. Mode orders are noted above the spectral peaks. Blue: theoretical reflectivity spectrum. The measured wavelengths of peak coupling agree very well with the calculations.39 (b) Measured normalized lock-in signal as a function of the detuning between the two pump waves and the difference between the pump and probe frequencies in the vicinity of the coupling peak to cladding mode m = 17. The offset of maximum coupling is designated as the zero point for convenience.39 (c) Same as panel (a), for a meter-long section of fiber coated with a thin layer of fluoroacrylate polymer.40
(a) Red: measured, normalized lock-in modulation signal of the output probe wave as a function of the probe wavelength. The pump’s wavelength is noted with a black dashed arrow. The standard, single-mode fiber under test was 50 cm long, stripped of its protective coating, and kept in air. The frequency difference between the two pump waves was adjusted to match the Brillouin frequency shift of the fiber. Multiple peaks are observed, corresponding to the coupling of the probe wave to cladding modes of odd orders between 11 and 21. Mode orders are noted above the spectral peaks. Blue: theoretical reflectivity spectrum. The measured wavelengths of peak coupling agree very well with the calculations.39 (b) Measured normalized lock-in signal as a function of the detuning between the two pump waves and the difference between the pump and probe frequencies in the vicinity of the coupling peak to cladding mode m = 17. The offset of maximum coupling is designated as the zero point for convenience.39 (c) Same as panel (a), for a meter-long section of fiber coated with a thin layer of fluoroacrylate polymer.40
Figure 8(b) shows a two-dimensional scan of the normalized lock-in signal in the same fiber as a function of both Ω and ωs near the peak of coupling to cladding mode m = 17.39 The width of the coupling spectrum with respect to changes in Ω about ΩB is 2π × 37 MHz, matching the Brillouin linewidth. The full width at half-maximum with respect to ωs about is 2π × 260 MHz. The expected width according to Eq. (22) is 2π × 185 MHz. The experimental value is somewhat broadened by sub-micron variations in the local cladding diameter along the fiber section under test. Figure 8(c) presents measured and calculated coupling spectra in a standard single-mode fiber that was coated with a thin layer of fluoroacrylate polymer with a refractive index ncoat of 1.405 RIU, below that of silica.40 The coupling to the cladding modes of the coated fiber is evident. Here too, measurements agree well with calculations.
Figure 9(a) shows the distributed mapping of coupling spectra to cladding mode m = 17 along 2 m of bare fiber. The mapping was obtained using Brillouin optical correlation domain analysis: both pump waves were jointly modulated by a periodic binary phase sequence with a symbol duration of 800 ps.39 The symbol duration corresponds to a spatial resolution of 8 cm. Two fiber sections, each 8 cm-long, were immersed in liquids: one in water and the other in ethanol. The probe frequencies of maximum coupling to the cladding mode are offset in both locations by 1.9 and 3.2 GHz, respectively.39 The offsets quantitatively agree with expectations. The spatially distributed analysis of liquids outside the fiber cladding was thereby demonstrated. The presence of liquids could not be detected using Brillouin analysis in the core mode only. The experimental uncertainty in repeating measurements of , in a fixed fiber position, was ±2π × 75 MHz.39 That uncertainty corresponds to errors between ±4 × 10−4 and ±4 × 10−3 RIU in the estimate of next, depending on its value. Variations in the coupling spectra among fiber positions kept in air are likely due to differences in the local cladding diameter, on the order of a few hundreds of nm.
(a) Measured, normalized lock-in modulation signal of the output probe wave as a function of the frequency detuning between pump and probe and the position z of a localized Brillouin dynamic grating. The measurements were based on correlation domain analysis. Data in each z are normalized to a maximum of unity. Coupling to cladding mode m = 17 is observed in all positions. The bare fiber under test was kept in the air, except for two 8 cm-wide sections that were immersed in water and ethanol (see legend). The optimal frequency offsets at the two locations are shifted with respect to the baseline by 1.9 and 3.2 GHz, respectively.39 (b) Detected voltage of the output probe wave as a function of position and probe wavelength offset. The measurements were based on time-domain analysis. The baseline difference between the pump and probe wavelengths was 2.4 nm. Coupling to a cladding mode is observed in five sections of fiber coated with a fluoroacrylate layer, each 1 m-long, separated by connectors with standard acrylate coating, in which cladding modes are not guided. All fibers were kept in the air. Coupling manifests in local dips in the output power of the probe wave in the core mode.39 (c) Same as panel (b), for two coated fiber sections kept in air.40 (d) Same as panel (c), 24 h following the immersion of the left coated fiber section only in acetone. The fiber section on the right served as a reference. The probe wavelength of maximum coupling to the cladding mode in the immersed section shifted by 10 pm, corresponding to a local change in the index outside the cladding by 0.047 RIU.40
(a) Measured, normalized lock-in modulation signal of the output probe wave as a function of the frequency detuning between pump and probe and the position z of a localized Brillouin dynamic grating. The measurements were based on correlation domain analysis. Data in each z are normalized to a maximum of unity. Coupling to cladding mode m = 17 is observed in all positions. The bare fiber under test was kept in the air, except for two 8 cm-wide sections that were immersed in water and ethanol (see legend). The optimal frequency offsets at the two locations are shifted with respect to the baseline by 1.9 and 3.2 GHz, respectively.39 (b) Detected voltage of the output probe wave as a function of position and probe wavelength offset. The measurements were based on time-domain analysis. The baseline difference between the pump and probe wavelengths was 2.4 nm. Coupling to a cladding mode is observed in five sections of fiber coated with a fluoroacrylate layer, each 1 m-long, separated by connectors with standard acrylate coating, in which cladding modes are not guided. All fibers were kept in the air. Coupling manifests in local dips in the output power of the probe wave in the core mode.39 (c) Same as panel (b), for two coated fiber sections kept in air.40 (d) Same as panel (c), 24 h following the immersion of the left coated fiber section only in acetone. The fiber section on the right served as a reference. The probe wavelength of maximum coupling to the cladding mode in the immersed section shifted by 10 pm, corresponding to a local change in the index outside the cladding by 0.047 RIU.40
Figure 9(b) presents a distributed measurement of coupling spectra to cladding mode m = 13 along five sections of standard fiber.40 The sections were 1 m-long each, and they were coated with a thin fluoroacrylate layer. Mapping was obtained through Brillouin optical time domain analysis: the magnitude of the second pump wave was modulated with repeating pulses of 10 ns duration, and the probe wave output power was measured as a function of time. The coupling with the cladding mode is evident in all sections. Differences among the exact wavelengths of maximum coupling are due to small scale variations in the cladding diameter and/or coating index.
Figures 9(c) and 9(d) present similar time-domain analyses of coupling spectra in two coated fiber sections connected in series.40 In panel (c), both sections were kept in air, whereas in panel (d), only the left section was immersed in acetone for 24 h, and the right section served as a reference (see Ref. 40). The probe wavelength of peak coupling in the immersed section shifted with respect to the reference by 10 pm.40 That offset corresponds to a change in the refractive index immediately outside the cladding of 0.047 RIU.40 Smaller offsets were already observed within minutes following immersion.40 The presence of acetone could be detected and localized based on its effect on the optical properties of the coating layer. The liquid could not be detected through measurements in the core mode alone.
V. RADIALLY SYMMETRIC ACOUSTIC CLADDING MODES OF STANDARD FIBERS
In the second part of this tutorial, we address the prospects of sensing outside the fiber using cladding modes that are acoustic rather than optical. In the previous discussion, acoustic waves were stimulated only in the core in order to scatter light into optical cladding modes. These modes, in turn, could monitor the refractive index outside the silica cladding boundary. We now rely yet again on optical pump waves in the core mode to stimulate acoustic waves. This time, however, the acoustic waves would propagate in cladding modes rather than core modes. The acoustic cladding modes are sensitive to the elastic properties of the surrounding media under test, and their oscillations are monitored by light in the single optical core mode.
A. Optical force induced by co-propagating pump tones
(a) Dispersion relations between axial wavenumber and angular frequency in the optical core mode and in one radially symmetric acoustic cladding mode. The acoustic cladding mode is characterized by a cut-off frequency Ω0m. Two co-propagating optical pump waves induce an electrostrictive force per unit volume. The angular frequency of the force is the difference between the two optical angular frequencies, and its wavenumber also equals the difference between the pump wavenumbers. The angular frequency and wavenumber of the force term may match those of the acoustic cladding mode close to its cut-off, where its phase velocity can equal that of the optical core mode. The stimulation of the acoustic cladding mode is accompanied by the coupling of optical power from the higher-frequency pump tone to the lower-frequency one. (b) Photoelastic scattering of an optical probe wave in the core mode by an acoustic cladding mode. The probe wave co-propagates with the two pump waves. It is significantly weaker than the pumps and does not contribute to the stimulation of the acoustic wave. Photoelastic scattering generates higher and lower sidebands and results in phase modulation.
(a) Dispersion relations between axial wavenumber and angular frequency in the optical core mode and in one radially symmetric acoustic cladding mode. The acoustic cladding mode is characterized by a cut-off frequency Ω0m. Two co-propagating optical pump waves induce an electrostrictive force per unit volume. The angular frequency of the force is the difference between the two optical angular frequencies, and its wavenumber also equals the difference between the pump wavenumbers. The angular frequency and wavenumber of the force term may match those of the acoustic cladding mode close to its cut-off, where its phase velocity can equal that of the optical core mode. The stimulation of the acoustic cladding mode is accompanied by the coupling of optical power from the higher-frequency pump tone to the lower-frequency one. (b) Photoelastic scattering of an optical probe wave in the core mode by an acoustic cladding mode. The probe wave co-propagates with the two pump waves. It is significantly weaker than the pumps and does not contribute to the stimulation of the acoustic wave. Photoelastic scattering generates higher and lower sidebands and results in phase modulation.
The force propagates along the fiber with the phase velocity of guided light in the optical core mode. Compared with the case of counter-propagating pump tones, the wavenumber q of the force term in Eq. (28) is smaller by six orders of magnitude. The direction of the force vector is also different. The two co-propagating tones induce a force that is almost entirely transverse, whereas the counter-propagating pumps induce an axial force term (see Sec. III).
The transverse profile of the force consists of three components within the squared brackets of Eq. (28). The first term is radially symmetric and points in the radial direction only. The remaining two terms depend on the azimuthal coordinate and follow a two-fold azimuthal symmetry. The radial symmetry of the fiber structure is removed by the direction of polarization of the pump waves. All three terms may contribute to the simulation of guided acoustic cladding modes, which maintain the same symmetries. The first force term may drive the oscillations of radial acoustic modes, whereas the latter two can generate torsional-radial modes of two-fold azimuthal symmetry.30,31 Of the two classes of modes, the optomechanical interactions involving the radial modes are stronger and more widely investigated. While the sensing of media outside the cladding boundary can be performed using torsional-radial acoustic cladding modes as well,44 we only consider the radial modes below for simplicity. The reader is referred to recent analyses of the more general case.74,75
B. Stimulation of transverse acoustic cladding modes near cut-off and the modal linewidths
We consider next the guided acoustic cladding modes that may be stimulated by the force per unit volume term of Eq. (29). These modes are denoted by R0m, where m is an integer. Each mode is characterized by a cut-off angular frequency Ω0m, below which it may no longer propagate in the axial direction [Fig. 10(a)]. As the acoustic angular frequency Ω approaches the cut-off value from above, the axial wavenumber becomes vanishingly small. The phase velocity of the acoustic modes, therefore, becomes arbitrarily high. Since the axial wavenumber q of the driving force is small, as noted earlier, the guided acoustic waves may be effectively stimulated only close to their cut-off. Therefore, we examine their properties at that limit. Note, however, that the acoustic axial wavenumber is not entirely zero, and the wave does propagate in the direction.
Normalized transverse profile of radial material displacement in radially symmetric acoustic cladding mode R06 of a standard bare fiber with a cladding diameter of 125 µm. The cut-off angular frequency Ω06 of the mode is 2π × 270 MHz.
Normalized transverse profile of radial material displacement in radially symmetric acoustic cladding mode R06 of a standard bare fiber with a cladding diameter of 125 µm. The cut-off angular frequency Ω06 of the mode is 2π × 270 MHz.
As an alternative to stimulation by a pair of pump tones, the acoustic cladding modes may also be driven by pump pulses of instantaneous power (W). Let us denote the Fourier transform of the instantaneous pump power as , in units of W × rad−1 × Hz−1. The magnitude of modal oscillations may be expressed in the angular frequency domain, (ac,m)(Ω), using the form of Eq. (36) with replaced by .73 The units of (ac,m)(Ω) are m2 × rad−1 × Hz−1. A packet of multiple acoustic cladding modes may be stimulated by short, broadband pump pulses.75
The modal linewidth Γ0m quantifies the losses of the acoustic cladding modes, and it is central to the comparatively new concept of sensing based on these modes. One source of loss is internal dissipation within the core and cladding of the optical fiber. These losses are relatively small. They are quantified by internal linewidth contributions, , that are mode dependent. The internal contributions are the only linewidths terms when a bare standard fiber is kept in air. They increase with modal order and scale quadratically with Ω0m.78 The linewidth may also be broadened by inhomogeneities in the cladding diameter.78 Typical values of are between 2π × 30 and 2π × 200 kHz.43–54,78
The linewidths are significantly modified when the bare fiber is placed in a medium of finite mechanical impedance Zext (kg × m−2 × s−1). We consider the medium to extend outside the cladding indefinitely. This assumption is useful for most settings in immersion in liquids. The presence of an outside liquid medium alters the boundary conditions: the stress at the outer cladding radius must equal the liquid pressure.79 In principle, a modified boundary condition equation can be formulated and solved to obtain a different discrete set of eigenvalues. These eigenvalues are complex: their real parts signify the cut-off frequencies of radial acoustic cladding modes of the fiber in liquid, and their imaginary parts represent modal linewidth contributions. While this solution is exact, it provides limited intuition. In addition, the differences in the cut-off angular frequencies between the solutions of the fiber in air or liquids are small. As an alternative to the exact solutions, we may assume that the cut-off frequencies remain the solutions of Eq. (31) and obtain excellent approximations for the modal linewidths through the following considerations.
Calculated decay rates of acoustic intensity in acoustic cladding modes as a function of the mechanical impedance of an infinite liquid outside the cladding boundary of a bare fiber.48 The impedances of ethanol, water, and polyimide are noted by dashed vertical lines (left to right).
Calculated decay rates of acoustic intensity in acoustic cladding modes as a function of the mechanical impedance of an infinite liquid outside the cladding boundary of a bare fiber.48 The impedances of ethanol, water, and polyimide are noted by dashed vertical lines (left to right).
C. Photoelastic scattering by guided acoustic modes
Calculated peak nonlinear optomechanical coefficients of radial acoustic cladding modes in a standard uncoated fiber as a function of the modal cut-off frequency .
Calculated peak nonlinear optomechanical coefficients of radial acoustic cladding modes in a standard uncoated fiber as a function of the modal cut-off frequency .
The photoelastic phase modulation of the optical probe may also be rationalized in terms of the traveling grating of the refractive index perturbation [Eq. (46)]. The index grating propagates in the positive direction with the same phase velocity as the optical core mode. Therefore, the probe wave that enters the fiber at z = 0 and a given instance t is subject to the same index perturbation through the entire fiber length. The index perturbation leads to the accumulation of an extra phase of , which varies in time at frequency Ω. The magnitude of the phase modulation equals . The characterization of photoelastic phase modulation spectra is the most common protocol in optical fiber sensors based on acoustic cladding modes.
The solution is precise only for relatively weak coupling, . For sufficiently large pump power levels and/or fiber lengths, the coupling of power between the two pump tones is accompanied by the generation of modulation sidebands of increasing order, as described earlier. In that case, the pair of nonlinear wave equations must be extended to a larger set, and the evolution of the two input tones deviates from that of Eqs. (68) and (69).82 Note that the nonlinear coefficient of the Kerr effect is purely real-valued; hence, it does not contribute to the coupling of power between the pump waves.82 By contrast, the generation of modulation sidebands takes place through photoelastic scattering and the Kerr effect combined, similar to the aforementioned phase modulation of a probe wave in the spontaneous regime.82 The monitoring of pump power levels can also provide the basis for spatially distributed analysis of acoustic cladding mode spectra.
D. Coated fibers and spatially distributed analysis
Thus far, it has been assumed that the fiber was stripped of any polymer protective coatings. However, the application of bare fibers outside the research laboratory is impractical. The presence of polymer coating layers may alter the preceding analysis considerably. Many types of coating, such as the highly popular dual-layer acrylates, absorb the stimulated acoustic waves that radiate out of the cladding before they may reach their outer boundary. In modeling acoustic cladding modes in such fibers, the coating may be considered infinite. The direct sensing of media beyond these coatings is not possible. The modal linewidth Γ0m is broadened by the presence of the coating due to the dissipation of acoustic radiation according to the mechanical impedance of the coating layer. Sensing may be carried out indirectly in cases where a target reagent modifies the elastic properties of the coating layer itself,50 similar to the optical cladding mode sensors discussed in earlier sections.
Unlike the case of optical cladding modes, certain polymer coating layers are sufficiently thin and have sufficiently low absorption to allow for the propagation of acoustic waves to their outer boundaries. These include polyimide and fluoroacrylate coating layers. When using these layers, the mechanical impedance of a liquid outside the coating boundary modifies the acoustic cladding mode spectra and may be monitored directly. This opportunity is not provided with the optical cladding modes of coated fibers. However, these measurements do raise difficulties that are not encountered when using bare fibers.
Without the coating, we have established a one-to-one, universal relation between the mechanical impedance Zext of a liquid substance under test and the modal linewidth Γ0m. That relation was independent of the modal order m. Moreover, the effect of the exact cladding radius aclad on the modal linewidth was small. If an intermediate coating layer of finite thickness is placed between the cladding and the outside medium, the spectra become markedly different (see Fig. 14). The modal linewidths for a given medium vary strongly among modes and heavily depend on small changes in coating thickness, well within specified tolerances. The linewidths of acoustic cladding modes for a given fiber section under test and a given liquid outside the coating cannot be predicted a priori. The specific modes used in the analysis should be chosen carefully, and pre-calibration on known test media is mandatory. However, quantitative sensing of liquids using the acoustic cladding modes of commercially available coated fibers has been achieved, as shown in Sec. VI.46,48
Calculated linewidths due to acoustic dissipation out of standard single-mode fibers coated with a thin layer of polyimide as functions of the mechanical impedance of a liquid medium outside the coating.48 (a) Linewidths of acoustic mode R05 (cut-off frequency near 178 MHz). (b) Linewidths of acoustic mode R09 (cut-off frequency near 325 MHz). In each panel, calculation results are shown for several outer radii of the coating layer (see legends). The expected linewidths for a bare fiber are plotted as well for comparison. The linewidths for a given medium outside the coating vary among modes and with the exact coating radius. The geometric sensitivity of mode R05 is much lower than that of mode R09. The mechanical impedances of ethanol, water, and polyimide are noted by vertical dashed lines in both panels. Licensed under CC BY.
Calculated linewidths due to acoustic dissipation out of standard single-mode fibers coated with a thin layer of polyimide as functions of the mechanical impedance of a liquid medium outside the coating.48 (a) Linewidths of acoustic mode R05 (cut-off frequency near 178 MHz). (b) Linewidths of acoustic mode R09 (cut-off frequency near 325 MHz). In each panel, calculation results are shown for several outer radii of the coating layer (see legends). The expected linewidths for a bare fiber are plotted as well for comparison. The linewidths for a given medium outside the coating vary among modes and with the exact coating radius. The geometric sensitivity of mode R05 is much lower than that of mode R09. The mechanical impedances of ethanol, water, and polyimide are noted by vertical dashed lines in both panels. Licensed under CC BY.
Finally, changes to the coating layer itself may be of interest, for example, in the research and development of materials, in production line quality control, or in preventive maintenance.49,50 The temperature dependence of acoustic velocities in coating layers has been mapped.49 Gamma radiation was successfully detected and quantified based on its effect on the acoustic velocity in a thin layer of fluoroacrylate coating,50 the same layer that also served in optical cladding modes monitoring immersion in acetone (Ref. 40, Sec. IV).
A major challenge for fiber sensors based on acoustic cladding modes has to do with their extension toward spatially distributed analysis. As shown earlier, the photoelastic scattering induced by these modes takes place in the forward direction. The scattering spectrum may be readily observed at the far end of the fiber. However, the location of a specific contribution of forward scattering may not be directly identified through time-of-flight analysis, which underlies the distributed mapping of backscatter.5 Most solutions proposed to address this challenge have been indirect: the forward scattering spectra have been deduced through the analysis of an auxiliary backscattering mechanism.
In one example, the optical time domain reflectometry of Rayleigh backscatter has been extended to dual-frequency operation.47 The measurements estimated the local power levels of two pump pulses, , through the analysis of collected Rayleigh backscatter in both time and frequency.47 The collected data were differentiated with respect to position to obtain an estimate of . With that estimate, the local value of could be evaluated using Eq. (67).47 In a different protocol, the magnitudes of multiple sidebands of a phase modulated probe wave, , were estimated through Brillouin optical time domain analysis.45 Each sideband served as a pump wave for the backward stimulated Brillouin scattering process, and its local magnitude could be estimated through measurements of an auxiliary backward Brillouin signal.45 With the mapping of multiple sidebands, the extent of phase modulation accumulated up to position z could be evaluated using Eq. (59). Here too, the obtained trace was differentiated with respect to the position to retrieve the local .45
Of the two indirect methods described earlier, the measurements assisted by backward Brillouin scattering have been more successful. The spatial resolution has been recently brought below 1 m, with over 200 resolution points.53,54 Yet performance remains modest. The differentiation of collected traces with respect to position is highly prone to noise and remains a drawback of indirect mapping protocols. The direct distributed analysis of forward scattering spectra has recently been achieved for the first time using the acoustic cladding modes of polarization maintaining fibers.51 The mapping relied on inter-modal scattering between the two non-degenerate principal axes of the fiber.51,85 There as well, however, the resolution was limited to 60 m with only 17 resolved locations.51 Further breakthroughs are necessary to obtain technologically viable distributed fiber sensing based on acoustic cladding modes.
Point-sensing of media outside a centimeter-long section of bare fiber, based on acoustic cladding modes, has been demonstrated last year.52 The measurement relied on the stimulation of acoustic cladding modes by pump waves in one core of a multi-core fiber and on monitoring the induced photoelastic perturbations to the reflectivity of a Bragg grating in a different core.52 In a series of recent studies by Sanchez et al., the local spectra of both radial and torsional-radial acoustic cladding modes were measured using long period gratings.86–89 The technique served for precise estimates of the fiber’s Poisson ratio87 and simultaneous and unambiguous measurements of temperature and strain.88
VI. EXPERIMENTAL RESULTS OF ACOUSTIC CLADDING MODE SENSING
An experimental setup for acoustic cladding modes fiber sensing, based on a Sagnac interferometer loop, is illustrated in Fig. 15(a).90 The technique was first proposed and employed by Kang and co-workers in 2009.90 The section of fiber under test is placed within the interferometer loop. Light from a first laser diode in the 1550 nm wavelength range is intensity modulated in an electro-optic Mach-Zehnder modulator to obtain pump pulses of nanosecond-scale duration and a period of several microseconds. The pump pulses are amplified by an erbium-doped fiber amplifier to average power levels of hundreds of mW and launched into the section under test in the clockwise direction only. The pump pulses stimulate wave packets of guided acoustic modes (see Sec. V B and Ref. 75). A polarization scrambler is used to suppress the contributions of non-radial modes.74 A tunable optical bandpass filter blocks the pump pulses from reaching the loop output.
(a) Schematic illustration of an experimental setup for the measurement of scattering spectra by acoustic cladding modes based on a Sagnac interferometer loop.50 EDFA: erbium-doped fiber amplifier; PC: polarization controller; EOM: electro-optic amplitude modulator. Licensed under CC BY. (b) Measured and calculated normalized optomechanical nonlinear coefficients of scattering by radial acoustic cladding modes in a standard uncoated single-mode fiber.74 The spectrum consists of a set of discrete and narrow peaks.
(a) Schematic illustration of an experimental setup for the measurement of scattering spectra by acoustic cladding modes based on a Sagnac interferometer loop.50 EDFA: erbium-doped fiber amplifier; PC: polarization controller; EOM: electro-optic amplitude modulator. Licensed under CC BY. (b) Measured and calculated normalized optomechanical nonlinear coefficients of scattering by radial acoustic cladding modes in a standard uncoated single-mode fiber.74 The spectrum consists of a set of discrete and narrow peaks.
Continuous wave light of a different wavelength in the 1550 nm range from a second laser diode serves as an optical probe. The probe wave is coupled into the loop in both directions. The clockwise propagating probe wave replica acquires instantaneous phase modulation in the fiber section under test due to the stimulated acoustic waves and the Kerr effect combined. For most practical settings, . The counterclockwise propagating probe acquires much weaker photoelastic phase modulation due to the lack of wavenumber matching.
The beating of the two probe wave components at the loop output converts the non-reciprocal photoelastic phase modulation into an intensity signal. Polarization controllers within the loop and at the input path of the probe wave are adjusted to obtain maximum intensity variations at the loop output.90 By contrast, environmental phase drifts along the fiber under test are common to both directions of propagation, and they are eliminated by the Sagnac loop arrangement.90 The output probe wave is detected by a photo-receiver. The detected voltage is digitized by an oscilloscope at a rate of several giga-samples per second for further offline signal processing. Traces are typically averaged over thousands of repeating pump pulses to improve the measurement signal-to-noise ratio.
The phase modulation of the probe wave comprises of a Kerr effect contribution and photoelastic scattering combined. However, the contribution of the instantaneous Kerr effect vanishes as soon as the pump pulse ends, whereas phase modulation through forward Brillouin scattering continues over acoustic lifetimes of hundreds of nanoseconds or longer. Time gating of collected traces can remove the first few nanoseconds and eliminate the Kerr effect from the analysis of probe phase modulation. Figure 15(b) shows the measured and calculated spectra of scattering by stimulated radial acoustic cladding modes in a standard, uncoated single-mode fiber.74 The spectrum consists of discrete peaks with linewidths on the order of 100–200 kHz. Measurements are in excellent agreement with expectations.
The spectra of stimulated acoustic modes were characterized using the same setup, with the bare fiber immersed in ethanol or water. The measured linewidths were used to estimate the mechanical impedance of the liquids using Eq. (39). Figure 16 (solid lines) shows the measured impedances as a function of the cut-off frequencies of the acoustic modes used in experiments.43 The dashed lines denote the literature values of the liquids’ impedances.91,92 The measurements retrieved the mechanical impedance with 1% accuracy. The results were the first demonstration of acoustic cladding mode sensing.43 The technique can identify the presence of liquids outside certain types of protective polymer coatings. Figure 17 shows calculated and measured spectra with air, ethanol, and water outside a standard fiber coated by a thin layer of polyimide.48 The liquids have a different effect on the linewidth of each mode. The modal response can be calibrated and accounted for. Similar results were obtained by Chow and Thevenaz.46
Solid lines—mechanical impedance of liquids estimated through the analysis of stimulated acoustic cladding modes as a function of the modal cut-off frequency.43 Dashed lines—reference values.91,92 Red (blue) traces correspond to a bare standard single-mode fiber in ethanol (water).
Measured (solid) and calculated (dashed) scattering spectra of stimulated radial acoustic cladding modes in a standard single-mode fiber, coated by a thin layer of polyimide.48 The fiber was kept in air (a), ethanol (b), and water (c).
Measured (solid) and calculated (dashed) scattering spectra of stimulated radial acoustic cladding modes in a standard single-mode fiber, coated by a thin layer of polyimide.48 The fiber was kept in air (a), ethanol (b), and water (c).
Figure 18 shows an example of a spatially distributed analysis of acoustic cladding modes.47 Measurements were obtained using pump pulse envelopes consisting of two tones detuned in angular frequency by a variable Ω. Rayleigh backscatter of the pump signal was collected and analyzed in both time and frequency and the local power levels of the two tones were estimated.47 The local nonlinear optomechanical coefficient of the acoustic cladding mode was then evaluated using Eq. (67). The standard single-mode fiber under test was 3 km long, and it was coated through most of its length with a standard dual-layer acrylate coating. A 100 m long section, located 2 km from the input end, was coated instead with a thin layer of polyimide. The cut-off frequency of radial acoustic cladding mode R07 is different in that section.
Measured nonlinear optomechanical coefficient of radial acoustic mode R07 as a function of frequency and position along 3 km of standard single-mode fiber under test.47 The fiber was coated with a standard dual-layer acrylate coating through most of its length. A 100 m-long section, located 2 km from the input end, was coated by a thin layer of polyimide instead. That section is characterized by a different modal cut-off frequency . The spectra were mapped based on the estimated local exchange of optical power between a pair of pump tones within a pulsed envelope.47 The two local power levels were resolved using the analysis of Rayleigh backscatter in both time and frequency domains.47
Measured nonlinear optomechanical coefficient of radial acoustic mode R07 as a function of frequency and position along 3 km of standard single-mode fiber under test.47 The fiber was coated with a standard dual-layer acrylate coating through most of its length. A 100 m-long section, located 2 km from the input end, was coated by a thin layer of polyimide instead. That section is characterized by a different modal cut-off frequency . The spectra were mapped based on the estimated local exchange of optical power between a pair of pump tones within a pulsed envelope.47 The two local power levels were resolved using the analysis of Rayleigh backscatter in both time and frequency domains.47
Figure 19 shows an example of spatially distributed sensing of liquids outside 730 m of standard fiber.45 The fiber was coated through most of its length, except for a 30 m long section that was stripped of its polymer coating.45 The measurements distinguish among air, ethanol, and water outside the bare fiber section. Here too, the acoustic cladding modes were stimulated by a pair of pump tones within a pulsed envelope.45 A readout probe pulse was launched with a certain delay following the pump tones. The probe pulse was phase modulated by the stimulated acoustic cladding modes, as shown in Eq. (58). Due to the time lag between pump and probe pulses, the phase modulation of the probe wave was free of Kerr effect contributions.45 The modulation induced upper and lower sidebands to the probe wave, separated by integer multiples of the acoustic angular frequency Ω [Eq. (59)]. The magnitudes of several sidebands were mapped as functions of fiber positions using standard backward Brillouin optical time-domain analysis.45 Based on the sidebands’ magnitudes, the extent of phase modulation accumulated up to a point of interest z could be evaluated. The estimate was differentiated with respect to the position to obtain the local contribution of photoelastic scattering by acoustic cladding modes. The spatial resolution of sensing protocols assisted by backward Brillouin scattering analysis has since been enhanced to less than 1 m.53,54
Measured relative nonlinear coefficients of forward Brillouin scattering through radial mode R07 as functions of acoustic frequency and position along a standard single-mode fiber under test.45 Spatially distributed mapping was carried out indirectly, using backward Brillouin scattering optical time-domain analysis. The 730 m long fiber was coated a with standard dual-layer acrylate coating, except for a 30 m long exposed section located 500 m from the input end. That section was kept in the air (a), immersed in ethanol (b), or immersed in water (c). The modal linewidths of the local scattering spectra at that section were 1.81, 2.86, and 4.12 MHz in the three panels, respectively.45 Licensed under CC BY.
Measured relative nonlinear coefficients of forward Brillouin scattering through radial mode R07 as functions of acoustic frequency and position along a standard single-mode fiber under test.45 Spatially distributed mapping was carried out indirectly, using backward Brillouin scattering optical time-domain analysis. The 730 m long fiber was coated a with standard dual-layer acrylate coating, except for a 30 m long exposed section located 500 m from the input end. That section was kept in the air (a), immersed in ethanol (b), or immersed in water (c). The modal linewidths of the local scattering spectra at that section were 1.81, 2.86, and 4.12 MHz in the three panels, respectively.45 Licensed under CC BY.
VII. SUMMARY AND DISCUSSION
This tutorial has addressed a long-standing challenge for the optical fiber sensor community: how can one detect and analyze media outside the boundaries of the cladding and coating of standard fibers, where light in the single optical core mode cannot reach? One of the most successful solutions has been the use of cladding modes instead. The transverse profiles of cladding modes do reach the outer boundaries of the fiber cladding and perhaps even into coating layers. For the most part, sensing demonstrations have relied on the optical cladding modes of the fiber.24,26–28 The properties of these modes may be affected by the refractive index of an outside substance. However, the coupling of light to and from the optical cladding modes has mandated the inscription of permanent fiber gratings, which restrict the sensors' operation to point measurements only. In recent years, the prospects of sensing using the acoustic cladding modes of the fibers have been introduced as well and have raised much interest.43–54 The stimulation and monitoring of acoustic cladding modes may retrieve the elastic properties of the outside media under test.
The tutorial has been dedicated to two sensing schemes: spatially distributed analysis of coupling spectra to optical cladding modes and sensing based on acoustic cladding modes. Both share optomechanics as a common underlying theme. In the former case, light is coupled to an optical cladding mode by a moving grating of photoelastic perturbations, which is associated with a longitudinal acoustic wave in the core of the fiber. The acoustic wave is generated through a backward stimulated Brillouin scattering process between a pair of pump waves. Acoustic stimulation may be turned on and off at will and can be confined to short fiber sections at arbitrary locations. In the latter case, optical pump waves stimulate an acoustic cladding mode in a forward Brillouin scattering process. The acoustic waves, in turn, are monitored through the coupling of power between the pump waves and/or through the photoelastic scattering of an additional optical probe. Both techniques do not require specialty fibers, modifications to the structure of standard fibers, or the inscription of permanent gratings.
Sensing through both optical and acoustic cladding modes may be carried out with certain coated fibers but is subject to significant limitations. The guiding of optical cladding modes requires that the refractive index of the coating is lower than that of silica and that absorption in the coating is not exceedingly high. Many standard coating materials do not meet these requirements. In addition, the cladding modes of coated fibers thus far used in sensing demonstrations decay within the coating and do not reach its outer edge. Therefore, these modes do not probe the outer medium directly. Sensing using these optical cladding modes is indirect and may only rely on the effects of the surrounding medium on the index of the coating layer. However, optical cladding mode sensing using coated fibers has recently been demonstrated (see Sec. IV). Higher-order optical cladding modes do reach outside the coating boundary; however, their spatial overlap with the optical core mode is greatly reduced. So far, coupling to these modes has not been achieved.
The use of coated fibers in acoustic cladding modes sensors also raises challenges. Here too, certain types of coating absorb the acoustic waves before they reach the outer edge of the coating. Fibers coated with these layers would only support indirect acoustic cladding modes sensing through the effect of the surroundings on the elastic properties of the coating. Compared with the optical cladding modes, however, coating layers that transmit the acoustic cladding modes to their outer edges are more readily found. With these layers, the elastic properties of an outside substance can be probed directly in addition to the study of the coating layer itself.
The techniques presented here are complementary. They may be used to characterize both the optical and elastic properties of the medium under test. Together, they provide a novel and powerful fiber sensing toolset. In one recent example, we combined the two techniques to monitor the effect of acetone on a layer of fluoroacrylate coating outside a standard fiber.40 We found that both the optical and elastic properties of the coating layer varied gradually over a time scale of hours. Immersion in acetone could not be identified by measurements in the optical core mode alone. Both sensing modalities described can become target-specific through proper functionalization of the cladding's outer interface or the coating layers. Most reported experiments were carried out with the fiber placed on a table or coiled up within a dish, and the contact with those surfaces did not compromise the sensing function. However, contact with a solid surface could potentially induce additional losses in optical cladding modes or modify the outward dissipation of acoustic cladding modes. The mounting of fibers in real-world sensing applications would require attention.
Of the two concepts, the use of the optical cladding modes is more sensitive and accurate, and it is more easily scaled to spatially continuous distributed analysis. The probe wave is coupled to an optical cladding mode in the opposite direction; hence, scattering events may be directly localized based on time-of-flight considerations. Protocols of distributed Brillouin optical analysis in the core mode are directly applicable to optical cladding mode sensing; both time-domain and correlation-domain analyses have been demonstrated (Refs. 39 and 40; see Sec. IV). The spatial resolution reached 8 cm. The measurements were sensitive enough to resolve changes to the index outside the cladding at the fourth decimal point.39,40 Although only a short range of 5 m has been demonstrated thus far, the technique is simply scalable to hundreds of meters in length.
Sensing through acoustic cladding modes is more rudimentary. Many demonstrations thus far could only distinguish between air and liquid or between water and ethanol.43,45–54 One experiment identified percent-level changes in the salinity of aqueous solutions,43 and another successfully monitored the dissolved level of sucrose.44 The main difficulty associated with acoustic cladding mode sensors is their distributed analysis: the forward scattering mechanism cannot be mapped directly based on time-of-flight. The most promising solution path to date has been the indirect mapping of local spectra using an auxiliary process of backward stimulated Brillouin scattering.45,53,54 The spatial resolution has reached 80 cm, with over 200 resolution points.54 Performance, however, remains modest. Local scattering contributions are identified through the differentiation of collected data with respect to position, a protocol that is highly susceptible to noise. The forward scattering spectra were successfully mapped in a direct manner using an inter-modal scattering process in polarization maintaining fibers.51 There too, only 17 fiber sections were resolved. Further innovation is required to turn the new modality of acoustic cladding modes fiber sensors into a technology.
In summary, recent advances in optical fiber sensors using optical and acoustic cladding modes have been introduced and explained. The concepts represent breakthroughs in addressing long-standing challenges in the optical fiber sensor community and hold promise for applications in chemical and biological sensing over long reaches. The reader is referred to a recent book75 and to the other references given throughout the text for more detailed reports of specific aspects. The experimental setups and results, in particular, could only be discussed here in a concise form. We hope this tutorial will help introduce these new concepts of cladding mode sensing to students and professionals in fiber-optics and optomechanics and encourage them to invest their own research efforts in similar directions.
AUTHOR DECLARATIONS
Conflict of Interest
The authors have no conflicts to disclose.
Author Contributions
Avi Zadok: Conceptualization (lead); Formal analysis (supporting); Supervision (lead); Writing – original draft (lead); Writing – review & editing (lead). Elad Zehavi: Formal analysis (equal); Investigation (equal); Writing – review & editing (supporting). Alon Bernstein: Formal analysis (equal); Investigation (equal); Writing – review & editing (supporting).
DATA AVAILABILITY
The data that support the findings of this study are available from the corresponding author upon reasonable request.
APPENDIX A: BOUNDARY CONDITIONS EQUATIONS AND TRANSVERSE PROFILES OF OPTICAL CLADDING MODES
The effective indices and the normalized transverse profiles of optical cladding modes are obtained through solutions to the boundary condition equation. The equation was derived and solved in an excellent reference by Erdogan.25 The results are repeated here for completeness and the convenience of the readers.
APPENDIX B: BOUNDARY CONDITIONS EQUATIONS AND TRANSVERSE PROFILES OF ACOUSTIC CORE MODES
Acoustic core modes are guided by the contrast in elastic properties between the core and cladding of standard fibers. The modes of interest are largely confined to the core; hence, we regard the cladding as infinite. We denote the velocities of dilatational acoustic waves in the core and cladding as and , respectively. In germanium-doped cores of standard fibers, .93,94 We assume that the differences in density and in velocity of acoustic shear waves between the two regions are negligible.94 While these approximations take away from the generality of the modal solutions, they nevertheless provide useful estimates for the acoustic core modes of standard optical fibers.