Hexagonal ZnO microrods were employed as whispering-gallery mode (WGM) optical microcavities to investigate exciton-polariton microphotoluminescence and lasing emission. Using a confocal microphotoluminescence system, the exciton-polariton emission with a large Rabi splitting of about 90 meV was observed from a ZnO microrod with the diameter of 9.38μm. The spatial-resolved spectra demonstrated a collective nonlinear blueshift in the WGM resonance peaks along a tapered microrod and proved the anticross dispersion property of the exciton-polariton. Furthermore, the exciton-polariton WGM lasing was stimulated and blueshifted in the strong coupling region under the excitation of a 355 nm nanosecond pulsed laser.

1.
H.
Deng
,
H.
Haug
, and
Y.
Yamamoto
,
Rev. Mod. Phys.
82
,
1489
(
2010
).
2.
H.
Deng
,
G.
Weihs
,
D.
Snoke
,
J.
Bloch
, and
Y.
Yamamoto
,
Proc. Natl. Acad. Sci. U.S.A.
100
,
15318
(
2003
).
3.
G.
Christmann
,
R.
Butté
,
E.
Feltin
,
J. F.
Carlin
, and
N.
Grandjean
,
Appl. Phys. Lett.
93
,
051102
(
2008
).
4.
R.
Huang
,
Y.
Yamamoto
,
R.
Andre
,
J.
Bleuse
,
M.
Muller
, and
H.
Ulmer-Tuffigo
,
Phys. Rev. B
65
,
165314
(
2002
).
5.
S.
Faure
,
T.
Guillet
,
P.
Lefebvre
,
T.
Bretagnon
, and
B.
Gil
,
Phys. Rev. B
78
,
235323
(
2008
).
6.
7.
A. A.
Toropov
,
O. V.
Nekrutkina
,
T. V.
Shubina
,
Th.
Gruber
,
C.
Kirchner
,
A.
Waag
,
K. F.
Karlsson
,
P. O.
Holtz
, and
B.
Monemar
,
Phys. Rev. B
69
,
165205
(
2004
).
8.
J. R.
Chen
,
T. C.
Lu
,
Y. C.
Wu
,
S. C.
Lin
,
W. R.
Liu
,
W. F.
Hsieh
,
C. C.
Kuo
, and
C. C.
Lee
,
Appl. Phys. Lett.
94
,
061103
(
2009
).
9.
A.
Kavokin
,
Phys. Status Solidi B
247
,
1898
(
2010
).
10.
C.
Sturm
,
H.
Hilmer
,
R.
Schmidt-Grund
, and
M.
Grundmann
,
New J. Phys.
11
,
073044
(
2009
).
11.
R.
Schmidt-Grund
,
B.
Rheinländer
,
C.
Czekalla
,
G.
Benndorf
,
H.
Hochmuth
,
M.
Lorenz
, and
M.
Grundmann
,
Appl. Phys. B: Lasers Opt.
93
,
331
(
2008
).
12.
L. K.
van Vugt
,
S.
Ruhle
,
P.
Ravindran
,
H. C.
Gerritsen
,
L.
Kuipers
, and
D.
Vanmaekelbergh
,
Phys. Rev. Lett.
97
,
147401
(
2006
).
13.
S.
Rühle
,
L. K.
van Vugt
,
H. Y.
Li
,
N. A.
Keizer
,
L.
Kuipers
, and
D.
Vanmaekelbergh
,
Nano Lett.
8
,
119
(
2008
).
14.
W. L.
Li
,
M.
Gao
,
X. X.
Zhang
,
D. F.
Liu
,
L. M.
Peng
, and
S. S.
Xie
,
Appl. Phys. Lett.
95
,
173109
(
2009
).
15.
L. X.
Sun
,
Z. H.
Chen
,
Q. J.
Ren
,
K.
Yu
,
L. H.
Bai
,
W. H.
Zhou
,
H.
Xiong
,
Z. Q.
Zhu
, and
X. C.
Shen
,
Phys. Rev. Lett.
100
,
156403
(
2008
).
16.
L. X.
Sun
,
H. X.
Dong
,
W.
Xie
,
Z. H.
An
,
X. C.
Shen
, and
Z. H.
Chen
,
Opt. Express
18
,
15371
(
2010
).
17.
D. J.
Gargas
,
M. C.
Moore
,
A.
Ni
,
S. W.
Chang
,
Z. Y.
Zhang
,
S. L.
Chuang
, and
P. D.
Yang
,
ACS. Nano.
4
,
3270
(
2010
).
18.
C.
Czekalla
,
C.
Sturm
,
R. S.
Grund
,
B. Q.
Cao
,
M.
Lorenz
, and
M.
Grundmann
,
Appl. Phys. Lett.
92
,
241102
(
2008
).
19.
J.
Dai
C. X.
Xu
,
K.
Zheng
,
C. G.
Lv
, and
Y. P.
Cui
,
Appl. Phys. Lett.
95
,
241110
(
2009
).
20.
W. L.
Li
,
M.
Gao
,
R.
Cheng
,
X. X.
Zhang
,
S. S.
Xie
, and
L. M.
Peng
,
Appl. Phys. Lett.
93
,
023117
(
2008
).
21.
J.
Wiersig
,
Phys. Rev. A
67
,
023807
(
2003
).
22.
L. X.
Sun
,
S. L.
Sun
,
H. X.
Dong
,
W.
Xie
,
M.
Richard
,
Lei
Zhou
,
L. S.
Dang
,
X. C.
Shen
, and
Z. H.
Chen
, arXiv:1007.4686v1 (unpublished).
23.
F.
Tassone
,
C.
Piermarocchi
,
V.
Savona
,
A.
Quattropani
, and
P.
Schwendimann
,
Phys. Rev. B
56
,
7554
(
1997
).
You do not currently have access to this content.