Hexagonal ZnO microrods were employed as whispering-gallery mode (WGM) optical microcavities to investigate exciton-polariton microphotoluminescence and lasing emission. Using a confocal microphotoluminescence system, the exciton-polariton emission with a large Rabi splitting of about 90 meV was observed from a ZnO microrod with the diameter of . The spatial-resolved spectra demonstrated a collective nonlinear blueshift in the WGM resonance peaks along a tapered microrod and proved the anticross dispersion property of the exciton-polariton. Furthermore, the exciton-polariton WGM lasing was stimulated and blueshifted in the strong coupling region under the excitation of a 355 nm nanosecond pulsed laser.
REFERENCES
1.
H.
Deng
, H.
Haug
, and Y.
Yamamoto
, Rev. Mod. Phys.
82
, 1489
(2010
).2.
H.
Deng
, G.
Weihs
, D.
Snoke
, J.
Bloch
, and Y.
Yamamoto
, Proc. Natl. Acad. Sci. U.S.A.
100
, 15318
(2003
).3.
G.
Christmann
, R.
Butté
, E.
Feltin
, J. F.
Carlin
, and N.
Grandjean
, Appl. Phys. Lett.
93
, 051102
(2008
).4.
R.
Huang
, Y.
Yamamoto
, R.
Andre
, J.
Bleuse
, M.
Muller
, and H.
Ulmer-Tuffigo
, Phys. Rev. B
65
, 165314
(2002
).5.
S.
Faure
, T.
Guillet
, P.
Lefebvre
, T.
Bretagnon
, and B.
Gil
, Phys. Rev. B
78
, 235323
(2008
).6.
J.
Lagois
, Phys. Rev. B
23
, 5511
(1981
).7.
A. A.
Toropov
, O. V.
Nekrutkina
, T. V.
Shubina
, Th.
Gruber
, C.
Kirchner
, A.
Waag
, K. F.
Karlsson
, P. O.
Holtz
, and B.
Monemar
, Phys. Rev. B
69
, 165205
(2004
).8.
J. R.
Chen
, T. C.
Lu
, Y. C.
Wu
, S. C.
Lin
, W. R.
Liu
, W. F.
Hsieh
, C. C.
Kuo
, and C. C.
Lee
, Appl. Phys. Lett.
94
, 061103
(2009
).9.
A.
Kavokin
, Phys. Status Solidi B
247
, 1898
(2010
).10.
C.
Sturm
, H.
Hilmer
, R.
Schmidt-Grund
, and M.
Grundmann
, New J. Phys.
11
, 073044
(2009
).11.
R.
Schmidt-Grund
, B.
Rheinländer
, C.
Czekalla
, G.
Benndorf
, H.
Hochmuth
, M.
Lorenz
, and M.
Grundmann
, Appl. Phys. B: Lasers Opt.
93
, 331
(2008
).12.
L. K.
van Vugt
, S.
Ruhle
, P.
Ravindran
, H. C.
Gerritsen
, L.
Kuipers
, and D.
Vanmaekelbergh
, Phys. Rev. Lett.
97
, 147401
(2006
).13.
S.
Rühle
, L. K.
van Vugt
, H. Y.
Li
, N. A.
Keizer
, L.
Kuipers
, and D.
Vanmaekelbergh
, Nano Lett.
8
, 119
(2008
).14.
W. L.
Li
, M.
Gao
, X. X.
Zhang
, D. F.
Liu
, L. M.
Peng
, and S. S.
Xie
, Appl. Phys. Lett.
95
, 173109
(2009
).15.
L. X.
Sun
, Z. H.
Chen
, Q. J.
Ren
, K.
Yu
, L. H.
Bai
, W. H.
Zhou
, H.
Xiong
, Z. Q.
Zhu
, and X. C.
Shen
, Phys. Rev. Lett.
100
, 156403
(2008
).16.
L. X.
Sun
, H. X.
Dong
, W.
Xie
, Z. H.
An
, X. C.
Shen
, and Z. H.
Chen
, Opt. Express
18
, 15371
(2010
).17.
D. J.
Gargas
, M. C.
Moore
, A.
Ni
, S. W.
Chang
, Z. Y.
Zhang
, S. L.
Chuang
, and P. D.
Yang
, ACS. Nano.
4
, 3270
(2010
).18.
C.
Czekalla
, C.
Sturm
, R. S.
Grund
, B. Q.
Cao
, M.
Lorenz
, and M.
Grundmann
, Appl. Phys. Lett.
92
, 241102
(2008
).19.
J.
Dai
C. X.
Xu
, K.
Zheng
, C. G.
Lv
, and Y. P.
Cui
, Appl. Phys. Lett.
95
, 241110
(2009
).20.
W. L.
Li
, M.
Gao
, R.
Cheng
, X. X.
Zhang
, S. S.
Xie
, and L. M.
Peng
, Appl. Phys. Lett.
93
, 023117
(2008
).21.
J.
Wiersig
, Phys. Rev. A
67
, 023807
(2003
).22.
L. X.
Sun
, S. L.
Sun
, H. X.
Dong
, W.
Xie
, M.
Richard
, Lei
Zhou
, L. S.
Dang
, X. C.
Shen
, and Z. H.
Chen
, arXiv:1007.4686v1 (unpublished).23.
F.
Tassone
, C.
Piermarocchi
, V.
Savona
, A.
Quattropani
, and P.
Schwendimann
, Phys. Rev. B
56
, 7554
(1997
).© 2011 American Institute of Physics.
2011
American Institute of Physics
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