We have investigated the effects of growth interval in pulsed laser deposition on structural, magnetic, and electrical transport properties of (111)-oriented double perovskite films. It was found that the degree of B-site ordering varied in a wide range by just changing the growth interval. Magnetization under 1 T and metallicity (the ratio of room-temperature resistivity to minimum resistivity at low temperatures) monotonically increased with increasing degree of ordering and reached values nearly identical to bulk. This technique, called pulsed laser interval deposition, may provide more efficient way to study relations between structural and physical properties in double perovskites than controlling growth parameters, such as temperature and oxygen partial pressure.
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13 December 2010
Research Article|
December 15 2010
Controlled B-site ordering in double perovskite films by using pulsed laser interval deposition Available to Purchase
S. Chakraverty;
S. Chakraverty
a)
1Institute for Materials Research,
Tohoku University
, Sendai 980-8577, Japan
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A. Ohtomo;
A. Ohtomo
2Department of Applied Chemistry,
Tokyo Institute of Technology
, Tokyo 152-8552, Japan
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M. Kawasaki
M. Kawasaki
1Institute for Materials Research,
Tohoku University
, Sendai 980-8577, Japan
3WPI Advanced Institute for Materials Research,
Tohoku University
, Sendai 980-8577, Japan
and CREST, Japan Science and Technology Agency
, Tokyo 102-0075, Japan
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S. Chakraverty
1,a)
A. Ohtomo
2
M. Kawasaki
1,3
1Institute for Materials Research,
Tohoku University
, Sendai 980-8577, Japan
2Department of Applied Chemistry,
Tokyo Institute of Technology
, Tokyo 152-8552, Japan
3WPI Advanced Institute for Materials Research,
Tohoku University
, Sendai 980-8577, Japan
and CREST, Japan Science and Technology Agency
, Tokyo 102-0075, Japan
a)
Electronic mail: [email protected].
Appl. Phys. Lett. 97, 243107 (2010)
Article history
Received:
September 13 2010
Accepted:
November 17 2010
Citation
S. Chakraverty, A. Ohtomo, M. Kawasaki; Controlled B-site ordering in double perovskite films by using pulsed laser interval deposition. Appl. Phys. Lett. 13 December 2010; 97 (24): 243107. https://doi.org/10.1063/1.3525578
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