We describe an ultrasensitive atomic magnetometer based on optically pumped potassium atoms operating in a spin-exchange relaxation free regime. We demonstrate magnetic field sensitivity of 160aT/Hz1/2 in a gradiometer arrangement with a measurement volume of 0.45cm3 and energy resolution per unit bandwidth of 44. As an example of an application enabled by such a magnetometer, we describe measurements of weak remnant rock magnetization as a function of temperature with a sensitivity on the order of 1010emu/cm3/Hz1/2 and temperatures up to 420°C.

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