The authors report on efficient spin injection from a n-Zn0.96Mn0.04Se layer into an InAs single quantum dot (SQD) in a p-i-n diode structure using magnetomicrophotoluminescence experiments. A circular polarization degree of up to 60% at B=5T is obtained from the InAs single dot emission while no polarized light is observed in a structure with no electrical doping of any of its layers. A pronounced dependence of the spin injection efficiency on the external bias is found resulting in a strong decrease of the SQD circular polarization degree when the biasing is applied in the forward direction. The experiments emphasize the impact of excess energy and current flow on the spin injection efficiency in a SQD.

1.
M.
Kroutvar
,
Y.
Ducommun
,
D.
Heiss
,
M.
Bichler
,
D.
Schuh
,
G.
Abstreiter
, and
J. J.
Finley
,
Nature (London)
432
,
81
(
2004
).
2.
R. I.
Dzhioev
,
K. V.
Kavokin
,
V. L.
Korenev
,
M. V.
Lazarev
,
B. Ya.
Meltscer
,
M. N.
Stepanova
,
B. P.
Zakharchenya
,
D.
Gammon
, and
D. S.
Katzer
,
Phys. Rev. B
66
,
245204
(
2002
).
3.
Y.
Ohno
,
R.
Terauchi
,
T.
Adachi
,
F.
Matsukura
, and
H.
Ohno
,
Phys. Rev. Lett.
83
,
4196
(
1999
).
4.
J. M.
Elzerman
,
R.
Hanson
,
L. H.
Willems Van Beveren
,
B.
Witkamp
,
L. M. K.
Vandersypen
, and
L. P.
Kouwenhoven
,
Nature (London)
430
,
431
(
2004
).
5.
I.
Malajovich
,
J. J.
Berry
,
N.
Samarth
, and
D. D.
Awschalom
,
Nature (London)
411
,
770
(
2001
).
6.
M.
Oestreich
,
J.
Hübner
,
D.
Hägele
,
P. J.
Klar
,
W.
Heimbrodt
,
W. W.
Rühle
,
D. E.
Ashenford
, and
B.
Lunn
,
Appl. Phys. Lett.
74
,
1251
(
1999
).
7.
R.
Fiederling
,
M.
Keim
,
G.
Reuscher
,
W.
Ossau
,
G.
Schmidt
,
A.
Waag
, and
L. W.
Molenkamp
,
Nature (London)
402
,
787
(
1999
).
8.
M.
Ghali
,
J.
Kossut
,
E.
Janik
,
K.
Regiński
, and
Ł.
Kłopotowski
,
Solid State Commun.
119
,
371
(
2001
).
9.
Y.
Ohno
,
D. K.
Young
,
B.
Beschoten
,
F.
Matsukura
,
H.
Ohno
, and
D. D.
Awschalom
,
Nature (London)
402
,
790
(
1999
).
10.
A. T.
Hanbicki
,
O. M. J.
Van’t Erve
,
R.
Magno
,
G.
Kioseoglou
,
C. H.
Li
,
B. T.
Jonker
,
R.
Mallory
,
M.
Yasar
, and
A.
Petrou
,
Appl. Phys. Lett.
82
,
4092
(
2003
).
11.
G.
Itskos
,
E.
Harbord
,
S. K.
Clowes
,
E.
Clarke
,
L. F.
Cohen
,
R.
Murray
,
P.
Van Dorpe
, and
W.
Van Roy
,
Appl. Phys. Lett.
88
,
022113
(
2006
).
12.
C. H.
Li
,
G.
Kioseoglou
,
O. M. J.
Van’t Erve
,
M. E.
Ware
,
D.
Gammon
,
R. M.
Stroud
,
B. T.
Jonker
,
R.
Allory
,
M.
Yasar
, and
A.
Petrou
,
Appl. Phys. Lett.
86
,
132503
(
2005
).
13.
W.
Löffler
,
D.
Tröndle
,
J.
Fallert
,
H.
Kalt
,
D.
Litvinov
,
D.
Gerthsen
,
J.
Lupaca-Schomber
,
T.
Passow
,
B.
Daniel
,
J.
Kvietkova
,
M.
Grün
,
C.
Klingshirn
, and
M.
Hetterich
,
Appl. Phys. Lett.
88
,
062105
(
2006
).
14.
J.
Seufert
,
G.
Bacher
,
H.
Schömig
,
A.
Forchel
,
L.
Hansen
,
G.
Schmidt
, and
L. W.
Molenkamp
,
Phys. Rev. B
69
,
035311
(
2004
).
15.
R.
Nicolini
,
L.
Vanzetti
,
Guido
Mula
,
G.
Bratina
,
L.
Sorba
,
A.
Franciosi
,
M.
Peressi
,
S.
Baroni
,
R.
Resta
,
A.
Baldereschi
,
J. E.
Angelo
, and
W. W.
Gerberich
,
Phys. Rev. Lett.
72
,
294
(
1994
).
16.
G.
Fishman
and
G.
Lampel
,
Phys. Rev. B
16
,
820
(
1977
).
17.

Note that the optical spin injection observed in undoped ZnMnTeGaAs heterostructures (Ref. 8) might be attributed to the significantly smaller band gap difference and/or the significant (factor of 10) larger thickness of the spin aligner in this ZnMnTeGaAs system as compared to our ZnMnSeGaAs structure.

18.
M.
Bayer
,
G.
Ortner
,
O.
Stern
,
A.
Kuther
,
A. A.
Gorbunov
,
A.
Forchel
,
P.
Hawrylak
,
S.
Fafard
,
K.
Hinzer
,
J. P.
Reithmaier
,
F.
Klopf
, and
F.
Schafer
,
Phys. Rev. B
65
,
195315
(
2002
).
19.

We assume a complete spin relaxation of the heavy holes before they reach the QD ground state.

20.
Diluted Magnetic Semiconductors
,
Semiconductor and Semimetals
Vol.
25
, edited by
J. K.
Furdyna
and
J.
Kossut
(
Academic
,
New York
,
1988
.
21.
P.
Van Dorpe
,
Z.
Liu
,
W.
Van Roy
,
V. F.
Motsny
,
M.
Sawicki
,
G.
Borghs
, and
J.
De Boeck
,
Appl. Phys. Lett.
84
,
3495
(
2004
).
22.
X.
Jiang
,
R.
Wang
,
S.
Van Dijken
,
R.
Shelby
,
R.
Macfarlane
,
G. S.
Solomon
,
J.
Harris
, and
S. S. P.
Parkin
,
Phys. Rev. Lett.
90
,
256603
(
2003
).
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