Inelastic light scattering from a single isolated silica sphere, of diameter as small as , has been measured as a function of sphere size by micro-Brillouin spectroscopy. The feasibility of recording spectra of a sample as tiny as this, and for which only one particle is needed, further enhances the capabilities of Brillouin light scattering as a powerful investigative tool. Such measurements afford the evaluation of the elastic properties of single nanospheres and a determination of the size polydispersity of an aggregate of particles from the asymmetric broadening of its Brillouin spectrum. Unlike conventional Brillouin scattering from acoustic waves, what is observed here is the inelastic scattering from the eigenvibrations of a nanosphere.
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9 January 2006
Research Article|
January 12 2006
Micro-Brillouin scattering from a single isolated nanosphere
Y. Li;
Y. Li
Department of Physics,
National University of Singapore
, 2 Science Drive 3, Singapore 117542, Singapore
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H. S. Lim;
H. S. Lim
Department of Physics,
National University of Singapore
, 2 Science Drive 3, Singapore 117542, Singapore
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S. C. Ng;
S. C. Ng
Department of Physics,
National University of Singapore
, 2 Science Drive 3, Singapore 117542, Singapore
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Z. K. Wang;
Z. K. Wang
Department of Physics,
National University of Singapore
, 2 Science Drive 3, Singapore 117542, Singapore
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M. H. Kuok;
M. H. Kuok
a)
Department of Physics,
National University of Singapore
, 2 Science Drive 3, Singapore 117542, Singapore
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E. Vekris;
E. Vekris
Department of Chemistry,
University of Toronto
, Toronto, Ontario M5S 3H6, Canada
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V. Kitaev;
V. Kitaev
Department of Chemistry,
University of Toronto
, Toronto, Ontario M5S 3H6, Canada
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F. C. Peiris;
F. C. Peiris
Department of Chemistry,
University of Toronto
, Toronto, Ontario M5S 3H6, Canada
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G. A. Ozin
G. A. Ozin
Department of Chemistry,
University of Toronto
, Toronto, Ontario M5S 3H6, Canada
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a)
Author to whom correspondence should be addressed; electronic mail: phykmh@nus.edu.sg
Appl. Phys. Lett. 88, 023112 (2006)
Article history
Received:
June 27 2005
Accepted:
November 18 2005
Citation
Y. Li, H. S. Lim, S. C. Ng, Z. K. Wang, M. H. Kuok, E. Vekris, V. Kitaev, F. C. Peiris, G. A. Ozin; Micro-Brillouin scattering from a single isolated nanosphere. Appl. Phys. Lett. 9 January 2006; 88 (2): 023112. https://doi.org/10.1063/1.2164924
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