We present a terahertz (THz) system based on a poled electro-optic (EO) polymer emitter-sensor pair for the generation and detection of broadband electromagnetic pulses free of spectral gaps. The gap-free THz spectrum obtained from the system is attributed to the amorphous form of the EO polymer films. Using 50-fs laser pulses centered at 800nm, a 100-μm thick emitter, and a 180-μm thick sensor, the observable bandwidth is 12THz. We also present an experimental study, in a systematic manner, on the effect of phase mismatch in the polymer emitter-sensor pair.

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