Two-dimensional tellurium (Te) has been intensely studied in recent years due to its outstanding electrical properties and excellent air stability. Simple and effective contact engineering is highly desirable to further improve its device performance. In this work, we demonstrate a simple strategy to largely improve the metal–Te contact quality by forming an ultrathin tellurium oxide layer in the contact region via O2 plasma treatment. The surface oxide doped the underlying Te layers degenerately due to charge transfer, establishing an Ohmic contact between Pd electrode and Te with negative Schottky barrier under flatband condition. This enables Te field-effect transistor to achieve outstanding electronic performance, including a record-low contact resistance of ∼0.16 kΩ·μm and a high field-effect mobility of ∼1015 cm2V−1s−1 (∼3002 cm2V−1s−1) at room temperature (low temperature). The simplicity and CMOS compatibility of O2 plasma treatment make it a promising candidate for applications in Te-based large-scale integrated circuits.
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Oxygen plasma induced improvement of contact resistance and mobility of tellurium field-effect transistor
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12 May 2025
Research Article|
May 13 2025
Oxygen plasma induced improvement of contact resistance and mobility of tellurium field-effect transistor
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Jinwei Hu;
Jinwei Hu
(Data curation, Formal analysis, Investigation, Methodology, Visualization, Writing – original draft)
Department of Physics, Engineering Research Center for Micro-Nano Optoelectronic Materials and Devices of Ministry of Education, Fujian Provincial Key Laboratory of Semiconductor Materials and Applications, Research Institute for Biomimetics and Soft Matter, Fujian Provincial Key Laboratory for Soft Functional Materials, Xiamen University
, Xiamen 361005, China
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Bosen Wang;
Bosen Wang
(Data curation, Formal analysis, Investigation, Methodology, Visualization, Writing – original draft)
Department of Physics, Engineering Research Center for Micro-Nano Optoelectronic Materials and Devices of Ministry of Education, Fujian Provincial Key Laboratory of Semiconductor Materials and Applications, Research Institute for Biomimetics and Soft Matter, Fujian Provincial Key Laboratory for Soft Functional Materials, Xiamen University
, Xiamen 361005, China
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Xingyun Li;
Xingyun Li
(Data curation, Formal analysis, Investigation, Methodology, Writing – review & editing)
Department of Physics, Engineering Research Center for Micro-Nano Optoelectronic Materials and Devices of Ministry of Education, Fujian Provincial Key Laboratory of Semiconductor Materials and Applications, Research Institute for Biomimetics and Soft Matter, Fujian Provincial Key Laboratory for Soft Functional Materials, Xiamen University
, Xiamen 361005, China
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Ming Yuwen;
Ming Yuwen
(Data curation, Formal analysis, Investigation, Methodology, Writing – review & editing)
Department of Physics, Engineering Research Center for Micro-Nano Optoelectronic Materials and Devices of Ministry of Education, Fujian Provincial Key Laboratory of Semiconductor Materials and Applications, Research Institute for Biomimetics and Soft Matter, Fujian Provincial Key Laboratory for Soft Functional Materials, Xiamen University
, Xiamen 361005, China
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Bo Zhang;
Bo Zhang
(Data curation, Formal analysis, Investigation, Methodology, Writing – review & editing)
Department of Physics, Engineering Research Center for Micro-Nano Optoelectronic Materials and Devices of Ministry of Education, Fujian Provincial Key Laboratory of Semiconductor Materials and Applications, Research Institute for Biomimetics and Soft Matter, Fujian Provincial Key Laboratory for Soft Functional Materials, Xiamen University
, Xiamen 361005, China
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Lianying Zhu;
Lianying Zhu
(Data curation, Formal analysis, Investigation, Methodology, Writing – review & editing)
Department of Physics, Engineering Research Center for Micro-Nano Optoelectronic Materials and Devices of Ministry of Education, Fujian Provincial Key Laboratory of Semiconductor Materials and Applications, Research Institute for Biomimetics and Soft Matter, Fujian Provincial Key Laboratory for Soft Functional Materials, Xiamen University
, Xiamen 361005, China
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Jun Xu
;
Jun Xu
a)
(Conceptualization, Funding acquisition, Project administration, Supervision, Writing – review & editing)
Department of Physics, Engineering Research Center for Micro-Nano Optoelectronic Materials and Devices of Ministry of Education, Fujian Provincial Key Laboratory of Semiconductor Materials and Applications, Research Institute for Biomimetics and Soft Matter, Fujian Provincial Key Laboratory for Soft Functional Materials, Xiamen University
, Xiamen 361005, China
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Deyi Fu
;
Deyi Fu
a)
(Conceptualization, Funding acquisition, Project administration, Supervision, Validation, Writing – review & editing)
Department of Physics, Engineering Research Center for Micro-Nano Optoelectronic Materials and Devices of Ministry of Education, Fujian Provincial Key Laboratory of Semiconductor Materials and Applications, Research Institute for Biomimetics and Soft Matter, Fujian Provincial Key Laboratory for Soft Functional Materials, Xiamen University
, Xiamen 361005, China
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Rong Zhang
Rong Zhang
(Conceptualization, Funding acquisition, Writing – review & editing)
Department of Physics, Engineering Research Center for Micro-Nano Optoelectronic Materials and Devices of Ministry of Education, Fujian Provincial Key Laboratory of Semiconductor Materials and Applications, Research Institute for Biomimetics and Soft Matter, Fujian Provincial Key Laboratory for Soft Functional Materials, Xiamen University
, Xiamen 361005, China
Search for other works by this author on:
Jinwei Hu
Data curation, Formal analysis, Investigation, Methodology, Visualization, Writing – original draft
Department of Physics, Engineering Research Center for Micro-Nano Optoelectronic Materials and Devices of Ministry of Education, Fujian Provincial Key Laboratory of Semiconductor Materials and Applications, Research Institute for Biomimetics and Soft Matter, Fujian Provincial Key Laboratory for Soft Functional Materials, Xiamen University
, Xiamen 361005, China
Bosen Wang
Data curation, Formal analysis, Investigation, Methodology, Visualization, Writing – original draft
Department of Physics, Engineering Research Center for Micro-Nano Optoelectronic Materials and Devices of Ministry of Education, Fujian Provincial Key Laboratory of Semiconductor Materials and Applications, Research Institute for Biomimetics and Soft Matter, Fujian Provincial Key Laboratory for Soft Functional Materials, Xiamen University
, Xiamen 361005, China
Xingyun Li
Data curation, Formal analysis, Investigation, Methodology, Writing – review & editing
Department of Physics, Engineering Research Center for Micro-Nano Optoelectronic Materials and Devices of Ministry of Education, Fujian Provincial Key Laboratory of Semiconductor Materials and Applications, Research Institute for Biomimetics and Soft Matter, Fujian Provincial Key Laboratory for Soft Functional Materials, Xiamen University
, Xiamen 361005, China
Ming Yuwen
Data curation, Formal analysis, Investigation, Methodology, Writing – review & editing
Department of Physics, Engineering Research Center for Micro-Nano Optoelectronic Materials and Devices of Ministry of Education, Fujian Provincial Key Laboratory of Semiconductor Materials and Applications, Research Institute for Biomimetics and Soft Matter, Fujian Provincial Key Laboratory for Soft Functional Materials, Xiamen University
, Xiamen 361005, China
Bo Zhang
Data curation, Formal analysis, Investigation, Methodology, Writing – review & editing
Department of Physics, Engineering Research Center for Micro-Nano Optoelectronic Materials and Devices of Ministry of Education, Fujian Provincial Key Laboratory of Semiconductor Materials and Applications, Research Institute for Biomimetics and Soft Matter, Fujian Provincial Key Laboratory for Soft Functional Materials, Xiamen University
, Xiamen 361005, China
Lianying Zhu
Data curation, Formal analysis, Investigation, Methodology, Writing – review & editing
Department of Physics, Engineering Research Center for Micro-Nano Optoelectronic Materials and Devices of Ministry of Education, Fujian Provincial Key Laboratory of Semiconductor Materials and Applications, Research Institute for Biomimetics and Soft Matter, Fujian Provincial Key Laboratory for Soft Functional Materials, Xiamen University
, Xiamen 361005, China
Jun Xu
Conceptualization, Funding acquisition, Project administration, Supervision, Writing – review & editing
a)
Department of Physics, Engineering Research Center for Micro-Nano Optoelectronic Materials and Devices of Ministry of Education, Fujian Provincial Key Laboratory of Semiconductor Materials and Applications, Research Institute for Biomimetics and Soft Matter, Fujian Provincial Key Laboratory for Soft Functional Materials, Xiamen University
, Xiamen 361005, China
Deyi Fu
Conceptualization, Funding acquisition, Project administration, Supervision, Validation, Writing – review & editing
a)
Department of Physics, Engineering Research Center for Micro-Nano Optoelectronic Materials and Devices of Ministry of Education, Fujian Provincial Key Laboratory of Semiconductor Materials and Applications, Research Institute for Biomimetics and Soft Matter, Fujian Provincial Key Laboratory for Soft Functional Materials, Xiamen University
, Xiamen 361005, China
Rong Zhang
Conceptualization, Funding acquisition, Writing – review & editing
Department of Physics, Engineering Research Center for Micro-Nano Optoelectronic Materials and Devices of Ministry of Education, Fujian Provincial Key Laboratory of Semiconductor Materials and Applications, Research Institute for Biomimetics and Soft Matter, Fujian Provincial Key Laboratory for Soft Functional Materials, Xiamen University
, Xiamen 361005, China
Appl. Phys. Lett. 126, 193101 (2025)
Article history
Received:
January 28 2025
Accepted:
April 27 2025
Citation
Jinwei Hu, Bosen Wang, Xingyun Li, Ming Yuwen, Bo Zhang, Lianying Zhu, Jun Xu, Deyi Fu, Rong Zhang; Oxygen plasma induced improvement of contact resistance and mobility of tellurium field-effect transistor. Appl. Phys. Lett. 12 May 2025; 126 (19): 193101. https://doi.org/10.1063/5.0260965
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