Transparent ferroelectric materials have been attracting enormous attention due to their simultaneously ultrahigh transparency and piezoelectricity, which are highly desirable for electro-optical-mechanical devices. However, it is very challenging to achieve excellent optical transparency in ferroelectric materials because of the severe light scattering of the domain wall. Here, a domain wall scattering model is developed to reveal the mechanism of light scattering caused by domain walls and to quantitatively calculate the scattering of light by different domain walls. The reliability of such a model is verified by the good agreement between theoretical predictions and recent experimental measurements. Based on the model, both domain wall type and orientation are found to greatly determine the transmittance of transparent ferroelectric crystals. The influence of domain size is also investigated. This work provides a theoretical basis for regulating the transmittance of transparent ferroelectric crystals through domain wall engineering.
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12 May 2025
Research Article|
May 13 2025
Domain wall scattering determining the transmittance of transparent ferroelectric crystals Available to Purchase
Zixiang Xiong
;
Zixiang Xiong
(Conceptualization, Data curation, Formal analysis, Investigation, Methodology, Validation, Visualization, Writing – original draft, Writing – review & editing)
1
Centre for Theoretical and Computational Physics, College of Physics, Qingdao University
, Qingdao 266071, People's Republic of China
2
College of Physics, University-Industry Joint Center for Ocean Observation and Broadband Communication, National Demonstration Center for Experimental Applied Physics Education, Qingdao University
, Qingdao 266071, People's Republic of China
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Jian Zhu;
Jian Zhu
(Data curation, Formal analysis, Investigation, Methodology, Validation, Visualization, Writing – original draft)
1
Centre for Theoretical and Computational Physics, College of Physics, Qingdao University
, Qingdao 266071, People's Republic of China
2
College of Physics, University-Industry Joint Center for Ocean Observation and Broadband Communication, National Demonstration Center for Experimental Applied Physics Education, Qingdao University
, Qingdao 266071, People's Republic of China
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Jiaxin Ma;
Jiaxin Ma
(Data curation, Formal analysis, Investigation, Methodology, Validation, Visualization)
1
Centre for Theoretical and Computational Physics, College of Physics, Qingdao University
, Qingdao 266071, People's Republic of China
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Kexin Zhang;
Kexin Zhang
(Data curation, Formal analysis, Investigation, Methodology, Validation, Visualization)
1
Centre for Theoretical and Computational Physics, College of Physics, Qingdao University
, Qingdao 266071, People's Republic of China
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Yongcheng Zhang
;
Yongcheng Zhang
a)
(Conceptualization, Formal analysis, Funding acquisition, Investigation, Methodology, Project administration, Resources, Supervision, Validation, Writing – original draft, Writing – review & editing)
1
Centre for Theoretical and Computational Physics, College of Physics, Qingdao University
, Qingdao 266071, People's Republic of China
2
College of Physics, University-Industry Joint Center for Ocean Observation and Broadband Communication, National Demonstration Center for Experimental Applied Physics Education, Qingdao University
, Qingdao 266071, People's Republic of China
Search for other works by this author on:
Jianyi Liu
Jianyi Liu
a)
(Conceptualization, Formal analysis, Funding acquisition, Investigation, Methodology, Project administration, Resources, Supervision, Validation, Writing – original draft, Writing – review & editing)
1
Centre for Theoretical and Computational Physics, College of Physics, Qingdao University
, Qingdao 266071, People's Republic of China
2
College of Physics, University-Industry Joint Center for Ocean Observation and Broadband Communication, National Demonstration Center for Experimental Applied Physics Education, Qingdao University
, Qingdao 266071, People's Republic of China
3
Guangdong Provincial Key Laboratory of Magnetoelectric Physics and Devices, School of Physics, Sun Yat-sen University, Guangzhou 510275
, People's Republic of China
4
Centre for Physical Mechanics and Biophysics, School of Physics, Sun Yat-sen University
, Guangzhou 510275, People's Republic of China
Search for other works by this author on:
Zixiang Xiong
1,2
Jian Zhu
1,2
Jiaxin Ma
1
Kexin Zhang
1
Yongcheng Zhang
1,2,a)
Jianyi Liu
1,2,3,4,a)
1
Centre for Theoretical and Computational Physics, College of Physics, Qingdao University
, Qingdao 266071, People's Republic of China
2
College of Physics, University-Industry Joint Center for Ocean Observation and Broadband Communication, National Demonstration Center for Experimental Applied Physics Education, Qingdao University
, Qingdao 266071, People's Republic of China
3
Guangdong Provincial Key Laboratory of Magnetoelectric Physics and Devices, School of Physics, Sun Yat-sen University, Guangzhou 510275
, People's Republic of China
4
Centre for Physical Mechanics and Biophysics, School of Physics, Sun Yat-sen University
, Guangzhou 510275, People's Republic of China
Appl. Phys. Lett. 126, 191901 (2025)
Article history
Received:
January 23 2025
Accepted:
April 25 2025
Citation
Zixiang Xiong, Jian Zhu, Jiaxin Ma, Kexin Zhang, Yongcheng Zhang, Jianyi Liu; Domain wall scattering determining the transmittance of transparent ferroelectric crystals. Appl. Phys. Lett. 12 May 2025; 126 (19): 191901. https://doi.org/10.1063/5.0260262
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