Narrow-gap Fe-doped III–V ferromagnetic semiconductors (FMSs), such as (In,Fe)Sb, (Ga,Fe)Sb, and (In,Fe)Sb, are promising candidates for active semiconductor spintronic devices thanks to their high Curie temperature (TC). In this work, we show that by growing (Ga,Fe)Sb thin films by the step-flow mode on vicinal GaAs (100) substrates with a high off-angle of 10°, we can achieve high-quality (Ga0.76,Fe0.24)Sb FMS with TC as high as 470–530 K, which are the highest TC reported so far for FMSs. The magnetic moment of Fe atoms in our sample reaches 4.5 μB/atom, which is close to the ideal magnetic moment of substitutional Fe3+ atoms (5 μB/atom) in a zinc blende crystal structure, and is twice that of α-Fe metal. Our work establishes a growth technique of very high TC FMSs for room-temperature semiconductor spintronic devices.
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21 April 2025
Research Article|
April 24 2025
Very high Curie temperature (470–530 K) in (Ga,Fe)Sb ferromagnetic semiconductor grown by step-flow mode on vicinal GaAs substrates Available to Purchase
Pham Nam Hai
;
Pham Nam Hai
a)
(Conceptualization, Funding acquisition, Project administration, Resources, Supervision, Validation, Visualization, Writing – original draft, Writing – review & editing)
1
Department of Electrical and Electronic Engineering, Tokyo Institute of Technology
, 2-12-1 Ookayama, Meguro, Tokyo 152-0033, Japan
a)Author to whom correspondence should be addressed: [email protected]
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Ken Takabayashi;
Ken Takabayashi
(Data curation, Formal analysis, Investigation, Methodology, Visualization)
1
Department of Electrical and Electronic Engineering, Tokyo Institute of Technology
, 2-12-1 Ookayama, Meguro, Tokyo 152-0033, Japan
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Kota Ejiri;
Kota Ejiri
(Investigation, Resources)
1
Department of Electrical and Electronic Engineering, Tokyo Institute of Technology
, 2-12-1 Ookayama, Meguro, Tokyo 152-0033, Japan
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Masaaki Tanaka
Masaaki Tanaka
(Resources, Validation, Writing – review & editing)
2
Department of Electrical Engineering & Information Systems, The University of Tokyo
, 7-3-1 Hongo, Bunkyo, Tokyo 113-8656, Japan
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Pham Nam Hai
1,a)
Ken Takabayashi
1
Kota Ejiri
1
Masaaki Tanaka
2
1
Department of Electrical and Electronic Engineering, Tokyo Institute of Technology
, 2-12-1 Ookayama, Meguro, Tokyo 152-0033, Japan
2
Department of Electrical Engineering & Information Systems, The University of Tokyo
, 7-3-1 Hongo, Bunkyo, Tokyo 113-8656, Japan
a)Author to whom correspondence should be addressed: [email protected]
Appl. Phys. Lett. 126, 162407 (2025)
Article history
Received:
July 11 2024
Accepted:
April 13 2025
Citation
Pham Nam Hai, Ken Takabayashi, Kota Ejiri, Masaaki Tanaka; Very high Curie temperature (470–530 K) in (Ga,Fe)Sb ferromagnetic semiconductor grown by step-flow mode on vicinal GaAs substrates. Appl. Phys. Lett. 21 April 2025; 126 (16): 162407. https://doi.org/10.1063/5.0227990
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