The in situ and ex situ temperature dependence of dielectric and piezoelectric properties of 0.1(Bi0.5K0.5)TiO3-0.6BiFeO3-0.3PbTiO3 (BKT-BFPT) ceramics were characterized, and related mechanisms were studied. The tetragonal distortion, Curie temperature Tc, depoling temperature Td, and piezoelectric coefficient d33 of BKT-BFPT are 0.06, 545 °C, 520 °C, and 205 pC/N, respectively. The in situ piezoelectric coefficient variation of BKT-BFPT ceramics from room temperature to 280 °C is only 10%, being 1/5 and 1/10 those of 0.36BiScO3-0.34PbTiO3 and Pb(Zr0.52Ti0.48)O3 ceramics. The better dielectric and piezoelectric thermal stabilities are owing to the temperature insensitive domain texture of BFPT-BKT ceramics due to their large lattice distortion. Resistivity results reflected that the higher depoling temperature derived from the ex situ measurement than that from the in situ test results from the high-temperature conductivity.

Topics
Ferromagnetism, Phase transitions, Piezoelectricity, Measurement theory, Dielectric properties, Ferroelectric materials, Materials properties, Polymers, X-ray diffraction, Ceramics
1.
F.
Li
,
D. B.
Lin
,
Z. B.
Chen
,
Z. X.
Cheng
,
J. L.
Wang
,
C. C.
Li
,
Z.
Xu
,
Q. W.
Huang
,
X. Z.
Liao
,
L. Q.
Chen
,
T. R.
Shrout
, and
S. J.
Zhang
,
Nat. Mater.
17
(
4
),
349
(
2018
).
https://doi.org/10.1038/s41563-018-0034-4
Google Scholar
Crossref
Search ADS
PubMed
 
2.
X. Y.
Gao
,
Z. X.
Cheng
,
Z. B.
Chen
,
Y.
Liu
,
X. Y.
Meng
,
X.
Zhang
,
J. L.
Wang
,
Q. H.
Guo
,
B.
Li
,
H. J.
Sun
,
Q. F.
Gu
,
H.
Hao
,
Q.
Shen
,
J. S.
Wu
,
X. Z.
Liao
,
S. P.
Ringer
,
H. X.
Liu
,
L. M.
Zhang
,
W.
Chen
,
F.
Li
, and
S. J.
Zhang
,
Nat. Commun.
12
(
1
),
881
(
2021
).
https://doi.org/10.1038/s41467-021-21202-7
Google Scholar
Crossref
Search ADS
PubMed
 
4.
D. I.
Woodward
,
I. M.
Reaney
,
R. E.
Eitel
, and
C. A.
Randall
,
J. Appl. Phys.
94
(
5
),
3313
(
2003
).
https://doi.org/10.1063/1.1595726
Google Scholar
Crossref
Search ADS
 
5.
S. J.
Zhang
,
C. A.
Randall
, and
T. R.
Shrout
,
Appl. Phys. Lett.
83
(
15
),
3150
(
2003
).
https://doi.org/10.1063/1.1619207
Google Scholar
Crossref
Search ADS
 
6.
C. J.
Stringer
,
T. R.
Shrout
,
C. A.
Randall
, and
I. M.
Reaney
,
J. Appl. Phys.
99
(
2
),
024106
(
2006
).
https://doi.org/10.1063/1.2163986
Google Scholar
Crossref
Search ADS
 
7.
H.
Qin
,
J.
Zhao
,
X.
Chen
,
H.
Li
,
S.
Wang
,
Y.
Du
,
H.
Zhou
,
P.
Li
, and
D.
Wang
,
Microstructures
3
,
2023035
(
2023
).
https://doi.org/10.20517/microstructures.2023.34
Google Scholar
Crossref
Search ADS
 
8.
R.
Dai
,
J. G.
Chen
, and
J. R.
Cheng
,
Ceram. Int.
40
(
8
),
13299
(
2014
).
https://doi.org/10.1016/j.ceramint.2014.05.042
Google Scholar
Crossref
Search ADS
 
9.
A.
Singh
 and
R.
Chatterjee
,
Ferroelectrics
433
,
180
(
2012
).
https://doi.org/10.1080/00150193.2012.722462
Google Scholar
Crossref
Search ADS
 
10.
D. F.
Chen
 and
J. R.
Cheng
,
J. Sol-Gel Sci. Technol.
85
(
2
),
431
(
2018
).
https://doi.org/10.1007/s10971-017-4549-y
Google Scholar
Crossref
Search ADS
 
11.
X. B.
Hou
 and
J.
Yu
,
J. Am. Ceram. Soc.
96
(
7
),
2218
(
2013
).
https://doi.org/10.1111/jace.12324
Google Scholar
Crossref
Search ADS
 
12.
J.
Bennett
,
A. J.
Bell
,
T. J.
Stevenson
, and
T. P.
Comyn
,
Scr. Mater.
68
(
7
),
491
(
2013
).
https://doi.org/10.1016/j.scriptamat.2012.11.029
Google Scholar
Crossref
Search ADS
 
13.
J.
Bennett
,
A. J.
Bell
,
T. J.
Stevenson
, and
T. P.
Comyn
,
Appl. Phys. Lett.
103
(
15
),
152901
(
2013
).
https://doi.org/10.1063/1.4824652
Google Scholar
Crossref
Search ADS
 
14.
T.
Sebastian
,
I.
Sterianou
,
D. C.
Sinclair
,
A. J.
Bell
,
D. A.
Hall
, and
I. M.
Reaney
,
J. Electroceram.
25
(
2–4
),
130
(
2010
).
https://doi.org/10.1007/s10832-010-9600-0
Google Scholar
Crossref
Search ADS
 
15.
J.
Jian
,
R.
Peng
,
F.
Luo
,
J. R.
Cheng
, and
J. G.
Chen
,
Ceram. Int.
45
(
11
),
13614
(
2019
).
https://doi.org/10.1016/j.ceramint.2019.03.154
Google Scholar
Crossref
Search ADS
 
16.
W.
Hu
,
X. L.
Tan
, and
K.
Rajan
,
J. Eur. Ceram. Soc.
31
(
5
),
801
(
2011
).
https://doi.org/10.1016/j.jeurceramsoc.2010.11.015
Google Scholar
Crossref
Search ADS
 
17.
J.
Fu
,
Z. D.
Yu
,
A. W.
Xie
,
Z. Y.
Yu
,
Z. Q.
Fu
,
X. W.
Jiang
,
T. Y.
Li
, and
R. Z.
Zuo
,
Acta Mater.
254
,
118991
(
2023
).
https://doi.org/10.1016/j.actamat.2023.118991
Google Scholar
Crossref
Search ADS
 
18.
L. L.
Fan
,
J.
Chen
,
S.
Li
,
H. J.
Kang
,
L. J.
Liu
,
L.
Fang
, and
X. R.
Xing
,
Appl. Phys. Lett.
102
(
2
),
022905
(
2013
).
https://doi.org/10.1063/1.4775763
Google Scholar
Crossref
Search ADS
 
19.
H. H.
Law
,
P. L.
Rossiter
, and
G. P.
Simon
,
J. Mater. Sci.
30
,
4901
(
1995
).
https://doi.org/10.1007/BF01154502
Google Scholar
Crossref
Search ADS
 
20.
J.
Bennett
,
T. R.
Shorut
,
S. J.
Zhang
,
P.
Mandal
,
A. J.
Bell
,
T. J.
Stevenson
, and
T. P.
Comyn
, “
Temperature dependent of the intrinsic and extrinsic contributions in BiFeO3-(K0.5Bi0.5)TiO3-PbTiO3 piezoelectric ceramics
,”
J. Appl. Phys.
116
,
094102
(
2014
).
https://doi.org/10.1063/1.4894443
Google Scholar
Crossref
Search ADS
 
21.
B.
Narayan
,
J. S.
Malhotra
,
R.
Pandey
,
K.
Yaddanapudi
,
P.
Nukala
,
B.
Dkhil
,
A.
Senyshyn
, and
R.
Ranjan
,
Nat. Mater.
17
(
5
),
427
(
2018
).
https://doi.org/10.1038/s41563-018-0060-2
Google Scholar
Crossref
Search ADS
PubMed
 
22.
F.
Li
,
L.
Jin
, and
R. P.
Guo
,
Appl. Phys. Lett.
105
(
23
),
232903
(
2014
).
https://doi.org/10.1063/1.4904019
Google Scholar
Crossref
Search ADS
 
23.
Y. F.
Chang
,
B.
Watson
,
M.
Fanton
,
R. J.
Meyer
, and
G. L.
Messing
,
Appl. Phys. Lett.
111
(
23
),
232901
(
2017
).
https://doi.org/10.1063/1.5006288
Google Scholar
Crossref
Search ADS
 
© 2024 Author(s). Published under an exclusive license by AIP Publishing.
2024
Author(s)
You do not currently have access to this content.