We demonstrate that a spintronic terahertz (THz) emitter can be driven by a chirped-pulse beating scheme to generate narrowband THz pulses, with continuous tuning of the frequency and linewidth by simply adjusting the laser chirp and/or the time delay between chirped pulses. As supported by model calculations, temporal shaping of the drive laser pulses can be exploited to manipulate the ultrafast demagnetization dynamics in the thin-film emitter, modulating the spin-polarized current in the ferromagnetic layer to access multi-cycle THz emission. Using a regenerative amplifier laser system with 50 fs transform-limited pulses chirped to 6 ps, we demonstrate narrowband THz generation over a frequency range from 0.4 to 2.3 THz, in addition to linewidths down to 40 GHz using 12 ps chirped pulses. Our proof-of-concept results pave the way to future narrowband THz sources with subgigahertz linewidth and center frequencies continuously tunable from 0.1 to 30 THz. By combining with the advantageous properties of spintronic THz emitters, from straightforward implementation to flexible polarization control, these sources open up opportunities for narrowband applications over the entire THz spectral range.
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20 November 2023
Research Article|
November 20 2023
Tunable multi-cycle terahertz pulse generation from a spintronic emitter
R. Ji
;
R. Ji
(Data curation, Formal analysis, Writing – original draft, Writing – review & editing)
1
Nano Engineering and Spintronic Technologies Group, Department of Computer Science, The University of Manchester
, Oxford Road, Manchester M13 9PL, United Kingdom
2
Department of Physics and Astronomy & Photon Science Institute, The University of Manchester
, Oxford Road, Manchester M13 9PL, United Kingdom
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M. T. Hibberd
;
M. T. Hibberd
(Conceptualization, Data curation, Writing – original draft, Writing – review & editing)
2
Department of Physics and Astronomy & Photon Science Institute, The University of Manchester
, Oxford Road, Manchester M13 9PL, United Kingdom
3
The Cockcroft Institute, Sci-Tech Daresbury
, Keckwick Lane, Daresbury, Warrington WA4 4AD, United Kingdom
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C.-H. Lin
;
C.-H. Lin
(Data curation, Writing – review & editing)
1
Nano Engineering and Spintronic Technologies Group, Department of Computer Science, The University of Manchester
, Oxford Road, Manchester M13 9PL, United Kingdom
2
Department of Physics and Astronomy & Photon Science Institute, The University of Manchester
, Oxford Road, Manchester M13 9PL, United Kingdom
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D. A. Walsh
;
D. A. Walsh
(Data curation, Writing – review & editing)
3
The Cockcroft Institute, Sci-Tech Daresbury
, Keckwick Lane, Daresbury, Warrington WA4 4AD, United Kingdom
4
Accelerator Science and Technology Centre, Science and Technology Facilities Council, Sci-Tech Daresbury
, Keckwick Lane, Daresbury, Warrington WA4 4AD, United Kingdom
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T. Thomson
;
T. Thomson
(Funding acquisition, Project administration, Supervision, Writing – review & editing)
1
Nano Engineering and Spintronic Technologies Group, Department of Computer Science, The University of Manchester
, Oxford Road, Manchester M13 9PL, United Kingdom
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P. W. Nutter
;
P. W. Nutter
(Funding acquisition, Project administration, Supervision, Writing – review & editing)
1
Nano Engineering and Spintronic Technologies Group, Department of Computer Science, The University of Manchester
, Oxford Road, Manchester M13 9PL, United Kingdom
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D. M. Graham
D. M. Graham
a)
(Conceptualization, Funding acquisition, Project administration, Supervision, Writing – original draft, Writing – review & editing)
2
Department of Physics and Astronomy & Photon Science Institute, The University of Manchester
, Oxford Road, Manchester M13 9PL, United Kingdom
3
The Cockcroft Institute, Sci-Tech Daresbury
, Keckwick Lane, Daresbury, Warrington WA4 4AD, United Kingdom
a)Author to whom correspondence should be addressed: [email protected]
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a)Author to whom correspondence should be addressed: [email protected]
Appl. Phys. Lett. 123, 212402 (2023)
Article history
Received:
September 12 2023
Accepted:
October 05 2023
Citation
R. Ji, M. T. Hibberd, C.-H. Lin, D. A. Walsh, T. Thomson, P. W. Nutter, D. M. Graham; Tunable multi-cycle terahertz pulse generation from a spintronic emitter. Appl. Phys. Lett. 20 November 2023; 123 (21): 212402. https://doi.org/10.1063/5.0176314
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