Single crystalline polar magnets (Mn1−xCox)2Mo3O8 (0 ≤ x ≤ 1) have been synthesized, and their magnetic properties have been studied. Magnetic interactions of the samples can be modulated drastically by Co-doping, and a ferrimagnetic to antiferromagnetic phase transition is identified at x = 0.35. For the samples hosting a ferrimagnetic state (0 ≤ x ≤ 0.3), square-like magnetic hysteresis loops are commonly identified, and the remnant magnetization and coercive field are revealed to strongly depend on the Co-content and temperature. The occupation ratio and magnetic nature of Co2+ are key ingredients to dictate the competition of various magnetic exchange couplings in the samples.
REFERENCES
1.
S.-W.
Cheong
,
D.
Talbayev
,
V.
Kiryukhin
, and
A.
Saxena
, npj Quantum Mater.
3
, 19
(2018
).2.
S.
Dong
,
H.
Xiang
, and
E.
Dagotto
, Natl. Sci. Rev.
6
, 629
–641
(2019
).3.
Y.
Wang
,
G. L.
Pascut
,
B.
Gao
,
T. A.
Tyson
,
K.
Haule
,
V.
Kiryukhin
, and
S. W.
Cheong
, Sci. Rep.
5
, 12268
(2015
).4.
T.
Kurumaji
,
S.
Ishiwata
, and
Y.
Tokura
, Phys. Rev. X
5
, 031034
(2015
).5.
W.
Wang
,
P. Z.
Li
,
Y. T.
Chang
,
M. F.
Liu
,
C. L.
Lu
,
X. B.
Lu
,
M.
Zeng
, and
J. M.
Liu
, Appl. Phys. Lett.
118
, 112901
(2021
).6.
Y. S.
Tang
,
J. H.
Zhang
,
L.
Lin
,
R.
Chen
,
J. F.
Wang
,
S. H.
Zheng
,
C.
Li
,
Y. Y.
Zhang
,
G. Z.
Zhou
,
L.
Huang
,
Z. B.
Yan
,
X. M.
Lu
,
D.
Wu
,
X. K.
Huang
,
X. P.
Jiang
, and
J. M.
Liu
, Phys. Rev. B
103
, 014112
(2021
).7.
Y. S.
Tang
,
S. M.
Wang
,
L.
Lin
,
C.
Li
,
S. H.
Zheng
,
C. F.
Li
,
J. H.
Zhang
,
Z. B.
Yan
,
X. P.
Jiang
, and
J. M.
Liu
, Phys. Rev. B
100
, 134112
(2019
).8.
S.
Yu
,
B.
Gao
,
J. W.
Kim
,
S. W.
Cheong
,
M. K. L.
Man
,
J.
Madeo
,
K. M.
Dani
, and
D.
Talbayev
, Phys. Rev. Lett.
120
, 037601
(2018
).9.
S.
Reschke
,
D. G.
Farkas
,
A.
Strinić
,
S.
Ghara
,
K.
Guratinder
,
O.
Zaharko
,
L.
Prodan
,
V.
Tsurkan
,
D.
Szaller
,
S.
Bordács
,
J.
Deisenhofer
, and
I.
Kézsmárki
, npj Quantum Mater.
7
, 1
(2022
).10.
T.
Kurumaji
,
Y.
Takahashi
,
J.
Fujioka
,
R.
Masuda
,
H.
Shishikura
,
S.
Ishiwata
, and
Y.
Tokura
, Phys. Rev. B
95
, 020405
(2017
).11.
Y. M.
Sheu
,
Y. M.
Chang
,
C. P.
Chang
,
Y. H.
Li
,
K. R.
Babu
,
G. Y.
Guo
,
T.
Kurumaji
, and
Y.
Tokura
, Phys. Rev. X
9
, 031038
(2019
).12.
T.
Ideue
,
T.
Kurumaji
,
S.
Ishiwata
, and
Y.
Tokura
, Nat. Mater.
16
, 797
–802
(2017
).13.
Y. S.
Tang
,
G. Z.
Zhou
,
L.
Lin
,
R.
Chen
,
J. F.
Wang
,
C. L.
Lu
,
L.
Huang
,
J. H.
Zhang
,
Z. B.
Yan
,
X. M.
Lu
,
X. K.
Huang
,
X. P.
Jiang
, and
J. M.
Liu
, Phys. Rev. B
105
, 064108
(2022
).14.
J.
Yang
,
D.
Su
,
J.
He
,
Y.
Ji
,
Q.
Guo
,
Y.
Meng
,
X.
Li
,
L.
Wang
,
X.
Shen
,
Y.
Yao
,
Y.
Long
,
Y.
Sun
, and
R.
Yu
, Phys. Rev. B
107
, 104408
(2023
).15.
D.
Bertrand
and
H.
Kerner-Czeskleba
, J. Phys. France.
36
, 379
–390
(1975
).16.
K.
Park
,
G. L.
Pascut
,
G.
Khanal
,
M. O.
Yokosuk
,
X.
Xu
,
B.
Gao
,
M. J.
Gutmann
,
A. P.
Litvinchuk
,
V.
Kiryukhin
,
S. W.
Cheong
,
D.
Vanderbilt
,
K.
Haule
, and
J. L.
Musfeldt
, Phys. Rev. B
104
, 195143
(2021
).17.
S.
Reschke
,
A. A.
Tsirlin
,
N.
Khan
,
L.
Prodan
,
V.
Tsurkan
,
I.
Kézsmárki
, and
J.
Deisenhofer
, Phys. Rev. B
102
, 094307
(2020
).18.
F.
Varret
,
H.
Czeskleba
,
F.
Hartmann-Boutron
, and
P.
Imbert
, J. Phys.
33
, 549
–564
(1972
).19.
L.
Prodan
,
I.
Filippova
,
A. O.
Zubtsovskii
,
S.
Shova
,
S.
Widmann
,
A. A.
Tsirlin
,
I.
Kézsmárki
, and
V.
Tsurkan
, Phys. Rev. B
106
, 174421
(2022
).20.
T.
Kurumaji
,
S.
Ishiwata
, and
Y.
Tokura
, Phys. Rev. B
95
, 045142
(2017
).21.
Y.
Chang
,
L.
Gao
,
Y.
Xie
,
B.
You
,
Y.
Liu
,
R.
Xiong
,
J.
Wang
,
C.
Lu
, and
J. M.
Liu
, ACS Appl. Mater. Interfaces
15
, 22204
–22211
(2023
).22.
P.
Strobel
and
Y.
Le Page
, J Cryst. Growth
61
, 329
–338
(1983
).23.
P.
Strobel
,
Y.
Le Page
, and
S. P.
Mcalister
, J Solid State Chem.
42
, 242
–250
(1982
).24.
A. K.
Nayak
,
M.
Nicklas
,
S.
Chadov
,
P.
Khuntia
,
C.
Shekhar
,
A.
Kalache
,
M.
Baenitz
,
Y.
Skourski
,
V. K.
Guduru
,
A.
Puri
,
U.
Zeitler
,
J. M.
Coey
, and
C.
Felser
, Nat. Mater.
14
, 679
–684
(2015
).25.
A.
Kumar
and
S. M.
Yusuf
, Phys. Rep.
556
, 1
–34
(2015
).© 2023 Author(s). Published under an exclusive license by AIP Publishing.
2023
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