Nanoscale engineered materials combined with wearable wireless technologies can deliver a new level of health monitoring. A reduced graphene oxide-nylon composite material is developed and tested, demonstrating its usefulness as a material for sensors in wearable, long-term electrocardiogram (ECG) monitoring via a comparison to one of the widely used ECG sensors. The structural analysis by scanning electron microscopy and atomic force microscopy shows a limited number of defects on a macroscopic scale. Fourier transform infrared and Raman spectroscopy confirm the presence of rGOx, and the ratio of D- and G-features as a function of thickness correlates with the resistivity analysis. The negligible effect of the defects and the tunability of electrical and optical properties, together with live ECG data, demonstrate its signal transduction capability. Other potential electronic and optical sensor uses beyond ECG are possible, given the controllable nature of the heterostructures and the correlation of transport and optical properties.
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2 January 2023
Research Article|
January 03 2023
Layered, tunable graphene oxide-nylon composite heterostructures for wearable electrocardiogram sensors
N. G. Hallfors
;
N. G. Hallfors
(Data curation, Investigation, Methodology, Validation, Writing – original draft)
1
Khalifa University
, Abu Dhabi 127788, United Arab Emirates
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D. Maksimovski;
D. Maksimovski
(Data curation, Formal analysis, Validation, Writing – original draft)
2
Colgate University
, Hamilton, New York 13346, USA
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I. A. H. Farhat
;
I. A. H. Farhat
(Data curation, Investigation, Resources, Validation, Visualization)
3
University of Waterloo
, Waterloo, Ontario N2L 3G1, Canada
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M. Abi Jaoude
;
M. Abi Jaoude
(Investigation, Methodology, Validation, Visualization, Writing – original draft, Writing – review & editing)
1
Khalifa University
, Abu Dhabi 127788, United Arab Emirates
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A. R. Devarajan
;
A. R. Devarajan
(Data curation, Investigation, Methodology, Validation, Writing – original draft)
1
Khalifa University
, Abu Dhabi 127788, United Arab Emirates
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K. Liao
;
K. Liao
(Conceptualization, Funding acquisition, Resources, Validation, Writing – original draft)
1
Khalifa University
, Abu Dhabi 127788, United Arab Emirates
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M. Ismail
;
M. Ismail
(Funding acquisition, Methodology, Project administration, Supervision)
4
Wayne State University
, Detroit, Michigan 48202, USA
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H. Pade
;
H. Pade
(Data curation, Investigation, Visualization)
2
Colgate University
, Hamilton, New York 13346, USA
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R. Y. Adhikari
;
R. Y. Adhikari
(Investigation, Methodology, Writing – review & editing)
2
Colgate University
, Hamilton, New York 13346, USA
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A. F. Isakovic
A. F. Isakovic
a)
(Conceptualization, Formal analysis, Investigation, Methodology, Project administration, Resources, Supervision, Visualization, Writing – original draft, Writing – review & editing)
2
Colgate University
, Hamilton, New York 13346, USA
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Appl. Phys. Lett. 122, 013701 (2023)
Article history
Received:
August 15 2022
Accepted:
December 16 2022
Citation
N. G. Hallfors, D. Maksimovski, I. A. H. Farhat, M. Abi Jaoude, A. R. Devarajan, K. Liao, M. Ismail, H. Pade, R. Y. Adhikari, A. F. Isakovic; Layered, tunable graphene oxide-nylon composite heterostructures for wearable electrocardiogram sensors. Appl. Phys. Lett. 2 January 2023; 122 (1): 013701. https://doi.org/10.1063/5.0120774
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