Core/shell CdSe/CdZnS nanoplatelets (NPLs) are a promising class of nanomaterials for lasing applications owing to their low thresholds and high stability of stimulated emission generation as compared with many other types of colloids. Moreover, they can be self-assembled into high-quality thin films by simple methods of deposition. However, the high throughput and reproducible methods for nanopatterning of such films for advanced light-emitting applications are still missing. In this work, we show direct laser writing on thin films assembled from CdSe/CdZnS NPLs using either spin-coating or the self-assembly method for the purpose of fabricating. Using theoretical calculations, we design the period of the structures to achieve high quality-factor optical modes in the emission band of NPLs. In these nanostructured NPL films, fabricated according to the design, we observe photoluminescence enhancement and directional outcoupling effects. The proposed approach holds great potential for LEDs with improved outcoupling and for distributed feedback lasers or lasers based on bound states in the continuum with directly written optical cavities.
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28 November 2022
Research Article|
November 28 2022
Direct laser writing of resonant periodic nanostructures in thin light-emitting films of CdSe/CdZnS core/shell nanoplatelets
Ruslan Azizov
;
Ruslan Azizov
a)
(Formal analysis, Investigation, Visualization, Writing – original draft)
1
School of Physics and Engineering, ITMO University
, 197101 St Petersburg, Russia
a)Authors to whom correspondence should be addressed: ruslan.azizov@metalab.ifmo.ru and s.makarov@metalab.ifmo.ru
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Ivan Sinev
;
Ivan Sinev
(Conceptualization, Investigation, Writing – review & editing)
1
School of Physics and Engineering, ITMO University
, 197101 St Petersburg, Russia
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Furkan Işık
;
Furkan Işık
(Investigation)
2
Department of Electrical and Electronics Engineering and Department of Physics, UNAM—Institute of Materials Science and Nanotechnology, Bilkent University
, Ankara 06800, Turkey
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Farzan Shabani
;
Farzan Shabani
(Investigation)
2
Department of Electrical and Electronics Engineering and Department of Physics, UNAM—Institute of Materials Science and Nanotechnology, Bilkent University
, Ankara 06800, Turkey
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Anatoly Pushkarev
;
Anatoly Pushkarev
(Investigation)
1
School of Physics and Engineering, ITMO University
, 197101 St Petersburg, Russia
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Iklim Yurdakul
;
Iklim Yurdakul
(Investigation)
2
Department of Electrical and Electronics Engineering and Department of Physics, UNAM—Institute of Materials Science and Nanotechnology, Bilkent University
, Ankara 06800, Turkey
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Savas Delikanli
;
Savas Delikanli
(Investigation)
2
Department of Electrical and Electronics Engineering and Department of Physics, UNAM—Institute of Materials Science and Nanotechnology, Bilkent University
, Ankara 06800, Turkey
3
Luminous! Center of Excellence for Semiconductor Lighting and Displays, School of Electrical and Electronic Engineering, School of Physical and Mathematical Sciences, School of Materials Science and Engineering, Nanyang Technological University
, Nanyang Avenue, Singapore 639798, Singapore
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Hilmi Volkan Demir
;
Hilmi Volkan Demir
(Conceptualization, Supervision, Writing – review & editing)
2
Department of Electrical and Electronics Engineering and Department of Physics, UNAM—Institute of Materials Science and Nanotechnology, Bilkent University
, Ankara 06800, Turkey
3
Luminous! Center of Excellence for Semiconductor Lighting and Displays, School of Electrical and Electronic Engineering, School of Physical and Mathematical Sciences, School of Materials Science and Engineering, Nanyang Technological University
, Nanyang Avenue, Singapore 639798, Singapore
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Sergey Makarov
Sergey Makarov
a)
(Conceptualization, Supervision, Writing – review & editing)
4
Qingdao Innovation and Development Center, Harbin Engineering University
, 266000 Qingdao, China
a)Authors to whom correspondence should be addressed: ruslan.azizov@metalab.ifmo.ru and s.makarov@metalab.ifmo.ru
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a)Authors to whom correspondence should be addressed: ruslan.azizov@metalab.ifmo.ru and s.makarov@metalab.ifmo.ru
Appl. Phys. Lett. 121, 223301 (2022)
Article history
Received:
June 30 2022
Accepted:
November 10 2022
Citation
Ruslan Azizov, Ivan Sinev, Furkan Işık, Farzan Shabani, Anatoly Pushkarev, Iklim Yurdakul, Savas Delikanli, Hilmi Volkan Demir, Sergey Makarov; Direct laser writing of resonant periodic nanostructures in thin light-emitting films of CdSe/CdZnS core/shell nanoplatelets. Appl. Phys. Lett. 28 November 2022; 121 (22): 223301. https://doi.org/10.1063/5.0106895
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