For a biased trap-filled insulator, the current transport is governed by the physics of charge injection from the metallic electrode and also the trap-limited space-charge conduction in the insulator. With a Schottky barrier at the interface of the metal-insulator junction, charge tunneling injection from a metal into the trap-filled insulator is different from an Ohmic contact. At sufficiently large amount of charge injection at high voltages, the charge transport becomes the trap-limited space-charge conduction. In this paper, we develop a consistent model to calculate the correct IV characteristics up to a breakdown field strength of 1 V/nm. Using this model, we analyze the transport characteristic of three different metal-insulator junctions (ITO/PPV, Al/h-BN, and Al/ZrO2) and identify the conduction mechanisms over a wide range of the applied voltage, insulator's thickness, and properties of the traps. Our findings report the interplay between various transport mechanisms, which is useful to characterize the correct current transport for novel insulators such as organic semiconductors, 2D insulators, and metal-oxide electronics.
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7 November 2022
Research Article|
November 08 2022
Tunneling injection to trap-limited space-charge conduction for metal-insulator junction
Special Collection:
Metal Oxide Thin-Film Electronics
Cherq Chua
;
Cherq Chua
(Investigation, Methodology, Writing – original draft)
Science, Mathematics and Technology (SMT), Singapore University of Technology and Design
, Singapore
487372
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Yee Sin Ang
;
Yee Sin Ang
a)
(Methodology, Supervision, Writing – review & editing)
Science, Mathematics and Technology (SMT), Singapore University of Technology and Design
, Singapore
487372a)Authors to whom correspondence should be addressed: yeesin_ang@sutd.edu.sg and ricky_ang@sutd.edu.sg
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Lay Kee Ang
Lay Kee Ang
a)
(Conceptualization, Supervision, Writing – review & editing)
Science, Mathematics and Technology (SMT), Singapore University of Technology and Design
, Singapore
487372a)Authors to whom correspondence should be addressed: yeesin_ang@sutd.edu.sg and ricky_ang@sutd.edu.sg
Search for other works by this author on:
a)Authors to whom correspondence should be addressed: yeesin_ang@sutd.edu.sg and ricky_ang@sutd.edu.sg
Note: This paper is part of the APL Special Collection on Metal Oxide Thin-Film Electronics.
Appl. Phys. Lett. 121, 192109 (2022)
Article history
Received:
September 08 2022
Accepted:
October 23 2022
Citation
Cherq Chua, Yee Sin Ang, Lay Kee Ang; Tunneling injection to trap-limited space-charge conduction for metal-insulator junction. Appl. Phys. Lett. 7 November 2022; 121 (19): 192109. https://doi.org/10.1063/5.0124748
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