We studied the formation and attenuation of GHz elastic waves in free-standing nanoporous gold films by MeV ultrafast electron diffraction and finite element simulations. By tracing the evolution of the high frequency acoustic waves in time domain, we found that the bicontinuous nanoporous structure in nanoporous gold films results in three-dimensionally acoustic response with low coherence, leading to fast attenuation of the elastic waves in comparison with solid gold films. The morphologically dominated dynamics indicates the nanoporosity plays an important role in the high-frequency acoustic energy relaxation, which shines a light on the applications of dealloyed nanoporous materials in nanodevices and sensors as GHz and THz acoustic filters and dampers.

1.
H. J.
Mamin
and
D.
Rugar
,
Appl. Phys. Lett.
79
,
3358
(
2001
).
2.
J.
Chaste
,
A.
Eichler
,
J.
Moser
 et al.,
Nat. Nanotechnol.
7
,
301
(
2012
).
3.
K.
Jensen
,
K.
Kim
, and
A.
Zettl
,
Nat. Nanotechnol.
3
,
533
(
2008
).
4.
C.
Thomsen
,
H. T.
Grahn
,
H. J.
Maris
, and
J.
Tauc
,
Phys. Rev. B
34
,
4129
(
1986
).
5.
C.
Thomsen
,
J.
Strait
,
Z.
Vardeny
 et al.,
Phys. Rev. Lett.
53
,
989
(
1984
).
6.
M.
Hu
,
X.
Wang
,
G. V.
Hartland
 et al.,
J. Am. Chem. Soc.
125
,
14925
(
2003
).
7.
P.
Zijlstra
,
A. L.
Tchebotareva
,
J. W. M.
Chon
,
M.
Gu
, and
M.
Orrit
,
Nano Lett.
8
,
3493
(
2008
).
8.
P. V.
Ruijgrok
,
P.
Zijlstra
,
A. L.
Tchebotareva
, and
M.
Orrit
,
Nano Lett.
12
,
1063
(
2012
).
9.
M.
Nisoli
,
S.
De Silvestri
,
A.
Cavalleri
 et al.,
Phys. Rev. B
55
,
R13424
(
1997
).
10.
11.
A.
Crut
,
P.
Maioli
,
N. D.
Fatti
, and
F.
Vallée
,
Phys. Rep.
549
,
1
(
2015
).
12.
M.
Nicoul
,
U.
Shymanovich
,
A.
Tarasevitch
,
D.
von der Linde
, and
K.
Sokolowski-Tinten
,
Appl. Phys. Lett.
98
,
191902
(
2011
).
13.
S.
Nie
,
X.
Wang
,
H.
Park
,
R.
Clinite
, and
J.
Cao
,
Phys. Rev. Lett.
96
,
025901
(
2006
).
14.
X.
Wang
,
S.
Nie
,
J.
Li
 et al.,
Appl. Phys. Lett.
92
,
121918
(
2008
).
15.
T.
Henighan
,
M.
Trigo
,
S.
Bonetti
 et al.,
Phys. Rev. B
93
,
220301
(
2016
).
16.
A. E. H.
Love
,
A Treatise on the Mathematical Theory of Elasticity
(
Cambridge University Press
,
1892
).
17.
C.
Prada
,
O.
Balogun
, and
T. W.
Murray
,
Appl. Phys. Lett.
87
,
194109
(
2005
).
18.
L. L.
Beranek
,
J. Acoust. Soc. Am.
13
,
248
(
1942
).
19.
N.
Lopez-Abdala
,
M.
Esmann
,
M. C.
Fuertes
 et al.,
J. Phys. Chem. C
124
,
17165
(
2020
).
20.
T.
Fujita
,
L. H.
Qian
,
K.
Inoke
,
J.
Erlebacher
, and
M. W.
Chen
,
Appl. Phys. Lett.
92
,
251902
(
2008
).
21.
S. P.
Weathersby
,
G.
Brown
,
M.
Centurion
 et al.,
Rev. Sci. Instrum.
86
,
073702
(
2015
).
22.
Q.
Zheng
,
X.
Shen
,
K.
Sokolowski-Tinten
 et al.,
J. Phys. Chem. C
122
,
16368
(
2018
).
23.
J.
Hohlfeld
,
S.-S.
Wellershoff
,
J.
Güdde
 et al.,
Chem. Phys.
251
,
237
(
2000
).
24.
B. O.
Wright
,
Phys. Rev. B
49
,
9985
(
1994
).
25.
S.
Nie
,
X.
Wang
,
J.
Li
,
R.
Clinite
, and
J.
Cao
,
Microsc. Res. Tech.
72
,
131
(
2009
).
26.
K.
Sokolowski-Tinten
,
X.
Shen
,
Q.
Zheng
 et al.,
Struct. Dyn.
4
,
054501
(
2017
).
27.
K. O.
Mclean
,
C. A.
Swenson
, and
C. R.
Case
,
J. Low Temp. Phys.
7
,
77
(
1972
).
28.
K. A.
Gschneidner
, Jr.
,
Solid State Phys.
16
,
275
(
1964
).
29.
A.
Cavalleri
,
C. W.
Siders
,
F. L. H.
Brown
 et al.,
Phys. Rev. Lett.
85
,
586
(
2000
).
30.
L.
Qian
and
M.
Chen
,
Appl. Phys. Lett.
91
,
083105
(
2007
).

Supplementary Material

You do not currently have access to this content.