We demonstrate nondegenerate photon pair generation by spontaneous parametric downconversion in a silver gallium sulfide AgGaS2 crystal. By tuning the pump wavelength, we achieve phase matching over a large spectral range. This allows to generate idler photons in the mid-infrared spectral range above a 6 μm wavelength with corresponding signal photons in the visible. Also, we show photon pair generation with broad spectral bandwidth. These results are a valuable step toward the development of quantum imaging and sensing techniques in the mid-infrared.
References
1.
M. G.
Basset
, F.
Setzpfandt
, F.
Steinlechner
, E.
Beckert
, T.
Pertsch
, and M.
Gräfe
, “Perspectives for applications of quantum imaging
,” Laser Photonics Rev.
13
, 1900097
(2019
).2.
S.
Mukamel
, M.
Freyberger
, W.
Schleich
, M.
Bellini
, A.
Zavatta
, G.
Leuchs
, C.
Silberhorn
, R. W.
Boyd
, L. L.
Sánchez-Soto
, A.
Stefanov
, M.
Barbieri
, A.
Paterova
, L.
Krivitsky
, S.
Shwartz
, K.
Tamasaku
, K.
Dorfman
, F.
Schlawin
, V.
Sandoghdar
, M.
Raymer
, A.
Marcus
, O.
Varnavski
, T.
Goodson
, Z.-Y.
Zhou
, B.-S.
Shi
, S.
Asban
, M.
Scully
, G.
Agarwal
, T.
Peng
, A. V.
Sokolov
, Z.-D.
Zhang
, M. S.
Zubairy
, I. A.
Vartanyants
, E.
del Valle
, and F.
Laussy
, “Roadmap on quantum light spectroscopy
,” J. Phys. B
53
, 072002
(2020
).3.
G. B.
Lemos
, V.
Borish
, G. D.
Cole
, S.
Ramelow
, R.
Lapkiewicz
, and A.
Zeilinger
, “Quantum imaging with undetected photons
,” Nature
512
, 409
–412
(2014
).4.
D. A.
Kalashnikov
, A. V.
Paterova
, S. P.
Kulik
, and L. A.
Krivitsky
, “Infrared spectroscopy with visible light
,” Nat. Photonics
10
, 98
–101
(2016
).5.
M. V.
Chekhova
and Z. Y.
Ou
, “Nonlinear interferometers in quantum optics
,” Adv. Opt. Photonics
8
, 104
(2016
).6.
I.
Kviatkovsky
, H. M.
Chrzanowski
, E. G.
Avery
, H.
Bartolomaeus
, and S.
Ramelow
, “Microscopy with undetected photons in the mid-infrared
,” Sci. Adv.
6
, eabd0264
(2020
).7.
C.
Lindner
, S.
Wolf
, J.
Kiessling
, and F.
Kühnemann
, “Fourier transform infrared spectroscopy with visible light
,” Opt. Express
28
, 4426
(2020
).8.
C.
Lindner
, J.
Kunz
, S. J.
Herr
, S.
Wolf
, J.
Kießling
, and F.
Kühnemann
, “Nonlinear interferometer for Fourier-transform mid-infrared gas spectroscopy using near-infrared detection
,” Opt. Express
29
, 4035
(2021
).9.
A. V.
Paterova
, H.
Yang
, C.
An
, D. A.
Kalashnikov
, and L. A.
Krivitsky
, “Tunable optical coherence tomography in the infrared range using visible photons
,” Quantum Sci. Technol.
3
, 025008
(2018
).10.
A.
Yabushita
and T.
Kobayashi
, “Spectroscopy by frequency-entangled photon pairs
,” Phys. Rev. A
69
, 013806
(2004
).11.
D. A.
Kalashnikov
, Z.
Pan
, A. I.
Kuznetsov
, and L. A.
Krivitsky
, “Quantum spectroscopy of plasmonic nanostructures
,” Phys. Rev. X
4
, 011049
(2014
).12.
G. K.
Kitaeva
, S. P.
Kovalev
, A. N.
Penin
, A. N.
Tuchak
, and P. V.
Yakunin
, “A method of calibration of terahertz wave brightness under nonlinear-optical detection
,” J. Infrared, Millimeter, Terahertz Waves
32
, 1144
–1156
(2011
).13.
M.
Kutas
, B.
Haase
, P.
Bickert
, F.
Riexinger
, D.
Molter
, and G.
von Freymann
, “Terahertz quantum sensing
,” Sci. Adv.
6
, eaaz8065
(2020
).14.
R. A.
McCracken
, F.
Graffitti
, and A.
Fedrizzi
, “Numerical investigation of mid-infrared single-photon generation
,” J. Opt. Soc. Am. B
35
, C38
(2018
).15.
L.
Maidment
, O.
Kara
, P. G.
Schunemann
, J.
Piper
, K.
McEwan
, and D. T.
Reid
, “Long-wave infrared generation from femtosecond and picosecond optical parametric oscillators based on orientation-patterned gallium phosphide
,” Appl. Phys. B
124
, 143
(2018
).16.
L. I.
Isaenko
and A. P.
Yelisseyev
, “Recent studies of nonlinear chalcogenide crystals for the mid-IR
,” Semicond. Sci. Technol.
31
, 123001
(2016
).17.
D. N.
Nikogosyan
, Nonlinear Optical Crystals: A Complete Survey
(Springer-Verlag
, 2005
).18.
R.
Boyd
and A.
Stentz
, “Nonlinear optics
,” in The Handbook of Photonics
, 2nd ed. (CRC Press
, 2006
).19.
G.
Boyd
, H.
Kasper
, and J.
McFee
, “Linear and nonlinear optical properties of AgGaS2, CuGaS2, and CuInS2, and theory of the wedge technique for the measurement of nonlinear coefficients
,” IEEE J. Quantum Electron.
7
, 563
–573
(1971
).20.
D. S.
Simon
, G.
Jaeger
, and A. V.
Sergienko
, Quantum Metrology, Imaging, and Communication
(Springer International Publishing
, 2017
).21.
Y.
Shih
, “Entangled biphoton source-property and preparation
,” Rep. Prog. Phys.
66
, 1009
–1044
(2003
).22.
E.
Takaoka
and K.
Kato
, “Thermo-optic dispersion formula for AgGaS2
,” Appl. Opt.
38
, 4577
(1999
).23.
R. S.
Bennink
, “Optimal collinear Gaussian beams for spontaneous parametric down-conversion
,” Phys. Rev. A
81
, 053805
(2010
).24.
A.
Yodh
, H.
Tom
, G.
Aumiller
, and R. S.
Miranda
, “Generation of tunable mid-infrared picosecond pulses at 76 MHz
,” J. Opt. Soc. Am. B
8
, 1663
–1667
(1991
).25.
P.
Canarelli
, Z.
Benko
, A.
Hielscher
, R.
Curl
, and F.
Tittel
, “Measurement of nonlinear coefficient and phase matching characteristics of AgGaS/sub 2
/,” IEEE J. Quantum Electron.
28
, 52
–55
(1992
).26.
E.
Bocquillon
, C.
Couteau
, M.
Razavi
, R.
Laflamme
, and G.
Weihs
, “Coherence measures for heralded single-photon sources
,” Phys. Rev. A
79
, 035801
(2009
).27.
S.
Bettelli
, “Comment on ‘Coherence measures for heralded single-photon sources
,’” Phys. Rev. A
81
, 037801
(2010
).28.
D.
Höckel
, L.
Koch
, and O.
Benson
, “Direct measurement of heralded single-photon statistics from a parametric down-conversion source
,” Phys. Rev. A
83
, 013802
(2011
).29.
Q.
Chen
, R.
Ge
, L.
Zhang
, F.
Li
, B.
Zhang
, Y.
Dai
, Y.
Fei
, X.
Wang
, X.
Jia
, Q.
Zhao
et al., “Mid-infrared single photon detector with superconductor Mo80Si20 nanowire
,” arXiv:2011.06699 (2020
).30.
V.
Verma
, B.
Korzh
, A.
Walter
, A.
Lita
, R.
Briggs
, M.
Colangelo
, Y.
Zhai
, E.
Wollman
, A.
Beyer
, J.
Allmaras
et al., “Single-photon detection in the mid-infrared up to 10 μm wavelength using tungsten silicide superconducting nanowire detectors
,” APL Photonics
6
, 056101
(2021
).31.
M.
Arahata
, Y.
Mukai
, B.
Cao
, T.
Tashima
, R.
Okamoto
, and S.
Takeuchi
, “Wavelength variable generation and detection of photon pairs in visible and mid-infrared regions via spontaneous parametric downconversion
,” J. Opt. Soc. Am. B
38
, 1934
–1941
(2021
).© 2021 Author(s). Published under an exclusive license by AIP Publishing.
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