Hyperbolic metamaterials are a family of nanophotonic architectures allowing for the unique control of photonic local density of states. Such a property makes metamaterials prospective to use them with light-emitting objects or to apply as meta-electrodes for optoelectronic devices, where the control of recombination properties plays a decisive role. On the other hand, layered quasi-2D halide perovskites (Ruddlesden–Popper phase) attract high attention due to their low cost, broadband spectral tunability, and outstanding optoelectronic properties. Here, we show how to accelerate photoluminescence with smart engineering of photonic density of states (i.e., via the Purcell effect) by depositing a perovskite film on a hyperbolic metamaterial. We experimentally confirm acceleration of radiative recombination by almost 3 times. This effect can be useful in light-emitting devices, where interplay between radiative and non-radiative channels of charge carrier recombination is crucial.
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1 March 2021
Research Article|
March 02 2021
Acceleration of radiative recombination in quasi-2D perovskite films on hyperbolic metamaterials
Special Collection:
Metastructures: From Physics to Application
Pavel Tonkaev
;
Pavel Tonkaev
a)
1
Department of Physics and Engineering, ITMO University
, 49 Kronverksky Pr., St. Petersburg, 197101, Russia
a)Author to whom correspondence should be addressed: [email protected]
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Sergey Anoshkin
;
Sergey Anoshkin
1
Department of Physics and Engineering, ITMO University
, 49 Kronverksky Pr., St. Petersburg, 197101, Russia
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Anatoly Pushkarev
;
Anatoly Pushkarev
1
Department of Physics and Engineering, ITMO University
, 49 Kronverksky Pr., St. Petersburg, 197101, Russia
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Radu Malureanu
;
Radu Malureanu
2
Department of Photonics Engineering, Technical University of Denmark
, Ørsteds Plads, Building 345A, DK-2800 Kongens Lyngby, Denmark
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Mikhail Masharin
;
Mikhail Masharin
1
Department of Physics and Engineering, ITMO University
, 49 Kronverksky Pr., St. Petersburg, 197101, Russia
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Pavel Belov
;
Pavel Belov
1
Department of Physics and Engineering, ITMO University
, 49 Kronverksky Pr., St. Petersburg, 197101, Russia
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Andrei Lavrinenko
;
Andrei Lavrinenko
2
Department of Photonics Engineering, Technical University of Denmark
, Ørsteds Plads, Building 345A, DK-2800 Kongens Lyngby, Denmark
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Sergey Makarov
Sergey Makarov
1
Department of Physics and Engineering, ITMO University
, 49 Kronverksky Pr., St. Petersburg, 197101, Russia
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a)Author to whom correspondence should be addressed: [email protected]
Note: This Paper is part of the APL Special Collection on Metastructures: From Physics to Applications.
Appl. Phys. Lett. 118, 091104 (2021)
Article history
Received:
December 31 2020
Accepted:
February 15 2021
Citation
Pavel Tonkaev, Sergey Anoshkin, Anatoly Pushkarev, Radu Malureanu, Mikhail Masharin, Pavel Belov, Andrei Lavrinenko, Sergey Makarov; Acceleration of radiative recombination in quasi-2D perovskite films on hyperbolic metamaterials. Appl. Phys. Lett. 1 March 2021; 118 (9): 091104. https://doi.org/10.1063/5.0042557
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