Ptychography is a high-resolution imaging technique, which does not require lenses for image magnification and which provides phase contrast with high sensitivity. Here, we propose to use x-ray ptychography for the imaging of surface structure in crystalline samples. We show that ptychography can be used to image atomic step structures using coherent diffraction patterns recorded along the crystal truncation rod of a crystal surface. In a proof-of-concept experiment on a Pt (111) sample, we present ptychographic reconstructions showing features consistent with surface steps. Due to the penetration power of x-rays, this method could find interesting applications for the study of surface structures under buried interfaces or in harsh environments.
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9 March 2015
Research Article|
March 12 2015
Ptychographic x-ray imaging of surfaces on crystal truncation rod
Chenhui Zhu;
Chenhui Zhu
a)
1Materials Science Division,
Argonne National Laboratory
, Argonne, Illinois 60439, USA
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Ross Harder;
Ross Harder
2Advanced Photon Source,
Argonne National Laboratory
, Argonne, Illinois 60439, USA
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Ana Diaz;
Ana Diaz
3
Paul Scherrer Institut
, Villigen PSI 5232, Switzerland
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Vladimir Komanicky;
Vladimir Komanicky
4Faculty of Sciences,
Safarik University
, Kosice 04154, Slovakia
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Andi Barbour;
Andi Barbour
1Materials Science Division,
Argonne National Laboratory
, Argonne, Illinois 60439, USA
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Ruqing Xu;
Ruqing Xu
2Advanced Photon Source,
Argonne National Laboratory
, Argonne, Illinois 60439, USA
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Xiaojing Huang;
Xiaojing Huang
5National Synchrotron Light Source II,
Brookhaven National Laboratory
, Upton, New York 11973, USA
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Yaohua Liu
;
Yaohua Liu
1Materials Science Division,
Argonne National Laboratory
, Argonne, Illinois 60439, USA
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Michael S. Pierce;
Michael S. Pierce
6School of Physics and Astronomy,
Rochester Institute of Technology
, Rochester, New York 14623, USA
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Andreas Menzel;
Andreas Menzel
3
Paul Scherrer Institut
, Villigen PSI 5232, Switzerland
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Hoydoo You
Hoydoo You
b)
1Materials Science Division,
Argonne National Laboratory
, Argonne, Illinois 60439, USA
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a)
Present address: Advanced Light Source, Lawrence Berkeley National Lab, 1 Cyclotron Road, Berkeley, California 94720, USA.
b)
Email: [email protected]
Appl. Phys. Lett. 106, 101604 (2015)
Article history
Received:
July 15 2014
Accepted:
February 22 2015
Citation
Chenhui Zhu, Ross Harder, Ana Diaz, Vladimir Komanicky, Andi Barbour, Ruqing Xu, Xiaojing Huang, Yaohua Liu, Michael S. Pierce, Andreas Menzel, Hoydoo You; Ptychographic x-ray imaging of surfaces on crystal truncation rod. Appl. Phys. Lett. 9 March 2015; 106 (10): 101604. https://doi.org/10.1063/1.4914927
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